IDEAS home Printed from https://ideas.repec.org/a/nat/natcom/v14y2023i1d10.1038_s41467-023-41292-9.html
   My bibliography  Save this article

Photoluminescence imaging of single photon emitters within nanoscale strain profiles in monolayer WSe2

Author

Listed:
  • Artem N. Abramov

    (ITMO University)

  • Igor Y. Chestnov

    (ITMO University)

  • Ekaterina S. Alimova

    (Peter The Great St. Petersburg Polytechnic University)

  • Tatiana Ivanova

    (ITMO University)

  • Ivan S. Mukhin

    (ITMO University
    St. Petersburg Academic University)

  • Dmitry N. Krizhanovskii

    (University of Sheffield)

  • Ivan A. Shelykh

    (ITMO University
    University of Iceland
    Abrikosov Center for Theoretical Physics, MIPT
    Russian Quantum Center)

  • Ivan V. Iorsh

    (ITMO University
    Abrikosov Center for Theoretical Physics, MIPT
    Russian Quantum Center)

  • Vasily Kravtsov

    (ITMO University)

Abstract

Local deformation of atomically thin van der Waals materials provides a powerful approach to create site-controlled chip-compatible single-photon emitters (SPEs). However, the microscopic mechanisms underlying the formation of such strain-induced SPEs are still not fully clear, which hinders further efforts in their deterministic integration with nanophotonic structures for developing practical on-chip sources of quantum light. Here we investigate SPEs with single-photon purity up to 98% created in monolayer WSe2 via nanoindentation. Using photoluminescence imaging in combination with atomic force microscopy, we locate single-photon emitting sites on a deep sub-wavelength spatial scale and reconstruct the details of the surrounding local strain potential. The obtained results suggest that the origin of the observed single-photon emission is likely related to strain-induced spectral shift of dark excitonic states and their hybridization with localized states of individual defects.

Suggested Citation

  • Artem N. Abramov & Igor Y. Chestnov & Ekaterina S. Alimova & Tatiana Ivanova & Ivan S. Mukhin & Dmitry N. Krizhanovskii & Ivan A. Shelykh & Ivan V. Iorsh & Vasily Kravtsov, 2023. "Photoluminescence imaging of single photon emitters within nanoscale strain profiles in monolayer WSe2," Nature Communications, Nature, vol. 14(1), pages 1-7, December.
    • Handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-41292-9
    DOI: 10.1038/s41467-023-41292-9
    as

    Download full text from publisher

    File URL: https://www.nature.com/articles/s41467-023-41292-9
    File Function: Abstract
    Download Restriction: no
    File URL: https://libkey.io/10.1038/s41467-023-41292-9?utm_source=ideas
    LibKey link: if access is restricted and if your library uses this service, LibKey will redirect you to where you can use your library subscription to access this item
    ---><---

    References listed on IDEAS

    as
    1. Luca Sortino & Panaiot G. Zotev & Catherine L. Phillips & Alistair J. Brash & Javier Cambiasso & Elena Marensi & A. Mark Fox & Stefan A. Maier & Riccardo Sapienza & Alexander I. Tartakovskii, 2021. "Bright single photon emitters with enhanced quantum efficiency in a two-dimensional semiconductor coupled with dielectric nano-antennas," Nature Communications, Nature, vol. 12(1), pages 1-9, December.
    2. Artur Branny & Santosh Kumar & Raphaël Proux & Brian D Gerardot, 2017. "Deterministic strain-induced arrays of quantum emitters in a two-dimensional semiconductor," Nature Communications, Nature, vol. 8(1), pages 1-7, August.
    3. Luca Sapienza & Marcelo Davanço & Antonio Badolato & Kartik Srinivasan, 2015. "Nanoscale optical positioning of single quantum dots for bright and pure single-photon emission," Nature Communications, Nature, vol. 6(1), pages 1-8, November.
    4. Matteo Barbone & Alejandro R.-P. Montblanch & Dhiren M. Kara & Carmen Palacios-Berraquero & Alisson R. Cadore & Domenico De Fazio & Benjamin Pingault & Elaheh Mostaani & Han Li & Bin Chen & Kenji Wata, 2018. "Charge-tuneable biexciton complexes in monolayer WSe2," Nature Communications, Nature, vol. 9(1), pages 1-6, December.
    5. Kamyar Parto & Shaimaa I. Azzam & Kaustav Banerjee & Galan Moody, 2021. "Defect and strain engineering of monolayer WSe2 enables site-controlled single-photon emission up to 150 K," Nature Communications, Nature, vol. 12(1), pages 1-8, December.
    6. Carmen Palacios-Berraquero & Dhiren M. Kara & Alejandro R.-P. Montblanch & Matteo Barbone & Pawel Latawiec & Duhee Yoon & Anna K. Ott & Marko Loncar & Andrea C. Ferrari & Mete Atatüre, 2017. "Large-scale quantum-emitter arrays in atomically thin semiconductors," Nature Communications, Nature, vol. 8(1), pages 1-6, August.
    Full references (including those not matched with items on IDEAS)

