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Amine-Ionic Liquid Blends in CO2 Capture Process for Sustainable Energy and Environment

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  • Muthumari Perumal
  • Dhanalakshmi Jayaraman

Abstract

In the present work, an experiment for CO 2 capture process were performed by absorption using various aqueous solvent blends of amine and ionic liquids. The solvent blends were prepared for various compositions by mixing TetraButylAmmonium Acetate [TBA][OAC] and TetraButylAmmonium Bromide [TBA][Br] ionic liquids with Monoethanolamine (MEA). The obtained results were compared with baseline MEA. It was observed that capture efficiency of CO 2 , absorption rate of CO 2 and CO 2 diffusion coefficient of MEA-[TBA][OAC] and MEA-[TBA][Br] solvent blends were comparatively higher than baseline 30%MEA. Moreover, the parameters such as density, viscosity, pH, carbon loading and surface tension of all the solvent blends were measured for before and after absorption process. The carbon loading of solvent blends MEA-[TBA][Br] (0.405 mole of CO 2 /mole of solvent) and MEA-[TBA][OAC](0.459 mole of CO 2 /mole of solvent) was slightly lower than baseline MEA (0.494 mole of CO 2 /mole of solvent). However, the viscosity of MEA-[TBA][Br] blends were remarkably lower than MEA-[TBA][OAC] blend and baseline MEA. This might be an important key factor in solvent recovery process with lesser energy demand for sustainable energy and environment.

Suggested Citation

  • Muthumari Perumal & Dhanalakshmi Jayaraman, 2023. "Amine-Ionic Liquid Blends in CO2 Capture Process for Sustainable Energy and Environment," Energy & Environment, , vol. 34(3), pages 517-532, May.
    • Handle: RePEc:sae:engenv:v:34:y:2023:i:3:p:517-532
    DOI: 10.1177/0958305X211070782
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    1. Aghaie, Mahsa & Rezaei, Nima & Zendehboudi, Sohrab, 2018. "A systematic review on CO2 capture with ionic liquids: Current status and future prospects," Renewable and Sustainable Energy Reviews, Elsevier, vol. 96(C), pages 502-525.
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