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Staggered circular nanoporous graphene converts electromagnetic waves into electricity

Author

Listed:
  • Hualiang Lv

    (The Ohio State University)

  • Yuxing Yao

    (California Institute of Technology)

  • Shucong Li

    (Harvard University)

  • Guanglei Wu

    (Fudan University
    Qingdao University)

  • Biao Zhao

    (Fudan University
    Fudan University)

  • Xiaodi Zhou

    (The Ohio State University)

  • Robert L. Dupont

    (The Ohio State University)

  • Ufuoma I. Kara

    (The Ohio State University)

  • Yimin Zhou

    (University of Michigan)

  • Shibo Xi

    (Institute of Chemical and Engineering Sciences, A*STAR)

  • Bo Liu

    (Hunan University)

  • Renchao Che

    (Fudan University
    Fudan University
    Zhejiang Laboratory)

  • Jincang Zhang

    (Zhejiang Laboratory)

  • Hongbin Xu

    (Massachusetts Institute of Technology)

  • Solomon Adera

    (University of Michigan)

  • Renbing Wu

    (Fudan University)

  • Xiaoguang Wang

    (The Ohio State University
    Sustainability Institute, The Ohio State University)

Abstract

Harvesting largely ignored and wasted electromagnetic (EM) energy released by electronic devices and converting it into direct current (DC) electricity is an attractive strategy not only to reduce EM pollution but also address the ever-increasing energy crisis. Here we report the synthesis of nanoparticle-templated graphene with monodisperse and staggered circular nanopores enabling an EM–heat–DC conversion pathway. We experimentally and theoretically demonstrate that this staggered nanoporous structure alters graphene’s electronic and phononic properties by synergistically manipulating its intralayer nanostructures and interlayer interactions. The staggered circular nanoporous graphene exhibits an anomalous combination of properties, which lead to an efficient absorption and conversion of EM waves into heat and in turn an output of DC electricity through the thermoelectric effect. Overall, our results advance the fundamental understanding of the structure–property relationships of ordered nanoporous graphene, providing an effective strategy to reduce EM pollution and generate electric energy.

Suggested Citation

  • Hualiang Lv & Yuxing Yao & Shucong Li & Guanglei Wu & Biao Zhao & Xiaodi Zhou & Robert L. Dupont & Ufuoma I. Kara & Yimin Zhou & Shibo Xi & Bo Liu & Renchao Che & Jincang Zhang & Hongbin Xu & Solomon , 2023. "Staggered circular nanoporous graphene converts electromagnetic waves into electricity," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
  • Handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-37436-6
    DOI: 10.1038/s41467-023-37436-6
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    References listed on IDEAS

    as
    1. Jeong Min Park & Yuan Cao & Kenji Watanabe & Takashi Taniguchi & Pablo Jarillo-Herrero, 2021. "Tunable strongly coupled superconductivity in magic-angle twisted trilayer graphene," Nature, Nature, vol. 590(7845), pages 249-255, February.
    2. Rahul Mukherjee & Abhay V. Thomas & Dibakar Datta & Eklavya Singh & Junwen Li & Osman Eksik & Vivek B. Shenoy & Nikhil Koratkar, 2014. "Defect-induced plating of lithium metal within porous graphene networks," Nature Communications, Nature, vol. 5(1), pages 1-10, September.
    3. Andreij C. Gadelha & Douglas A. A. Ohlberg & Cassiano Rabelo & Eliel G. S. Neto & Thiago L. Vasconcelos & João L. Campos & Jessica S. Lemos & Vinícius Ornelas & Daniel Miranda & Rafael Nadas & Fabiano, 2021. "Localization of lattice dynamics in low-angle twisted bilayer graphene," Nature, Nature, vol. 590(7846), pages 405-409, February.
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