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Direct carbon fuel cell operation on brown coal

Author

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  • Rady, Adam C.
  • Giddey, Sarbjit
  • Kulkarni, Aniruddha
  • Badwal, Sukhvinder P.S.
  • Bhattacharya, Sankar
  • Ladewig, Bradley P.

Abstract

The performance of a Victorian brown coal with minimal pre-treatment was assessed in a solid oxide electrolyte based direct carbon fuel cell (DCFC) at 700 and 800°C. In order to evaluate the effect of inherent inorganic species in the coal on the electrochemical performance of DCFCs (voltage – power density – current density), characteristics of button cells fuelled with raw and acid washed (demineralised) coal were compared along with commercially available XC72 carbon black. Peak power densities of 65 and 67mWcm−2 were observed for demineralised coal char and carbon black respectively at 800°C, whereas the raw coal char achieved a superior power density of 89mWcm−2. The availability of reactive species at the anode, namely CO, is believed to be the primary differentiator of cell performance, and is related to variations in the physical and chemical makeup of carbon fuels. The reactivity of these fuels in the presence of CO2 to generate CO (and power) via Boudouard gasification was assessed in the 700–800°C temperature range via thermogravimetric analysis.

Suggested Citation

  • Rady, Adam C. & Giddey, Sarbjit & Kulkarni, Aniruddha & Badwal, Sukhvinder P.S. & Bhattacharya, Sankar & Ladewig, Bradley P., 2014. "Direct carbon fuel cell operation on brown coal," Applied Energy, Elsevier, vol. 120(C), pages 56-64.
    • Handle: RePEc:eee:appene:v:120:y:2014:i:c:p:56-64
    DOI: 10.1016/j.apenergy.2014.01.046
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    References listed on IDEAS

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    1. Keith Burnard & Sankar Bhattacharya, 2011. "Power Generation from Coal: Ongoing Developments and Outlook," IEA Energy Papers 2011/14, OECD Publishing.
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    4. Lithnes Kalaivani Palniandy & Li Wan Yoon & Wai Yin Wong & Siek-Ting Yong & Ming Meng Pang, 2019. "Application of Biochar Derived from Different Types of Biomass and Treatment Methods as a Fuel Source for Direct Carbon Fuel Cells," Energies, MDPI, vol. 12(13), pages 1-15, June.
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    6. Chen, Qianyang & Qiu, Qianyuan & Yan, Xiaomin & Zhou, Mingyang & Zhang, Yapeng & Liu, Zhijun & Cai, Weizi & Wang, Wei & Liu, Jiang, 2020. "A compact and seal-less direct carbon solid oxide fuel cell stack stepping into practical application," Applied Energy, Elsevier, vol. 278(C).
    7. Duan, Nan-Qi & Tan, Yuan & Yan, Dong & Jia, Lichao & Chi, Bo & Pu, Jian & Li, Jian, 2016. "Biomass carbon fueled tubular solid oxide fuel cells with molten antimony anode," Applied Energy, Elsevier, vol. 165(C), pages 983-989.
    8. Hao, Wenbin & Mi, Yongli, 2016. "Evaluation of waste paper as a source of carbon fuel for hybrid direct carbon fuel cells," Energy, Elsevier, vol. 107(C), pages 122-130.
    9. Rizkiana, Jenny & Guan, Guoqing & Widayatno, Wahyu Bambang & Hao, Xiaogang & Wang, Zhongde & Zhang, Zhonglin & Abudula, Abuliti, 2015. "Oil production from mild pyrolysis of low-rank coal in molten salts media," Applied Energy, Elsevier, vol. 154(C), pages 944-950.
    10. Hao, Wenbin & He, Xiaojin & Mi, Yongli, 2014. "Achieving high performance in intermediate temperature direct carbon fuel cells with renewable carbon as a fuel source," Applied Energy, Elsevier, vol. 135(C), pages 174-181.
    11. Jiao, Yong & Tian, Wenjuan & Chen, Huili & Shi, Huangang & Yang, Binbin & Li, Chao & Shao, Zongping & Zhu, Zhenping & Li, Si-Dian, 2015. "In situ catalyzed Boudouard reaction of coal char for solid oxide-based carbon fuel cells with improved performance," Applied Energy, Elsevier, vol. 141(C), pages 200-208.
    12. Wu, Hao & Xiao, Jie & Zeng, Xiaoyuan & Li, Xue & Yang, Jing & Zou, Yuling & Liu, Sudongfang & Dong, Peng & Zhang, Yingjie & Liu, Jiang, 2019. "A high performance direct carbon solid oxide fuel cell – A green pathway for brown coal utilization," Applied Energy, Elsevier, vol. 248(C), pages 679-687.
    13. Zhang, Ji & Liang, Yanna & Harpalani, Satya, 2016. "Optimization of methane production from bituminous coal through biogasification," Applied Energy, Elsevier, vol. 183(C), pages 31-42.
    14. Ozalp, N. & Abedini, H. & Abuseada, M. & Davis, R. & Rutten, J. & Verschoren, J. & Ophoff, C. & Moens, D., 2022. "An overview of direct carbon fuel cells and their promising potential on coupling with solar thermochemical carbon production," Renewable and Sustainable Energy Reviews, Elsevier, vol. 162(C).
    15. Xie, Heping & Zhai, Shuo & Chen, Bin & Liu, Tao & Zhang, Yuan & Ni, Meng & Shao, Zongping, 2020. "Coal pretreatment and Ag-infiltrated anode for high-performance hybrid direct coal fuel cell," Applied Energy, Elsevier, vol. 260(C).

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