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. Emanuil S. Yanev & Thomas P. Darlington & Sophia A. Ladyzhets & Matthew C. Strasbourg & Chiara Trovatello & Song Liu & Daniel A. Rhodes & Kobi Hall & Aditya Sinha & Nicholas J. Borys & James C. Hone &, 2024. "Programmable nanowrinkle-induced room-temperature exciton localization in monolayer WSe2," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    2. Pablo Hernández López & Sebastian Heeg & Christoph Schattauer & Sviatoslav Kovalchuk & Abhijeet Kumar & Douglas J. Bock & Jan N. Kirchhof & Bianca Höfer & Kyrylo Greben & Denis Yagodkin & Lukas Linhar, 2022. "Strain control of hybridization between dark and localized excitons in a 2D semiconductor," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    3. Luca Sortino & Panaiot G. Zotev & Catherine L. Phillips & Alistair J. Brash & Javier Cambiasso & Elena Marensi & A. Mark Fox & Stefan A. Maier & Riccardo Sapienza & Alexander I. Tartakovskii, 2021. "Bright single photon emitters with enhanced quantum efficiency in a two-dimensional semiconductor coupled with dielectric nano-antennas," Nature Communications, Nature, vol. 12(1), pages 1-9, December.
    4. Huan Zhao & Michael T. Pettes & Yu Zheng & Han Htoon, 2021. "Site-controlled telecom-wavelength single-photon emitters in atomically-thin MoTe2," Nature Communications, Nature, vol. 12(1), pages 1-7, December.
    5. M. Iqbal Bakti Utama & Hongfei Zeng & Tumpa Sadhukhan & Anushka Dasgupta & S. Carin Gavin & Riddhi Ananth & Dmitry Lebedev & Wei Wang & Jia-Shiang Chen & Kenji Watanabe & Takashi Taniguchi & Tobin J. , 2023. "Chemomechanical modification of quantum emission in monolayer WSe2," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    6. Longlong Yang & Yu Yuan & Bowen Fu & Jingnan Yang & Danjie Dai & Shushu Shi & Sai Yan & Rui Zhu & Xu Han & Hancong Li & Zhanchun Zuo & Can Wang & Yuan Huang & Kuijuan Jin & Qihuang Gong & Xiulai Xu, 2023. "Revealing broken valley symmetry of quantum emitters in WSe2 with chiral nanocavities," Nature Communications, Nature, vol. 14(1), pages 1-11, December.
    7. Wei Liu & Viktor Ivády & Zhi-Peng Li & Yuan-Ze Yang & Shang Yu & Yu Meng & Zhao-An Wang & Nai-Jie Guo & Fei-Fei Yan & Qiang Li & Jun-Feng Wang & Jin-Shi Xu & Xiao Liu & Zong-Quan Zhou & Yang Dong & Xi, 2022. "Coherent dynamics of multi-spin V $${}_{{{{{{{{\rm{B}}}}}}}}}^{-}$$ B − center in hexagonal boron nitride," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    8. Ryan J. Gelly & Dylan Renaud & Xing Liao & Benjamin Pingault & Stefan Bogdanovic & Giovanni Scuri & Kenji Watanabe & Takashi Taniguchi & Bernhard Urbaszek & Hongkun Park & Marko Lončar, 2022. "Probing dark exciton navigation through a local strain landscape in a WSe2 monolayer," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    9. Roberto Rosati & Robert Schmidt & Samuel Brem & Raül Perea-Causín & Iris Niehues & Johannes Kern & Johann A. Preuß & Robert Schneider & Steffen Michaelis de Vasconcellos & Rudolf Bratschitsch & Ermin , 2021. "Dark exciton anti-funneling in atomically thin semiconductors," Nature Communications, Nature, vol. 12(1), pages 1-7, December.
