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Dust emission reduction enhanced gas-to-particle conversion of ammonia in the North China Plain

Author

Listed:
  • Yongchun Liu

    (Beijing University of Chemical Technology)

  • Junlei Zhan

    (Beijing University of Chemical Technology)

  • Feixue Zheng

    (Beijing University of Chemical Technology)

  • Boying Song

    (Beijing University of Chemical Technology)

  • Yusheng Zhang

    (Beijing University of Chemical Technology)

  • Wei Ma

    (Beijing University of Chemical Technology)

  • Chenjie Hua

    (Beijing University of Chemical Technology)

  • Jiali Xie

    (Beijing University of Chemical Technology)

  • Xiaolei Bao

    (Hebei Chemical & Pharmaceutical College
    Hebei Provincial Academy of Environmental Sciences)

  • Chao Yan

    (University of Helsinki
    Nanjing University)

  • Federico Bianchi

    (University of Helsinki)

  • Tuukka Petäjä

    (Beijing University of Chemical Technology
    University of Helsinki
    Nanjing University)

  • Aijun Ding

    (Nanjing University)

  • Yu Song

    (Peking University)

  • Hong He

    (Chinese Academy of Sciences)

  • Markku Kulmala

    (Beijing University of Chemical Technology
    University of Helsinki)

Abstract

Ammonium salt is an important component of particulate matter with aerodynamic diameter less than 2.5 µm (PM2.5) and has significant impacts on air quality, climate, and natural ecosystems. However, a fundamental understanding of the conversion kinetics from ammonia to ammonium in unique environments of high aerosol loading is lacking. Here, we report the uptake coefficient of ammonia (γNH3) on ambient PM2.5 varying from 2.2 × 10−4 to 6.0 × 10−4 in the North China Plain. It is significantly lower than those on the model particles under simple conditions reported in the literature. The probability-weighted γNH3 increases obviously, which is well explained by the annual decrease in aerosol pH due to the significant decline in alkali and alkali earth metal contents from the emission source of dust. Our results elaborate on the complex interactions between primary emissions and the secondary formation of aerosols and the important role of dust in atmospheric chemistry.

Suggested Citation

  • Yongchun Liu & Junlei Zhan & Feixue Zheng & Boying Song & Yusheng Zhang & Wei Ma & Chenjie Hua & Jiali Xie & Xiaolei Bao & Chao Yan & Federico Bianchi & Tuukka Petäjä & Aijun Ding & Yu Song & Hong He , 2022. "Dust emission reduction enhanced gas-to-particle conversion of ammonia in the North China Plain," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
  • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-34733-4
    DOI: 10.1038/s41467-022-34733-4
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    References listed on IDEAS

    as
    1. Rong Ma & Ke Li & Yixin Guo & Bo Zhang & Xueli Zhao & Soeren Linder & ChengHe Guan & Guoqian Chen & Yujie Gan & Jing Meng, 2021. "Mitigation potential of global ammonia emissions and related health impacts in the trade network," Nature Communications, Nature, vol. 12(1), pages 1-13, December.
    2. Xuejun Liu & Ying Zhang & Wenxuan Han & Aohan Tang & Jianlin Shen & Zhenling Cui & Peter Vitousek & Jan Willem Erisman & Keith Goulding & Peter Christie & Andreas Fangmeier & Fusuo Zhang, 2013. "Enhanced nitrogen deposition over China," Nature, Nature, vol. 494(7438), pages 459-462, February.
    3. João Almeida & Siegfried Schobesberger & Andreas Kürten & Ismael K. Ortega & Oona Kupiainen-Määttä & Arnaud P. Praplan & Alexey Adamov & Antonio Amorim & Federico Bianchi & Martin Breitenlechner & And, 2013. "Molecular understanding of sulphuric acid–amine particle nucleation in the atmosphere," Nature, Nature, vol. 502(7471), pages 359-363, October.
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