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Partially oxidized atomic cobalt layers for carbon dioxide electroreduction to liquid fuel

Author

Listed:
  • Shan Gao

    (Hefei National Laboratory for Physical Sciences at Microscale, Collaborative Innovation Center of Chemistry for Energy Materials, University of Science and Technology of China)

  • Yue Lin

    (Hefei National Laboratory for Physical Sciences at Microscale, Collaborative Innovation Center of Chemistry for Energy Materials, University of Science and Technology of China)

  • Xingchen Jiao

    (Hefei National Laboratory for Physical Sciences at Microscale, Collaborative Innovation Center of Chemistry for Energy Materials, University of Science and Technology of China)

  • Yongfu Sun

    (Hefei National Laboratory for Physical Sciences at Microscale, Collaborative Innovation Center of Chemistry for Energy Materials, University of Science and Technology of China
    Hefei Science Center of CAS)

  • Qiquan Luo

    (Hefei National Laboratory for Physical Sciences at Microscale, Collaborative Innovation Center of Chemistry for Energy Materials, University of Science and Technology of China)

  • Wenhua Zhang

    (Hefei National Laboratory for Physical Sciences at Microscale, Collaborative Innovation Center of Chemistry for Energy Materials, University of Science and Technology of China)

  • Dianqi Li

    (Hefei National Laboratory for Physical Sciences at Microscale, Collaborative Innovation Center of Chemistry for Energy Materials, University of Science and Technology of China)

  • Jinlong Yang

    (Hefei National Laboratory for Physical Sciences at Microscale, Collaborative Innovation Center of Chemistry for Energy Materials, University of Science and Technology of China)

  • Yi Xie

    (Hefei National Laboratory for Physical Sciences at Microscale, Collaborative Innovation Center of Chemistry for Energy Materials, University of Science and Technology of China
    Hefei Science Center of CAS)

Abstract

Electroreduction of carbon dioxide into useful fuels helps to reduce fossil-fuel consumption and carbon dioxide emissions, but activating carbon dioxide requires impractically high overpotentials; here a metal atomic layer combined with its native oxide that requires low overpotentials to reduce carbon dioxide is developed, adapted from an existing cobalt-based catalyst.

Suggested Citation

  • Shan Gao & Yue Lin & Xingchen Jiao & Yongfu Sun & Qiquan Luo & Wenhua Zhang & Dianqi Li & Jinlong Yang & Yi Xie, 2016. "Partially oxidized atomic cobalt layers for carbon dioxide electroreduction to liquid fuel," Nature, Nature, vol. 529(7584), pages 68-71, January.
    • Handle: RePEc:nat:nature:v:529:y:2016:i:7584:d:10.1038_nature16455
    DOI: 10.1038/nature16455
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    Cited by:

