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Life cycle assessment of the Fischer-Tropsch biofuels production by supercritical water reforming of the bio-oil aqueous phase

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  • Gutiérrez Ortiz, F.J.
  • Alonso-Fariñas, B.
  • Campanario, F.J.
  • Kruse, A.

Abstract

This paper is aimed at performing an environmental evaluation regarding biofuel production. The process combines four sections: biomass fast pyrolysis to bio-oil with two phases, oil-phase upgrading by hydrotreating, using H2 obtained by steam reforming, and a new process to produce Fischer-Tropsch biofuels from supercritical water reforming of the aqueous phase. This phase can be valorised in the latter process entirely so natural gas is reformed to H2 (case-study 1), or partially so a fraction of this aqueous phase is reformed (case-study 2), or all this phase is reformed to H2 (case-study 3). The two former can include CO2 storage and aqueous phase concentrations were 15, 25 and 35 wt% organic compounds. At 25 wt%, the global warming potential is 11 g CO2-eq/MJ-biofuel for the case 2 with CO2 storage, while it was 11.3, 12.6, 27.7 and 34 g CO2-eq/MJ-biofuel for the cases 3, 2 without CO2 storage, 1 with and without CO2 storage, respectively. Thus, the case-study 2 with CO2 storage gives the minimum global warming potential, allowing significant reductions with respect to the use of fossil fuels. For the other categories, the case-study1 presents the lowest impacts. Similar trends are found at 15 and 35 wt%.

Suggested Citation

  • Gutiérrez Ortiz, F.J. & Alonso-Fariñas, B. & Campanario, F.J. & Kruse, A., 2020. "Life cycle assessment of the Fischer-Tropsch biofuels production by supercritical water reforming of the bio-oil aqueous phase," Energy, Elsevier, vol. 210(C).
    • Handle: RePEc:eee:energy:v:210:y:2020:i:c:s0360544220317564
    DOI: 10.1016/j.energy.2020.118648
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    1. Zoppi, Giulia & Tito, Edoardo & Bianco, Isabella & Pipitone, Giuseppe & Pirone, Raffaele & Bensaid, Samir, 2023. "Life cycle assessment of the biofuel production from lignocellulosic biomass in a hydrothermal liquefaction – aqueous phase reforming integrated biorefinery," Renewable Energy, Elsevier, vol. 206(C), pages 375-385.
    2. Hosseinzadeh-Bandbafha, Homa & Nizami, Abdul-Sattar & Kalogirou, Soteris A. & Gupta, Vijai Kumar & Park, Young-Kwon & Fallahi, Alireza & Sulaiman, Alawi & Ranjbari, Meisam & Rahnama, Hassan & Aghbashl, 2022. "Environmental life cycle assessment of biodiesel production from waste cooking oil: A systematic review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 161(C).
    3. Hu, Yaping & Lin, Junhao & Liao, Qinxiong & Sun, Shichang & Ma, Rui & Fang, Lin & Liu, Xiangli, 2021. "CO2-assisted catalytic municipal sludge for carbonaceous biofuel via sub- and supercritical water gasification," Energy, Elsevier, vol. 233(C).

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