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Air-breathing membraneless laminar flow-based fuel cells: Do they breathe enough oxygen?

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  • Xuan, Jin
  • Leung, D.Y.C.
  • Wang, Huizhi
  • Leung, Michael K.H.
  • Wang, Bin
  • Ni, Meng

Abstract

Laminar flow-based fuel cell (LFFC) is a relatively new type of fuel cell that does not require the use of proton exchange membrane. While the first-generation LFFC uses dissolved oxygen at the cathode, the second-generation LFFC (2G-LFFC) adopts a more advanced air-breathing design for achieving high power density. The architecture and operational mechanisms of a 2G-LFFC are more complex. In order to gain detailed understanding of the 2G-LFFC, an integrated CFD/electrochemical kinetics modeling study has been conducted to analyze the cell limiting factors and sufficiency of the oxidant supply from air. It is found that under most typical operating conditions, the 2G-LFFC free-breathing mode can supply sufficient oxygen to the electrode reactive surface for cathode half-cell reaction, indicating that the air breathing process is not a limiting factor to the cell performance. However, oxygen starvation will become a major performance limiting factor when the anode is enhanced for higher current density. The results presented in this paper provide useful design guidance for future development of LFFC.

Suggested Citation

  • Xuan, Jin & Leung, D.Y.C. & Wang, Huizhi & Leung, Michael K.H. & Wang, Bin & Ni, Meng, 2013. "Air-breathing membraneless laminar flow-based fuel cells: Do they breathe enough oxygen?," Applied Energy, Elsevier, vol. 104(C), pages 400-407.
    • Handle: RePEc:eee:appene:v:104:y:2013:i:c:p:400-407
    DOI: 10.1016/j.apenergy.2012.10.063
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    References listed on IDEAS

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    1. Xuan, Jin & Leung, Michael K.H. & Leung, Dennis Y.C. & Wang, Huizhi, 2012. "Laminar flow-based fuel cell working under critical conditions: The effect of parasitic current," Applied Energy, Elsevier, vol. 90(1), pages 87-93.
    2. Jung, Chi-Young & Shim, Hyo-Sub & Koo, Sang-Man & Lee, Sang-Hwan & Yi, Sung-Chul, 2012. "Investigations of the temperature distribution in proton exchange membrane fuel cells," Applied Energy, Elsevier, vol. 93(C), pages 733-741.
    3. Nam, Jinmoo & Chippar, Purushothama & Kim, Whangi & Ju, Hyunchul, 2010. "Numerical analysis of gas crossover effects in polymer electrolyte fuel cells (PEFCs)," Applied Energy, Elsevier, vol. 87(12), pages 3699-3709, December.
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    Cited by:

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    9. Ouyang, Tiancheng & Chen, Jingxian & Liu, Wenjun & Xu, Peihang & Lu, Jie & Zhao, Zhongkai, 2022. "A comprehensive evaluation for microfluidic fuel cells from anti-vibration viewpoint using phase field theory," Renewable Energy, Elsevier, vol. 189(C), pages 676-693.
    10. Muhammad Tanveer & Kwang-Yong Kim, 2021. "Flow Configurations of Membraneless Microfluidic Fuel Cells: A Review," Energies, MDPI, vol. 14(12), pages 1-33, June.
    11. Lan, Qiao & Ye, Dingding & Zhu, Xun & Chen, Rong & Liao, Qiang, 2022. "Enhanced gas removal and cell performance of a microfluidic fuel cell by a paper separator embedded in the microchannel," Energy, Elsevier, vol. 239(PB).
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