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The use of ilmenite as oxygen carrier with kerosene in a 300W CLC laboratory reactor with continuous circulation

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  • Moldenhauer, Patrick
  • Rydén, Magnus
  • Mattisson, Tobias
  • Younes, Mourad
  • Lyngfelt, Anders

Abstract

An ilmenite oxygen carrier was tested in a laboratory scale chemical-looping reactor with a nominal thermal capacity of 300Wth. Ilmenite is a mineral iron–titanium oxide, which has been used extensively as an oxygen carrier in chemical-looping combustion. Two different kinds of fuels were used, a sulfur-free kerosene and one kerosene that contained 0.57 mass% sulfur. Both fuels were continuously evaporated and directly fed into the chemical-looping reactor. Experiments were conducted for 50h with the sulfur-free kerosene and for 30h with the sulfurous kerosene. CO2 yields above 99% were achieved with both types of fuel. A significant and lasting improvement in the oxygen carrier’s reactivity was observed, presumably an effect of using sulfurous kerosene. No evidence of sulfur was found on the particles’ surface.

Suggested Citation

  • Moldenhauer, Patrick & Rydén, Magnus & Mattisson, Tobias & Younes, Mourad & Lyngfelt, Anders, 2014. "The use of ilmenite as oxygen carrier with kerosene in a 300W CLC laboratory reactor with continuous circulation," Applied Energy, Elsevier, vol. 113(C), pages 1846-1854.
    • Handle: RePEc:eee:appene:v:113:y:2014:i:c:p:1846-1854
    DOI: 10.1016/j.apenergy.2013.06.009
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    Cited by:

    1. Tomasz Czakiert & Jaroslaw Krzywanski & Anna Zylka & Wojciech Nowak, 2022. "Chemical Looping Combustion: A Brief Overview," Energies, MDPI, vol. 15(4), pages 1-19, February.
    2. Nandy, Anirban & Loha, Chanchal & Gu, Sai & Sarkar, Pinaki & Karmakar, Malay K. & Chatterjee, Pradip K., 2016. "Present status and overview of Chemical Looping Combustion technology," Renewable and Sustainable Energy Reviews, Elsevier, vol. 59(C), pages 597-619.
    3. Iloeje, Chukwunwike O. & Zhao, Zhenlong & Ghoniem, Ahmed F., 2017. "A reduced fidelity model for the rotary chemical looping combustion reactor," Applied Energy, Elsevier, vol. 190(C), pages 725-739.
    4. Hu, Wenting & Donat, Felix & Scott, S.A. & Dennis, J.S., 2016. "Kinetics of oxygen uncoupling of a copper based oxygen carrier," Applied Energy, Elsevier, vol. 161(C), pages 92-100.
    5. Ogidiama, Oghare Victor & Abu-Zahra, Mohammad R.M. & Shamim, Tariq, 2018. "Techno-economic analysis of a poly-generation solar-assisted chemical looping combustion power plant," Applied Energy, Elsevier, vol. 228(C), pages 724-735.
    6. Xu, Lei & Sun, Hongming & Li, Zhenshan & Cai, Ningsheng, 2016. "Experimental study of copper modified manganese ores as oxygen carriers in a dual fluidized bed reactor," Applied Energy, Elsevier, vol. 162(C), pages 940-947.
    7. Jacobs, M. & Van Noyen, J. & Larring, Y. & Mccann, M. & Pishahang, M. & Amini, S. & Ortiz, M. & Galluci, F. & Sint-Annaland, M.V. & Tournigant, D. & Louradour, E. & Snijkers, F., 2015. "Thermal and mechanical behaviour of oxygen carrier materials for chemical looping combustion in a packed bed reactor," Applied Energy, Elsevier, vol. 157(C), pages 374-381.
    8. Güleç, Fatih & Meredith, Will & Sun, Cheng-Gong & Snape, Colin E., 2019. "Selective low temperature chemical looping combustion of higher alkanes with Cu- and Mn- oxides," Energy, Elsevier, vol. 173(C), pages 658-666.
    9. Iloeje, Chukwunwike O. & Zhao, Zhenlong & Ghoniem, Ahmed F., 2018. "Design and techno-economic optimization of a rotary chemical looping combustion power plant with CO2 capture," Applied Energy, Elsevier, vol. 231(C), pages 1179-1190.
    10. García-Labiano, F. & de Diego, L.F. & Gayán, P. & Abad, A. & Cabello, A. & Adánez, J. & Sprachmann, G., 2014. "Energy exploitation of acid gas with high H2S content by means of a chemical looping combustion system," Applied Energy, Elsevier, vol. 136(C), pages 242-249.
    11. Adnan, Muflih A. & Azis, Muhammad Mufti & Quddus, Mohammad R. & Hossain, Mohammad M., 2018. "Integrated liquid fuel based chemical looping combustion – parametric study for efficient power generation and CO2 capture," Applied Energy, Elsevier, vol. 228(C), pages 2398-2406.
    12. Wang, Haiming & Liu, Guicai & Veksha, Andrei & Giannis, Apostolos & Lim, Teik-Thye & Lisak, Grzegorz, 2021. "Effective H2S control during chemical looping combustion by iron ore modified with alkaline earth metal oxides," Energy, Elsevier, vol. 218(C).
    13. García-Labiano, Francisco & de Diego, Luis F. & Cabello, Arturo & Gayán, Pilar & Abad, Alberto & Adánez, Juan & Sprachmann, Gerald, 2016. "Sulphuric acid production via Chemical Looping Combustion of elemental sulphur," Applied Energy, Elsevier, vol. 178(C), pages 736-745.

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