    10. Shuai Zhang & Baichang Li & Xinzhong Chen & Francesco L. Ruta & Yinming Shao & Aaron J. Sternbach & A. S. McLeod & Zhiyuan Sun & Lin Xiong & S. L. Moore & Xinyi Xu & Wenjing Wu & Sara Shabani & Lin Zh, 2022. "Nano-spectroscopy of excitons in atomically thin transition metal dichalcogenides," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    11. Song Li & Gergő Thiering & Péter Udvarhelyi & Viktor Ivády & Adam Gali, 2022. "Carbon defect qubit in two-dimensional WS2," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    12. Stuart J. Masson & Ana Asenjo-Garcia, 2022. "Universality of Dicke superradiance in arrays of quantum emitters," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    13. N. Fang & Y. R. Chang & S. Fujii & D. Yamashita & M. Maruyama & Y. Gao & C. F. Fong & D. Kozawa & K. Otsuka & K. Nagashio & S. Okada & Y. K. Kato, 2024. "Room-temperature quantum emission from interface excitons in mixed-dimensional heterostructures," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    14. Paweł Holewa & Daniel A. Vajner & Emilia Zięba-Ostój & Maja Wasiluk & Benedek Gaál & Aurimas Sakanas & Marek Burakowski & Paweł Mrowiński & Bartosz Krajnik & Meng Xiong & Kresten Yvind & Niels Gregers, 2024. "High-throughput quantum photonic devices emitting indistinguishable photons in the telecom C-band," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    15. Le Zhang & Han Wang & Xinrong Zong & Yongheng Zhou & Taihong Wang & Lin Wang & Xiaolong Chen, 2022. "Probing interlayer shear thermal deformation in atomically-thin van der Waals layered materials," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    16. Kai-Qiang Lin & Jonas D. Ziegler & Marina A. Semina & Javid V. Mamedov & Kenji Watanabe & Takashi Taniguchi & Sebastian Bange & Alexey Chernikov & Mikhail M. Glazov & John M. Lupton, 2022. "High-lying valley-polarized trions in 2D semiconductors," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    17. Hongbing Cai & Abdullah Rasmita & Qinghai Tan & Jia-Min Lai & Ruihua He & Xiangbin Cai & Yan Zhao & Disheng Chen & Naizhou Wang & Zhao Mu & Zumeng Huang & Zhaowei Zhang & John J. H. Eng & Yuanda Liu &, 2023. "Interlayer donor-acceptor pair excitons in MoSe2/WSe2 moiré heterobilayer," Nature Communications, Nature, vol. 14(1), pages 1-7, December.
    18. Xiaotong Chen & Zhen Lian & Yuze Meng & Lei Ma & Su-Fei Shi, 2023. "Excitonic Complexes in Two-Dimensional Transition Metal Dichalcogenides," Nature Communications, Nature, vol. 14(1), pages 1-5, December.
    19. Jack B. Muir & Jesper Levinsen & Stuart K. Earl & Mitchell A. Conway & Jared H. Cole & Matthias Wurdack & Rishabh Mishra & David J. Ing & Eliezer Estrecho & Yuerui Lu & Dmitry K. Efimkin & Jonathan O., 2022. "Interactions between Fermi polarons in monolayer WS2," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    20. Raj Pandya & Richard Y. S. Chen & Qifei Gu & Jooyoung Sung & Christoph Schnedermann & Oluwafemi S. Ojambati & Rohit Chikkaraddy & Jeffrey Gorman & Gianni Jacucci & Olimpia D. Onelli & Tom Willhammar &, 2021. "Microcavity-like exciton-polaritons can be the primary photoexcitation in bare organic semiconductors," Nature Communications, Nature, vol. 12(1), pages 1-11, December.

    More about this item

    Statistics

    Access and download statistics

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-41292-9. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: Sonal Shukla or Springer Nature Abstracting and Indexing (email available below). General contact details of provider: http://www.nature.com .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.