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An experimental study on carbon dioxide hydrate formation using a gas-inducing agitated reactor

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  • Li, Airong
  • Jiang, Lele
  • Tang, Siyao

Abstract

The capture, storage and transportation technology of carbon dioxide based on hydrate formation is an innovative conception. This work presents an experimental investigation on CO2 hydrate formation as a function of rotation speed (0, 200, 400, 600, 800 rpm), temperatures (274.15–279.15 K) and initial pressures (2.09, 3.17, 4.03, 5.04, 6.02 MPa) by using a gas-inducing agitated reactor. It was found that stable CO2 hydrate formation was efficiently enhanced at the stage of CO2 dissolution and nucleation in the liquid phase by the gas-inducing agitated reactor through mechanical agitation and gas recycle. The induction time was shortened from 261 to 24 min with an increase of agitation speed. Reactor design is one of the important effects on CO2 hydrate formation. In addition, temperature and initial pressure also have strong effects on CO2 hydrate formation and storage capacity. The induction time of nucleation was greatly reduced with a decrease in cooling temperature and an increase in initial pressure. The amount of CO2 consumed and storage capacity were also increased.

Suggested Citation

  • Li, Airong & Jiang, Lele & Tang, Siyao, 2017. "An experimental study on carbon dioxide hydrate formation using a gas-inducing agitated reactor," Energy, Elsevier, vol. 134(C), pages 629-637.
    • Handle: RePEc:eee:energy:v:134:y:2017:i:c:p:629-637
    DOI: 10.1016/j.energy.2017.06.023
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    References listed on IDEAS

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    1. Choi, Jae Woo & Chung, Jin Tack & Kang, Yong Tae, 2014. "CO2 hydrate formation at atmospheric pressure using high efficiency absorbent and surfactants," Energy, Elsevier, vol. 78(C), pages 869-876.
    2. E. Dendy Sloan, 2003. "Fundamental principles and applications of natural gas hydrates," Nature, Nature, vol. 426(6964), pages 353-359, November.
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    Cited by:

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    2. Liu, Fa-Ping & Li, Ai-Rong & Wang, Cheng & Ma, Yu-Ling, 2023. "Controlling and tuning CO2 hydrate nucleation and growth by metal-based ionic liquids," Energy, Elsevier, vol. 269(C).
    3. Wang, Lanyun & Zhang, Yajuan & Xie, Huilong & Lu, Xiaoran & Wen, Xinglin & Liu, Zhen & Zhou, Huajian & Liu, Zejian & Xu, Yongliang, 2022. "Effect of voltage and initial temperature on thermodynamics and kinetics of CO2 hydrate formation in an electrostatic spraying reactor," Energy, Elsevier, vol. 239(PD).
    4. Jie Wang & Airong Li & Faping Liu & Zedong Luo, 2021. "Experimental study on in situ dissociation kinetics of CO2 hydrate in pure water and water/sediments systems," Greenhouse Gases: Science and Technology, Blackwell Publishing, vol. 11(2), pages 331-341, April.
    5. Park, Joon Ho & Park, Jungjoon & Lee, Jae Won & Kang, Yong Tae, 2023. "Progress in CO2 hydrate formation and feasibility analysis for cold thermal energy harvesting application," Renewable and Sustainable Energy Reviews, Elsevier, vol. 187(C).
    6. Aminnaji, Morteza & Qureshi, M Fahed & Dashti, Hossein & Hase, Alfred & Mosalanejad, Abdolali & Jahanbakhsh, Amir & Babaei, Masoud & Amiri, Amirpiran & Maroto-Valer, Mercedes, 2024. "CO2 Gas hydrate for carbon capture and storage applications – Part 1," Energy, Elsevier, vol. 300(C).
    7. Cheng, Chuanxiao & Lai, Zhengxiang & Jin, Tingxiang & Jing, Zhiyong & Geng, Wangning & Qi, Tian & Zhu, Shiquan & Zhang, Jun & Liu, Jianxiu & Wang, Fan & Dong, Hongsheng & Zhang, Lunxiang, 2022. "Rapid nucleation and growth of tetrafluoroethane hydrate in the cyclic process of boiling–condensation," Energy, Elsevier, vol. 256(C).
    8. Liu, Fa-Ping & Li, Ai-Rong & Qing, Sheng-Lan & Luo, Ze-Dong & Ma, Yu-Ling, 2022. "Formation kinetics, mechanism of CO2 hydrate and its applications," Renewable and Sustainable Energy Reviews, Elsevier, vol. 159(C).
    9. Liu, Fa-Ping & Li, Ai-Rong & Wang, Jie & Luo, Ze-Dong, 2021. "Iron-based ionic liquid ([BMIM][FeCl4]) as a promoter of CO2 hydrate nucleation and growth," Energy, Elsevier, vol. 214(C).

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