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Direct production of olefins from syngas with ultrahigh carbon efficiency

Author

Listed:
  • Hailing Yu

    (Chinese Academy of Sciences
    University of the Chinese Academy of Sciences)

  • Caiqi Wang

    (Chinese Academy of Sciences
    University of the Chinese Academy of Sciences)

  • Tiejun Lin

    (Chinese Academy of Sciences)

  • Yunlei An

    (Chinese Academy of Sciences)

  • Yuchen Wang

    (Chinese Academy of Sciences
    ShanghaiTech University)

  • Qingyu Chang

    (Chinese Academy of Sciences)

  • Fei Yu

    (Chinese Academy of Sciences)

  • Yao Wei

    (University of the Chinese Academy of Sciences
    Chinese Academy of Sciences)

  • Fanfei Sun

    (Chinese Academy of Sciences)

  • Zheng Jiang

    (Chinese Academy of Sciences)

  • Shenggang Li

    (Chinese Academy of Sciences
    ShanghaiTech University)

  • Yuhan Sun

    (Chinese Academy of Sciences
    ShanghaiTech University)

  • Liangshu Zhong

    (Chinese Academy of Sciences
    ShanghaiTech University)

Abstract

Syngas conversion serves as a competitive strategy to produce olefins chemicals from nonpetroleum resources. However, the goal to achieve desirable olefins selectivity with limited undesired C1 by-products remains a grand challenge. Herein, we present a non-classical Fischer-Tropsch to olefins process featuring high carbon efficiency that realizes 80.1% olefins selectivity with ultralow total selectivity of CH4 and CO2 (

Suggested Citation

  • Hailing Yu & Caiqi Wang & Tiejun Lin & Yunlei An & Yuchen Wang & Qingyu Chang & Fei Yu & Yao Wei & Fanfei Sun & Zheng Jiang & Shenggang Li & Yuhan Sun & Liangshu Zhong, 2022. "Direct production of olefins from syngas with ultrahigh carbon efficiency," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-33715-w
    DOI: 10.1038/s41467-022-33715-w
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    References listed on IDEAS

    as
    1. Yaru Zhang & Xiaoli Yang & Xiaofeng Yang & Hongmin Duan & Haifeng Qi & Yang Su & Binglian Liang & Huabing Tao & Bin Liu & De Chen & Xiong Su & Yanqiang Huang & Tao Zhang, 2020. "Tuning reactivity of Fischer–Tropsch synthesis by regulating TiOx overlayer over Ru/TiO2 nanocatalysts," Nature Communications, Nature, vol. 11(1), pages 1-8, December.
    2. Jingxiu Xie & Pasi P. Paalanen & Tom W. van Deelen & Bert M. Weckhuysen & Manuel J. Louwerse & Krijn P. de Jong, 2019. "Promoted cobalt metal catalysts suitable for the production of lower olefins from natural gas," Nature Communications, Nature, vol. 10(1), pages 1-10, December.
    3. Jun Zhou & Zhe Gao & Guolei Xiang & Tianyu Zhai & Zikai Liu & Weixin Zhao & Xin Liang & Leyu Wang, 2022. "Interfacial compatibility critically controls Ru/TiO2 metal-support interaction modes in CO2 hydrogenation," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
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