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Selective and rapid extraction of trace amount of gold from complex liquids with silver(I)-organic frameworks

Author

Listed:
  • Jie Luo

    (Jinan University)

  • Xiao Luo

    (Jinan University)

  • Mo Xie

    (Jinan University)

  • Hao-Zhen Li

    (Jinan University)

  • Haiyan Duan

    (Jinan University)

  • Hou-Gan Zhou

    (Jinan University)

  • Rong-Jia Wei

    (Jinan University)

  • Guo-Hong Ning

    (Jinan University)

  • Dan Li

    (Jinan University)

Abstract

The design of adsorbents for rapid, selective extraction of ultra-trace amounts of gold from complex liquids is desirable from both an environmental and economical point of view. However, the development of such materials remains challenging. Herein, we report the fabrication of two vinylene-linked two-dimensional silver(I)-organic frameworks prepared via Knoevenagel condensation. This material enables selective sensing of gold with a low limit of detection of 60 ppb, as well as selective uptake of ultra-trace gold from complex aqueous mixtures including distilled water with 15 competing metal ions, leaching solution of electronic waste (e-waste), wastewater, and seawater. The present adsorbent delivers a gold adsorption capacity of 954 mg g−1, excellent selectivity and reusability, and can rapidly and selectively extract ultra-trace gold from seawater down to ~20 ppb (94% removal in 10 minutes). In addition, the purity of recovered gold from e-waste reaches 23.8 Karat (99.17% pure).

Suggested Citation

  • Jie Luo & Xiao Luo & Mo Xie & Hao-Zhen Li & Haiyan Duan & Hou-Gan Zhou & Rong-Jia Wei & Guo-Hong Ning & Dan Li, 2022. "Selective and rapid extraction of trace amount of gold from complex liquids with silver(I)-organic frameworks," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-35467-z
    DOI: 10.1038/s41467-022-35467-z
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    References listed on IDEAS

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    1. Luke M. M. Kinsman & Bryne T. Ngwenya & Carole A. Morrison & Jason B. Love, 2021. "Tuneable separation of gold by selective precipitation using a simple and recyclable diamide," Nature Communications, Nature, vol. 12(1), pages 1-8, December.
    2. Yao Chen & Mengjiao Xu & Jieya Wen & Yu Wan & Qingfei Zhao & Xia Cao & Yong Ding & Zhong Lin Wang & Hexing Li & Zhenfeng Bian, 2021. "Selective recovery of precious metals through photocatalysis," Nature Sustainability, Nature, vol. 4(7), pages 618-626, July.
    3. Eric Williams, 2011. "Environmental effects of information and communications technologies," Nature, Nature, vol. 479(7373), pages 354-358, November.
    4. Zhichang Liu & Marco Frasconi & Juying Lei & Zachary J. Brown & Zhixue Zhu & Dennis Cao & Julien Iehl & Guoliang Liu & Albert C. Fahrenbach & Youssry Y. Botros & Omar K. Farha & Joseph T. Hupp & Chad , 2013. "Selective isolation of gold facilitated by second-sphere coordination with α-cyclodextrin," Nature Communications, Nature, vol. 4(1), pages 1-9, October.
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    Cited by:

    1. Yu-Xin Chen & Haidong Yu & Lihua Wu & Yuan-Jun Tong & Jianqiao Xu & Huan Pang & Chao Wu & Tian Tian & Gangfeng Ouyang, 2024. "Unlocking multi-photon excited luminescence in pyrazolate trinuclear gold clusters for dynamic cell imaging," Nature Communications, Nature, vol. 15(1), pages 1-14, December.
    2. Kaixing Fu & Xia Liu & Xiaolin Zhang & Shiqing Zhou & Nanwen Zhu & Yong Pei & Jinming Luo, 2024. "Utilizing cost-effective pyrocarbon for highly efficient gold retrieval from e-waste leachate," Nature Communications, Nature, vol. 15(1), pages 1-13, December.

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