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Process integration of chemical looping combustion with oxygen uncoupling in a biomass-fired combined heat and power plant

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  • Peltola, Petteri
  • Saari, Jussi
  • Tynjälä, Tero
  • Hyppänen, Timo

Abstract

Bioenergy with CO2 capture and storage (BECCS) has been introduced as a promising negative emission technology (NET) that opens up the possibility of producing power and heat with negative CO2 emissions. By combining 1.5D reactor modelling with flowsheet simulation of a complete full-scale cogeneration plant, this study assesses the applicability and potential of an advanced CO2 capture technology, namely chemical looping with oxygen uncoupling (CLOU), for CO2 capture from a biomass-fired combined heat and power (CHP) plant generating electricity, district heat (DH) at 75–90 °C supply and 45 °C return temperatures, and process steam at 10 and 4.5 bar(a) pressures. Nordic wood (50% wet-basis moisture) is used as fuel. The key performance indicators of the CLOU-integrated CHP plant were quantified and compared with those of a non-CCS reference plant. Part-load operation at reduced DH loads was considered. At 100% fuel load, the CLOU plant captured 99.0% of the CO2 from the combustion of biomass and still achieved a net efficiency of 80.1%LHV, a value very close to that of the reference plant without CO2 capture or flue gas condensation (81.1%LHV). Depending on the fuel load, the specific negative CO2 emissions from the CLOU plant ranged from 439 to 504 kgCO2/MWh.

Suggested Citation

  • Peltola, Petteri & Saari, Jussi & Tynjälä, Tero & Hyppänen, Timo, 2020. "Process integration of chemical looping combustion with oxygen uncoupling in a biomass-fired combined heat and power plant," Energy, Elsevier, vol. 210(C).
    • Handle: RePEc:eee:energy:v:210:y:2020:i:c:s0360544220316583
    DOI: 10.1016/j.energy.2020.118550
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    References listed on IDEAS

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    2. Krzywanski, J. & Czakiert, T. & Nowak, W. & Shimizu, T. & Zylka, A. & Idziak, K. & Sosnowski, M. & Grabowska, K., 2022. "Gaseous emissions from advanced CLC and oxyfuel fluidized bed combustion of coal and biomass in a complex geometry facility:A comprehensive model," Energy, Elsevier, vol. 251(C).
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    4. Wang, Xudong & Shao, Yali & Jin, Baosheng, 2021. "Thermodynamic evaluation and modelling of an auto-thermal hybrid system of chemical looping combustion and air separation for power generation coupling with CO2 cycles," Energy, Elsevier, vol. 236(C).
    5. Chen, Heng & Wang, Yihan & Li, Jiarui & Xu, Gang & Lei, Jing & Liu, Tong, 2022. "Thermodynamic analysis and economic assessment of an improved geothermal power system integrated with a biomass-fired cogeneration plant," Energy, Elsevier, vol. 240(C).
    6. Yang, Li & Li, Caifu & Song, Chen & Zhu, Dan & Zhao, Jiangyuan & Liu, Fang & Liu, Xiaorui, 2023. "Spatial migration of lattice oxygen for copper-iron based oxygen carriers in chemical looping combustion," Energy, Elsevier, vol. 285(C).
    7. Farajollahi, Hossein & Hossainpour, Siamak, 2023. "Techno-economic assessment of biomass and coal co-fueled chemical looping combustion unit integrated with supercritical CO2 cycle and Organic Rankine cycle," Energy, Elsevier, vol. 274(C).

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