    1. Junyuan Duan & Tianyang Liu & Yinghe Zhao & Ruoou Yang & Yang Zhao & Wenbin Wang & Youwen Liu & Huiqiao Li & Yafei Li & Tianyou Zhai, 2022. "Active and conductive layer stacked superlattices for highly selective CO2 electroreduction," Nature Communications, Nature, vol. 13(1), pages 1-11, December.
    2. Zhiwen Jiang & Carine Clavaguéra & Changjiang Hu & Sergey A. Denisov & Shuning Shen & Feng Hu & Jun Ma & Mehran Mostafavi, 2023. "Direct time-resolved observation of surface-bound carbon dioxide radical anions on metallic nanocatalysts," Nature Communications, Nature, vol. 14(1), pages 1-11, December.
    3. Nannan Meng & Zhitan Wu & Yanmei Huang & Jie Zhang & Maoxin Chen & Haibin Ma & Hongjiao Li & Shibo Xi & Ming Lin & Wenya Wu & Shuhe Han & Yifu Yu & Quan-Hong Yang & Bin Zhang & Kian Ping Loh, 2024. "High yield electrosynthesis of oxygenates from CO using a relay Cu-Ag co-catalyst system," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    4. Guifeng Ma & Olga A. Syzgantseva & Yan Huang & Dragos Stoian & Jie Zhang & Shuliang Yang & Wen Luo & Mengying Jiang & Shumu Li & Chunjun Chen & Maria A. Syzgantseva & Sen Yan & Ningyu Chen & Li Peng &, 2023. "A hydrophobic Cu/Cu2O sheet catalyst for selective electroreduction of CO to ethanol," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    5. Huihui Zhang & Chang Xu & Xiaowen Zhan & Yu Yu & Kaifu Zhang & Qiquan Luo & Shan Gao & Jinlong Yang & Yi Xie, 2022. "Mechanistic insights into CO2 conversion chemistry of copper bis-(terpyridine) molecular electrocatalyst using accessible operando spectrochemistry," Nature Communications, Nature, vol. 13(1), pages 1-11, December.
    6. Xin Chen & Junxiang Chen & Huayu Chen & Qiqi Zhang & Jiaxuan Li & Jiwei Cui & Yanhui Sun & Defa Wang & Jinhua Ye & Lequan Liu, 2023. "Promoting water dissociation for efficient solar driven CO2 electroreduction via improving hydroxyl adsorption," Nature Communications, Nature, vol. 14(1), pages 1-12, December.
    7. Jiqing Jiao & Qing Yuan & Meijie Tan & Xiaoqian Han & Mingbin Gao & Chao Zhang & Xuan Yang & Zhaolin Shi & Yanbin Ma & Hai Xiao & Jiangwei Zhang & Tongbu Lu, 2023. "Constructing asymmetric double-atomic sites for synergistic catalysis of electrochemical CO2 reduction," Nature Communications, Nature, vol. 14(1), pages 1-12, December.
    8. Hongfei Wang & Zhipeng Yu & Jie Zhou & Chengming Li & Ananthanarasimhan Jayanarasimhan & Xiqiang Zhao & Hao Zhang, 2023. "A Scientometric Review of CO 2 Electroreduction Research from 2005 to 2022," Energies, MDPI, vol. 16(2), pages 1-21, January.
    9. Chunjun Chen & Xupeng Yan & Yahui Wu & Xiudong Zhang & Shoujie Liu & Fanyu Zhang & Xiaofu Sun & Qinggong Zhu & Lirong Zheng & Jing Zhang & Xueqing Xing & Zhonghua Wu & Buxing Han, 2023. "Oxidation of metallic Cu by supercritical CO2 and control synthesis of amorphous nano-metal catalysts for CO2 electroreduction," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    10. Seung-Jae Shin & Hansol Choi & Stefan Ringe & Da Hye Won & Hyung-Suk Oh & Dong Hyun Kim & Taemin Lee & Dae-Hyun Nam & Hyungjun Kim & Chang Hyuck Choi, 2022. "A unifying mechanism for cation effect modulating C1 and C2 productions from CO2 electroreduction," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    11. An, Xiaowei & Li, Shasha & Hao, Xiaoqiong & Xie, Zhengkun & Du, Xiao & Wang, Zhongde & Hao, Xiaogang & Abudula, Abuliti & Guan, Guoqing, 2021. "Common strategies for improving the performances of tin and bismuth-based catalysts in the electrocatalytic reduction of CO2 to formic acid/formate," Renewable and Sustainable Energy Reviews, Elsevier, vol. 143(C).
    12. Nehil Shreyash & Muskan Sonker & Sushant Bajpai & Saurabh Kr Tiwary & Mohd Ashhar Khan & Subham Raj & Tushar Sharma & Susham Biswas, 2021. "The Review of Carbon Capture-Storage Technologies and Developing Fuel Cells for Enhancing Utilization," Energies, MDPI, vol. 14(16), pages 1-34, August.
    13. Zhibo Yao & Hao Cheng & Yifei Xu & Xinyu Zhan & Song Hong & Xinyi Tan & Tai-Sing Wu & Pei Xiong & Yun-Liang Soo & Molly Meng-Jung Li & Leiduan Hao & Liang Xu & Alex W. Robertson & Bingjun Xu & Ming Ya, 2024. "Hydrogen radical-boosted electrocatalytic CO2 reduction using Ni-partnered heteroatomic pairs," Nature Communications, Nature, vol. 15(1), pages 1-15, December.
    14. Juncai Dong & Yangyang Liu & Jiajing Pei & Haijing Li & Shufang Ji & Lei Shi & Yaning Zhang & Can Li & Cheng Tang & Jiangwen Liao & Shiqing Xu & Huabin Zhang & Qi Li & Shenlong Zhao, 2023. "Continuous electroproduction of formate via CO2 reduction on local symmetry-broken single-atom catalysts," Nature Communications, Nature, vol. 14(1), pages 1-13, December.
    15. Fenghui Ye & Shishi Zhang & Qingqing Cheng & Yongde Long & Dong Liu & Rajib Paul & Yunming Fang & Yaqiong Su & Liangti Qu & Liming Dai & Chuangang Hu, 2023. "The role of oxygen-vacancy in bifunctional indium oxyhydroxide catalysts for electrochemical coupling of biomass valorization with CO2 conversion," Nature Communications, Nature, vol. 14(1), pages 1-14, December.
    16. Jiahui Bi & Pengsong Li & Jiyuan Liu & Shuaiqiang Jia & Yong Wang & Qinggong Zhu & Zhimin Liu & Buxing Han, 2023. "Construction of 3D copper-chitosan-gas diffusion layer electrode for highly efficient CO2 electrolysis to C2+ alcohols," Nature Communications, Nature, vol. 14(1), pages 1-10, December.

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