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Strong angular and spectral narrowing of electroluminescence in an integrated Tamm-plasmon-driven halide perovskite LED

Author

Listed:
  • Zher Ying Ooi

    (University of Cambridge)

  • Alberto Jiménez-Solano

    (Max Planck Institute for Solid State Research
    Campus de Rabanales)

  • Krzysztof Gałkowski

    (University of Cambridge
    Nicolaus Copernicus University
    Wroclaw University of Science and Technology)

  • Yuqi Sun

    (University of Cambridge)

  • Jordi Ferrer Orri

    (University of Cambridge
    University of Cambridge)

  • Kyle Frohna

    (University of Cambridge)

  • Hayden Salway

    (University of Cambridge)

  • Simon Kahmann

    (University of Cambridge
    University of Cambridge)

  • Shenyu Nie

    (University of Cambridge)

  • Guadalupe Vega

    (Campus de Rabanales
    Calle Américo Vespucio 49)

  • Shaoni Kar

    (University of Cambridge)

  • Michał P. Nowak

    (Military University of Technology)

  • Sebastian Maćkowski

    (Nicolaus Copernicus University)

  • Piotr Nyga

    (Military University of Technology)

  • Caterina Ducati

    (University of Cambridge)

  • Neil C. Greenham

    (University of Cambridge)

  • Bettina V. Lotsch

    (Max Planck Institute for Solid State Research
    Ludwig-Maximilians-Universität (LMU)
    Lichtenbergstrasse 4a)

  • Miguel Anaya

    (University of Cambridge
    Calle Américo Vespucio 49)

  • Samuel D. Stranks

    (University of Cambridge
    University of Cambridge)

Abstract

Next-generation light-emitting applications such as displays and optical communications require judicious control over emitted light, including intensity and angular dispersion. To date, this remains a challenge as conventional methods require cumbersome optics. Here, we report highly directional and enhanced electroluminescence from a solution-processed quasi-2-dimensional halide perovskite light-emitting diode by building a device architecture to exploit hybrid plasmonic-photonic Tamm plasmon modes. By exploiting the processing and bandgap tunability of the halide perovskite device layers, we construct the device stack to optimise both optical and charge-injection properties, leading to narrow forward electroluminescence with an angular full-width half-maximum of 36.6° compared with the conventional isotropic control device of 143.9°, and narrow electroluminescence spectral full-width half-maximum of 12.1 nm. The device design is versatile and tunable to work with emission lines covering the visible spectrum with desired directionality, thus providing a promising route to modular, inexpensive, and directional operating light-emitting devices.

Suggested Citation

  • Zher Ying Ooi & Alberto Jiménez-Solano & Krzysztof Gałkowski & Yuqi Sun & Jordi Ferrer Orri & Kyle Frohna & Hayden Salway & Simon Kahmann & Shenyu Nie & Guadalupe Vega & Shaoni Kar & Michał P. Nowak &, 2024. "Strong angular and spectral narrowing of electroluminescence in an integrated Tamm-plasmon-driven halide perovskite LED," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
  • Handle: RePEc:nat:natcom:v:15:y:2024:i:1:d:10.1038_s41467-024-49838-1
    DOI: 10.1038/s41467-024-49838-1
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