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Absorption of nitric oxide from simulated flue gas using different absorbents at room temperature and atmospheric pressure

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  • Yu, Hesheng
  • Zhu, Qunyi
  • Tan, Zhongchao

Abstract

Effective removal of nitrogen oxides (NOx) from flue gas allows more fossil fuels to be produced and utilized with less negative impact on the environment. It would be more cost-effective, however, if nitric oxide (NO) is oxidized to soluble nitrate and nitrite and then removed from the air by existing desulfurization wet scrubbers. This paper compares the effectiveness of three different oxidants for this purpose, namely, ethylenediaminetetraacetic acid; iron (2+) (Fe(II)–EDTA), hexamminecobalt(II) chloride ([Co(NH3)6]Cl2), and hydrogen peroxide (H2O2). Experimental results using column reactors showed that [Co(NH3)6]Cl2 was more effective over the same period of time. The best initial NO removal efficiency of about 96.45% was measured at the inlet flow rate of 500ml/min; the temperature of approximately 19°C; the pH value of around 10.5; and the concentrations of [Co(NH3)6]Cl2 , NO and O2 of 0.06mol/L, 500ppm and 5.0%, respectively.

Suggested Citation

  • Yu, Hesheng & Zhu, Qunyi & Tan, Zhongchao, 2012. "Absorption of nitric oxide from simulated flue gas using different absorbents at room temperature and atmospheric pressure," Applied Energy, Elsevier, vol. 93(C), pages 53-58.
    • Handle: RePEc:eee:appene:v:93:y:2012:i:c:p:53-58
    DOI: 10.1016/j.apenergy.2011.03.039
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    References listed on IDEAS

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    1. Roy, Sounak & Hegde, M.S. & Madras, Giridhar, 2009. "Catalysis for NOx abatement," Applied Energy, Elsevier, vol. 86(11), pages 2283-2297, November.
    2. Gao, Xiang & Ding, Honglei & Du, Zhen & Wu, Zuliang & Fang, Mengxiang & Luo, Zhongyang & Cen, Kefa, 2010. "Gas-liquid absorption reaction between (NH4)2SO3 solution and SO2 for ammonia-based wet flue gas desulfurization," Applied Energy, Elsevier, vol. 87(8), pages 2647-2651, August.
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    1. Li, Kangkang & Yu, Hai & Qi, Guojie & Feron, Paul & Tade, Moses & Yu, Jingwen & Wang, Shujuan, 2015. "Rate-based modelling of combined SO2 removal and NH3 recycling integrated with an aqueous NH3-based CO2 capture process," Applied Energy, Elsevier, vol. 148(C), pages 66-77.
    2. Xu, Yin & Jin, Baosheng & Zhao, Yongling & Hu, Eric J. & Chen, Xiaole & Li, Xiaochuan, 2018. "Numerical simulation of aqueous ammonia-based CO2 absorption in a sprayer tower: An integrated model combining gas-liquid hydrodynamics and chemistry," Applied Energy, Elsevier, vol. 211(C), pages 318-333.

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