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Heterodimensional Kondo superlattices with strong anisotropy

Author

Listed:
  • Qi Feng

    (Beijing Institute of Technology)

  • Junxi Duan

    (Beijing Institute of Technology)

  • Ping Wang

    (Beijing Institute of Technology)

  • Wei Jiang

    (Beijing Institute of Technology)

  • Huimin Peng

    (Beijing Institute of Technology)

  • Jinrui Zhong

    (Beijing Institute of Technology)

  • Jin Cao

    (Beijing Institute of Technology)

  • Yuqing Hu

    (Beijing Institute of Technology)

  • Qiuli Li

    (Beijing Institute of Technology)

  • Qinsheng Wang

    (Beijing Institute of Technology)

  • Jiadong Zhou

    (Beijing Institute of Technology)

  • Yugui Yao

    (Beijing Institute of Technology)

Abstract

Localized magnetic moments in non-magnetic materials, by interacting with the itinerary electrons, can profoundly change the metallic properties, developing various correlated phenomena such as the Kondo effect, heavy fermion, and unconventional superconductivity. In most Kondo systems, the localized moments are introduced through magnetic impurities. However, the intrinsic magnetic properties of materials can also be modulated by the dimensionality. Here, we report the observation of Kondo effect in a heterodimensional superlattice VS2-VS, in which arrays of the one-dimensional (1D) VS chains are encapsulated by two-dimensional VS2 layers. In such a heterodimensional Kondo superlattice, we observe the typical Kondo effect but with intriguing anisotropic field dependence. This unique anisotropy is determined to originate from the magnetic anisotropy which has the root in the unique 1D chains in the structure, as corroborated by the first-principles calculation. Our results open up a novel avenue of studying exotic correlated physics in heterodimensional materials.

Suggested Citation

  • Qi Feng & Junxi Duan & Ping Wang & Wei Jiang & Huimin Peng & Jinrui Zhong & Jin Cao & Yuqing Hu & Qiuli Li & Qinsheng Wang & Jiadong Zhou & Yugui Yao, 2024. "Heterodimensional Kondo superlattices with strong anisotropy," Nature Communications, Nature, vol. 15(1), pages 1-7, December.
    • Handle: RePEc:nat:natcom:v:15:y:2024:i:1:d:10.1038_s41467-024-49618-x
    DOI: 10.1038/s41467-024-49618-x
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    References listed on IDEAS

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    1. Qian Lv & Junyang Tan & Zhijie Wang & Peng Gu & Haiyun Liu & Lingxiao Yu & Yinping Wei & Lin Gan & Bilu Liu & Jia Li & Feiyu Kang & Hui-Ming Cheng & Qihua Xiong & Ruitao Lv, 2023. "Ultrafast charge transfer in mixed-dimensional WO3-x nanowire/WSe2 heterostructures for attomolar-level molecular sensing," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    2. D. Goldhaber-Gordon & Hadas Shtrikman & D. Mahalu & David Abusch-Magder & U. Meirav & M. A. Kastner, 1998. "Kondo effect in a single-electron transistor," Nature, Nature, vol. 391(6663), pages 156-159, January.
    3. Jiadong Zhou & Wenjie Zhang & Yung-Chang Lin & Jin Cao & Yao Zhou & Wei Jiang & Huifang Du & Bijun Tang & Jia Shi & Bingyan Jiang & Xun Cao & Bo Lin & Qundong Fu & Chao Zhu & Wei Guo & Yizhong Huang &, 2022. "Heterodimensional superlattice with in-plane anomalous Hall effect," Nature, Nature, vol. 609(7925), pages 46-51, September.
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