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Process integration of a Calcium-looping process with a natural gas combined cycle power plant for CO2 capture and its improvement by exhaust gas recirculation

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  • Hu, Yue
  • Ahn, Hyungwoong

Abstract

In this study, it was sought to find an efficient way to integrate a Ca-looping process with a Natural Gas Combined Cycle (NGCC) power plant for its post-combustion CO2 capture. Compared to its application to coal combustion flue gas, Ca-looping would incur augmented energy penalty when integrated with a NGCC of which the flue gas contains only 4.0mol% CO2. The reduced CO2 concentration in the feed requires the carbonator to operate at a lower temperature and more solids to circulate between carbonator and calciner for keeping up the carbon capture efficiency at 90%. However, this study demonstrated that such negative effects could be alleviated greatly by implementing 40% exhaust gas recirculation to the NGCC with the CO2 concentration in the flue gas increasing up to 6.8%. Accordingly, the resulting net power efficiency increased notably 1.6% points in comparison to its equivalent non-EGR NGCC case and it was only 0.9% points less than amine capture case. This study exhibited that exhaust gas recirculation would be crucial in decarbonising a NGCC power plant by Ca-looping.

Suggested Citation

  • Hu, Yue & Ahn, Hyungwoong, 2017. "Process integration of a Calcium-looping process with a natural gas combined cycle power plant for CO2 capture and its improvement by exhaust gas recirculation," Applied Energy, Elsevier, vol. 187(C), pages 480-488.
    • Handle: RePEc:eee:appene:v:187:y:2017:i:c:p:480-488
    DOI: 10.1016/j.apenergy.2016.11.014
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    References listed on IDEAS

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    1. Lindqvist, Karl & Jordal, Kristin & Haugen, Geir & Hoff, Karl Anders & Anantharaman, Rahul, 2014. "Integration aspects of reactive absorption for post-combustion CO2 capture from NGCC (natural gas combined cycle) power plants," Energy, Elsevier, vol. 78(C), pages 758-767.
    2. Ortiz, C. & Chacartegui, R. & Valverde, J.M. & Becerra, J.A., 2016. "A new integration model of the calcium looping technology into coal fired power plants for CO2 capture," Applied Energy, Elsevier, vol. 169(C), pages 408-420.
    3. Perejón, Antonio & Romeo, Luis M. & Lara, Yolanda & Lisbona, Pilar & Martínez, Ana & Valverde, Jose Manuel, 2016. "The Calcium-Looping technology for CO2 capture: On the important roles of energy integration and sorbent behavior," Applied Energy, Elsevier, vol. 162(C), pages 787-807.
    4. Valverde, J.M. & Sanchez-Jimenez, P.E. & Perez-Maqueda, L.A., 2014. "Role of precalcination and regeneration conditions on postcombustion CO2 capture in the Ca-looping technology," Applied Energy, Elsevier, vol. 136(C), pages 347-356.
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    6. Xiang, Yanlei & Cai, Lei & Guan, Yanwen & Liu, Wenbin & Han, Yixiao & Liang, Ying, 2018. "Study on the configuration of bottom cycle in natural gas combined cycle power plants integrated with oxy-fuel combustion," Applied Energy, Elsevier, vol. 212(C), pages 465-477.
    7. Li, Hongwei & Tang, Zhigang & Xing, Xiao & Guo, Dong & Cui, Longpeng & Mao, Xian-zhong, 2018. "Study of CO2 capture by seawater and its reinforcement," Energy, Elsevier, vol. 164(C), pages 1135-1144.
    8. Song, Chunfeng & Liu, Qingling & Ji, Na & Deng, Shuai & Zhao, Jun & Kitamura, Yutaka, 2017. "Natural gas purification by heat pump assisted MEA absorption process," Applied Energy, Elsevier, vol. 204(C), pages 353-361.
    9. Kong, Mengdi & Ye, Xuemin & Liu, Di & Li, Chunxi, 2024. "Comprehensive evaluation of medical waste gasification low-carbon multi-generation system based on AHP–EWM–GFCE method," Energy, Elsevier, vol. 296(C).
    10. Shi, Jiewen & Li, Yingjie & Zhang, Qing & Ma, Xiaotong & Duan, Lunbo & Zhou, Xingang, 2017. "CO2 capture performance of a novel synthetic CaO/sepiolite sorbent at calcium looping conditions," Applied Energy, Elsevier, vol. 203(C), pages 412-421.
    11. Strojny, Magdalena & Gładysz, Paweł & Hanak, Dawid P. & Nowak, Wojciech, 2023. "Comparative analysis of CO2 capture technologies using amine absorption and calcium looping integrated with natural gas combined cycle power plant," Energy, Elsevier, vol. 284(C).

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