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Conductance stable and mechanically durable bi-layer EGaIn composite-coated stretchable fiber for 1D bioelectronics

Author

Listed:
  • Gun-Hee Lee

    (Korea Advanced Institute of Science and Technology (KAIST)
    Korea Advanced Institute of Science and Technology (KAIST)
    Korea Advanced Institute of Science and Technology (KAIST))

  • Do Hoon Lee

    (Korea Advanced Institute of Science and Technology (KAIST))

  • Woojin Jeon

    (Korea Advanced Institute of Science and Technology (KAIST))

  • Jihwan Yoon

    (Seoul National University)

  • Kwangguk Ahn

    (Seoul National University)

  • Kum Seok Nam

    (Korea Advanced Institute of Science and Technology (KAIST))

  • Min Kim

    (Korea Advanced Institute of Science and Technology (KAIST))

  • Jun Kyu Kim

    (Korea Advanced Institute of Science and Technology (KAIST))

  • Yong Hoe Koo

    (Ulsan National Institute of Science and Technology (UNIST))

  • Jinmyoung Joo

    (Ulsan National Institute of Science and Technology (UNIST))

  • WooChul Jung

    (Korea Advanced Institute of Science and Technology (KAIST))

  • Jaehong Lee

    (Daegu Gyeongbuk Institute of Science and Technology (DGIST))

  • Jaewook Nam

    (Seoul National University)

  • Seongjun Park

    (Korea Advanced Institute of Science and Technology (KAIST)
    KAIST Institute for Health Science and Technology
    KAIST Institute for NanoCentury)

  • Jae-Woong Jeong

    (Korea Advanced Institute of Science and Technology (KAIST)
    KAIST Institute for Health Science and Technology)

  • Steve Park

    (Korea Advanced Institute of Science and Technology (KAIST)
    KAIST Institute for Health Science and Technology
    KAIST Institute for NanoCentury)

Abstract

Deformable semi-solid liquid metal particles (LMP) have emerged as a promising substitute for rigid conductive fillers due to their excellent electrical properties and stable conductance under strain. However, achieving a compact and robust coating of LMP on fibers remains a persistent challenge, mainly due to the incompatibility of conventional coating techniques with LMP. Additionally, the limited durability and absence of initial electrical conductivity of LMP restrict their widespread application. In this study, we propose a solution process that robustly and compactly assembles mechanically durable and initially conductive LMP on fibers. Specifically, we present a shearing-based deposition of polymer-attached LMP followed by additional coating with CNT-attached LMP to create bi-layer LMP composite with exceptional durability, electrical conductivity, stretchability, and biocompatibility on various fibers. The versatility and reliability of this manufacturing strategy for 1D electronics are demonstrated through the development of sewn electrical circuits, smart clothes, stretchable biointerfaced fiber, and multifunctional fiber probes.

Suggested Citation

  • Gun-Hee Lee & Do Hoon Lee & Woojin Jeon & Jihwan Yoon & Kwangguk Ahn & Kum Seok Nam & Min Kim & Jun Kyu Kim & Yong Hoe Koo & Jinmyoung Joo & WooChul Jung & Jaehong Lee & Jaewook Nam & Seongjun Park & , 2023. "Conductance stable and mechanically durable bi-layer EGaIn composite-coated stretchable fiber for 1D bioelectronics," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    • Handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-39928-x
    DOI: 10.1038/s41467-023-39928-x
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    References listed on IDEAS

    as
    1. Gun-Hee Lee & Ye Rim Lee & Hanul Kim & Do A Kwon & Hyeonji Kim & Congqi Yang & Siyoung Q. Choi & Seongjun Park & Jae-Woong Jeong & Steve Park, 2022. "Rapid meniscus-guided printing of stable semi-solid-state liquid metal microgranular-particle for soft electronics," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    2. Yoonseob Kim & Jian Zhu & Bongjun Yeom & Matthew Di Prima & Xianli Su & Jin-Gyu Kim & Seung Jo Yoo & Ctirad Uher & Nicholas A. Kotov, 2013. "Stretchable nanoparticle conductors with self-organized conductive pathways," Nature, Nature, vol. 500(7460), pages 59-63, August.
    3. Naoji Matsuhisa & Martin Kaltenbrunner & Tomoyuki Yokota & Hiroaki Jinno & Kazunori Kuribara & Tsuyoshi Sekitani & Takao Someya, 2015. "Printable elastic conductors with a high conductivity for electronic textile applications," Nature Communications, Nature, vol. 6(1), pages 1-11, November.
    4. Xiaodan Gu & Leo Shaw & Kevin Gu & Michael F. Toney & Zhenan Bao, 2018. "The meniscus-guided deposition of semiconducting polymers," Nature Communications, Nature, vol. 9(1), pages 1-16, December.
    5. Pedro Alhais Lopes & Bruno C. Santos & Anibal T. Almeida & Mahmoud Tavakoli, 2021. "Reversible polymer-gel transition for ultra-stretchable chip-integrated circuits through self-soldering and self-coating and self-healing," Nature Communications, Nature, vol. 12(1), pages 1-10, December.
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