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High reversible cycling performance of carbon dioxide electrolysis by flat-tube solid oxide cell

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  • Li, Chaolei
  • Wu, Anqi
  • Xi, Chengqiao
  • Guan, Wanbing
  • Chen, Liang
  • Singhal, Subhash C.

Abstract

Solid oxide cells (SOCs) are promising for CO2 electrolysis. In this work, performance and stability of flat-tube SOCs during periodic cycles of CO2 electrolysis and hydrogen fuel discharge were studied. The cell underwent 26 reversible cycles of operation for 624 h. When the cell was electrolyzed with a current density of −200 mA/cm2 at 1.07 V, the CO yield was 205.79 sccm and the CO2 conversion rate reached 45.7%. When the cell was operated in electrolysis mode, the degradation rate was 0.74 mV/h. Excluding the air heat consumption, the energy conversion efficiency was 81.42%; when the cell was operated at 0.6 slm hydrogen and +200 mA/cm2, the degradation rate was 0.385 mV/h. Compared with long-term constant current electrolysis, the alternate operation of charge and discharge used in this study is more typical of the actual application conditions.

Suggested Citation

  • Li, Chaolei & Wu, Anqi & Xi, Chengqiao & Guan, Wanbing & Chen, Liang & Singhal, Subhash C., 2022. "High reversible cycling performance of carbon dioxide electrolysis by flat-tube solid oxide cell," Applied Energy, Elsevier, vol. 314(C).
    • Handle: RePEc:eee:appene:v:314:y:2022:i:c:s0306261922003816
    DOI: 10.1016/j.apenergy.2022.118969
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    References listed on IDEAS

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    1. Lu, Lianmei & Liu, Wu & Wang, Jianxin & Wang, Yudong & Xia, Changrong & Zhou, Xiao-Dong & Chen, Ming & Guan, Wanbing, 2020. "Long-term stability of carbon dioxide electrolysis in a large-scale flat-tube solid oxide electrolysis cell based on double-sided air electrodes," Applied Energy, Elsevier, vol. 259(C).
    2. Zheng, Yifeng & Wang, Shun & Pan, Zehua & Yin, Bo, 2021. "Electrochemical CO2 reduction to CO using solid oxide electrolysis cells with high-performance Ta-doped bismuth strontium ferrite air electrode," Energy, Elsevier, vol. 228(C).
    3. Liu, Zhao & Han, Beibei & Lu, Zhiyi & Guan, Wanbing & Li, Yuanyuan & Song, Changjiang & Chen, Liang & Singhal, Subhash C., 2021. "Efficiency and stability of hydrogen production from seawater using solid oxide electrolysis cells," Applied Energy, Elsevier, vol. 300(C).
    4. Muhammad Jabir & Hazlee Azil Illias & Safdar Raza & Hazlie Mokhlis, 2017. "Intermittent Smoothing Approaches for Wind Power Output: A Review," Energies, MDPI, vol. 10(10), pages 1-23, October.
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    1. Yao, Yue & Ma, Yue & Wang, Chenpeng & Ye, Hao & Liu, Yinglong & Liu, Jiawei & Zhao, Xiaobo & Tao, Tao & Yao, Yingbang & Lu, Shengguo & Yang, Huazheng & Liang, Bo, 2022. "A cofuel channel microtubular solid oxide fuel/electrolysis cell," Applied Energy, Elsevier, vol. 327(C).

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