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Rapid formation of methane hydrate in environment-friendly leucine-based complex systems

Author

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  • Qin, Yue
  • Shang, Liyan
  • Lv, Zhenbo
  • Liu, Zhiming
  • He, Jianyu
  • Li, Xu
  • Binama, Maxime
  • Yang, Lingyun
  • Wang, Deyang

Abstract

Given the growing demand for natural gas (NG) in energy supply systems worldwide, solidified natural gas (SNG) is viewed as a potential NG storage and transportation method owing to its numerous advantages. However, using significant amounts of sodium dodecyl sulfate (SDS) to improve its slow formation kinetics has a negative influence on the environment, and severe foaming hinders the system's recovery. To overcome the associated issues, the main promoter has been chosen to be the ecologically safe and non-foaming L-leucine, with low concentrations of SDS and NaCl, as well as glass beads of various particle sizes, added to achieve synergistic effects. The hydrophobic micro-regions created by the leucine molecules, as well as the porous hydrate characteristics, considerably enhanced hydrate formation in the leucine-based complex system. At the effective promotion concentration, the SDS dosage is reduced by 60–90%. Owing to their strong promotion effect and non-foaming feature, yielding almost non-toxic properties, the LS1 and LN4 systems may be employed commercially. With a target of advancing SNG technology, this study serves as a reference for future developments of SNG technology based on the idea of environmental friendliness.

Suggested Citation

  • Qin, Yue & Shang, Liyan & Lv, Zhenbo & Liu, Zhiming & He, Jianyu & Li, Xu & Binama, Maxime & Yang, Lingyun & Wang, Deyang, 2022. "Rapid formation of methane hydrate in environment-friendly leucine-based complex systems," Energy, Elsevier, vol. 254(PA).
    • Handle: RePEc:eee:energy:v:254:y:2022:i:pa:s0360544222011173
    DOI: 10.1016/j.energy.2022.124214
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    2. Zhou, Shi-Dong & Xiao, Yan-Yun & Ni, Xing-Ya & Li, Xiao-Yan & Wu, Zhi-Min & Liu, Yang & Lv, Xiao-Fang, 2024. "Kinetics studies of CO2 hydrate formation in the presence of l-methionine coupled with multi-walled carbon nanotubes," Energy, Elsevier, vol. 298(C).

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