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Mass transfer of ammonia escape and CO2 absorption in CO2 capture using ammonia solution in bubbling reactor

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  • Ma, Shuangchen
  • Chen, Gongda
  • Zhu, Sijie
  • Han, Tingting
  • Yu, Weijing

Abstract

The mass transfer of CO2 capture using ammonia solution in the bubbling reactor was studied; according to double film theory, the mass transfer coefficient models and interface area model were built. Through our experiments, the overall volumetric mass transfer coefficients were obtained, while the interface areas in unit volume were estimated. The volumetric mass transfer coefficients of ammonia escaping during the experiment were 1.39×10−5–4.34×10−5mol/(m3sPa), and the volumetric mass transfer coefficients of CO2 absorption were 2.86×10−5–17.9×10−5mol/(m3sPa). The estimated interface area of unit volume in the bubbling reactor ranged from 75.19 to 256.41m2/m3, making the bubbling reactor a viable choice to obtain higher mass transfer performance than the packed tower or spraying tower.

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  • Ma, Shuangchen & Chen, Gongda & Zhu, Sijie & Han, Tingting & Yu, Weijing, 2016. "Mass transfer of ammonia escape and CO2 absorption in CO2 capture using ammonia solution in bubbling reactor," Applied Energy, Elsevier, vol. 162(C), pages 354-362.
    • Handle: RePEc:eee:appene:v:162:y:2016:i:c:p:354-362
    DOI: 10.1016/j.apenergy.2015.10.089
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    5. Chu, Fengming & Yang, Lijun & Du, Xiaoze & Yang, Yongping, 2017. "Mass transfer and energy consumption for CO2 absorption by ammonia solution in bubble column," Applied Energy, Elsevier, vol. 190(C), pages 1068-1080.
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    8. Yifang Liu & Fengming Chu & Lijun Yang & Xiaoze Du & Yongping Yang, 2018. "CO2 absorption characteristics in a random packed column with various geometric structures and working conditions," Greenhouse Gases: Science and Technology, Blackwell Publishing, vol. 8(1), pages 120-132, February.
    9. Song, Chunfeng & Xie, Meilian & Qiu, Yiting & Liu, Qingling & Sun, Luchang & Wang, Kailiang & Kansha, Yasuki, 2019. "Integration of CO2 absorption with biological transformation via using rich ammonia solution as a nutrient source for microalgae cultivation," Energy, Elsevier, vol. 179(C), pages 618-627.
    10. Chu, Fengming & Liu, Yifang & Yang, Lijun & Du, Xiaoze & Yang, Yongping, 2017. "Ammonia escape mass transfer and heat transfer characteristics of CO2 absorption in packed absorbing column," Applied Energy, Elsevier, vol. 205(C), pages 1596-1604.
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