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Silicon-chip-based mid-infrared dual-comb spectroscopy

Author

Listed:
  • Mengjie Yu

    (Columbia University
    Cornell University)

  • Yoshitomo Okawachi

    (Columbia University)

  • Austin G. Griffith

    (Cornell University)

  • Nathalie Picqué

    (Max-Planck-Institut für Quantenoptik
    Ludwig-Maximilians-Universität München, Fakultät für Physik
    CNRS, Univ. Paris-Sud, Université Paris-Saclay)

  • Michal Lipson

    (Columbia University)

  • Alexander L. Gaeta

    (Columbia University)

Abstract

The development of a spectroscopy device on a chip that could realize real-time fingerprinting with label-free and high-throughput detection of trace molecules represents one of the big challenges in sensing. Dual-comb spectroscopy (DCS) in the mid-infrared is a powerful technique offering high acquisition rates and signal-to-noise ratios through use of only a single detector with no moving parts. Here, we present a nanophotonic silicon-on-insulator platform designed for mid-infrared (mid-IR) DCS. A single continuous-wave low-power pump source generates two mutually coherent mode-locked frequency combs spanning from 2.6 to 4.1 μm in two silicon microresonators. A proof-of-principle experiment of vibrational absorption DCS in the liquid phase is achieved acquiring spectra of acetone spanning from 2900 to 3100 nm at 127-GHz (4.2-cm−1) resolution. These results represent a significant step towards a broadband, mid-IR spectroscopy instrument on a chip for liquid/condensed matter phase studies.

Suggested Citation

  • Mengjie Yu & Yoshitomo Okawachi & Austin G. Griffith & Nathalie Picqué & Michal Lipson & Alexander L. Gaeta, 2018. "Silicon-chip-based mid-infrared dual-comb spectroscopy," Nature Communications, Nature, vol. 9(1), pages 1-6, December.
    • Handle: RePEc:nat:natcom:v:9:y:2018:i:1:d:10.1038_s41467-018-04350-1
    DOI: 10.1038/s41467-018-04350-1
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    Cited by:

    1. Teng Tan & Zhongye Yuan & Hao Zhang & Guofeng Yan & Siyu Zhou & Ning An & Bo Peng & Giancarlo Soavi & Yunjiang Rao & Baicheng Yao, 2021. "Multispecies and individual gas molecule detection using Stokes solitons in a graphene over-modal microresonator," Nature Communications, Nature, vol. 12(1), pages 1-8, December.
    2. Chengying Bao & Zhiquan Yuan & Lue Wu & Myoung-Gyun Suh & Heming Wang & Qiang Lin & Kerry J. Vahala, 2021. "Architecture for microcomb-based GHz-mid-infrared dual-comb spectroscopy," Nature Communications, Nature, vol. 12(1), pages 1-8, December.
    3. Kaiheng Zou & Kai Pang & Hao Song & Jintao Fan & Zhe Zhao & Haoqian Song & Runzhou Zhang & Huibin Zhou & Amir Minoofar & Cong Liu & Xinzhou Su & Nanzhe Hu & Andrew McClung & Mahsa Torfeh & Amir Arbabi, 2022. "High-capacity free-space optical communications using wavelength- and mode-division-multiplexing in the mid-infrared region," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    4. Carolin P. Bauer & Zofia A. Bejm & Michelle K. Bollier & Justinas Pupeikis & Benjamin Willenberg & Ursula Keller & Christopher R. Phillips, 2024. "High-sensitivity dual-comb and cross-comb spectroscopy across the infrared using a widely tunable and free-running optical parametric oscillator," Nature Communications, Nature, vol. 15(1), pages 1-13, December.
    5. Rui Niu & Ming Li & Shuai Wan & Yu Robert Sun & Shui-Ming Hu & Chang-Ling Zou & Guang-Can Guo & Chun-Hua Dong, 2023. "kHz-precision wavemeter based on reconfigurable microsoliton," Nature Communications, Nature, vol. 14(1), pages 1-6, December.
    6. Daowang Peng & Chenglin Gu & Zhong Zuo & Yuanfeng Di & Xing Zou & Lulu Tang & Lunhua Deng & Daping Luo & Yang Liu & Wenxue Li, 2023. "Dual-comb optical activity spectroscopy for the analysis of vibrational optical activity induced by external magnetic field," Nature Communications, Nature, vol. 14(1), pages 1-11, December.
    7. Rebecca Cheng & Mengjie Yu & Amirhassan Shams-Ansari & Yaowen Hu & Christian Reimer & Mian Zhang & Marko Lončar, 2024. "Frequency comb generation via synchronous pumped χ(3) resonator on thin-film lithium niobate," Nature Communications, Nature, vol. 15(1), pages 1-7, December.
    8. Mingming Nie & Kunpeng Jia & Yijun Xie & Shining Zhu & Zhenda Xie & Shu-Wei Huang, 2022. "Synthesized spatiotemporal mode-locking and photonic flywheel in multimode mesoresonators," Nature Communications, Nature, vol. 13(1), pages 1-9, December.

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