IDEAS home Printed from https://ideas.repec.org/a/nat/natcom/v13y2022i1d10.1038_s41467-022-31553-4.html
   My bibliography  Save this article

Ion-cluster-mediated ultrafast self-healable ionoconductors for reconfigurable electronics

Author

Listed:
  • Yong Min Kim

    (University of Seoul)

  • Jin Han Kwon

    (University of Seoul)

  • Seonho Kim

    (Inha University)

  • U Hyeok Choi

    (Inha University)

  • Hong Chul Moon

    (University of Seoul)

Abstract

Implementing self-healing capabilities in a deformable platform is one of the critical challenges for achieving future wearable electronics with high durability and reliability. Conventional systems are mostly based on polymeric materials, so their self-healing usually proceeds at elevated temperatures to promote chain flexibility and reduce healing time. Here, we propose an ion-cluster-driven self-healable ionoconductor composed of rationally designed copolymers and ionic liquids. After complete cleavage, the ionoconductor can be repaired with high efficiency (∼90.3%) within 1 min even at 25 °C, which is mainly attributed to the dynamic formation of ion clusters between the charged moieties in copolymers and ionic liquids. By taking advantages of the superior self-healing performance, stretchability (∼1130%), non-volatility (over 6 months), and ability to be easily shaped as desired through cutting and re-assembly protocol, reconfigurable, deformable light-emitting electroluminescent displays are successfully demonstrated as promising electronic platforms for future applications.

Suggested Citation

  • Yong Min Kim & Jin Han Kwon & Seonho Kim & U Hyeok Choi & Hong Chul Moon, 2022. "Ion-cluster-mediated ultrafast self-healable ionoconductors for reconfigurable electronics," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-31553-4
    DOI: 10.1038/s41467-022-31553-4
    as

    Download full text from publisher

    File URL: https://www.nature.com/articles/s41467-022-31553-4
    File Function: Abstract
    Download Restriction: no
    File URL: https://libkey.io/10.1038/s41467-022-31553-4?utm_source=ideas
    LibKey link: if access is restricted and if your library uses this service, LibKey will redirect you to where you can use your library subscription to access this item
    ---><---

    References listed on IDEAS

    as
    1. Jason F. Patrick & Maxwell J. Robb & Nancy R. Sottos & Jeffrey S. Moore & Scott R. White, 2016. "Polymers with autonomous life-cycle control," Nature, Nature, vol. 540(7633), pages 363-370, December.
    2. Youngho Eom & Seon-Mi Kim & Minkyung Lee & Hyeonyeol Jeon & Jaeduk Park & Eun Seong Lee & Sung Yeon Hwang & Jeyoung Park & Dongyeop X. Oh, 2021. "Mechano-responsive hydrogen-bonding array of thermoplastic polyurethane elastomer captures both strength and self-healing," Nature Communications, Nature, vol. 12(1), pages 1-11, December.
    3. Yicheng Zhao & Jing Wei & Heng Li & Yin Yan & Wenke Zhou & Dapeng Yu & Qing Zhao, 2016. "A polymer scaffold for self-healing perovskite solar cells," Nature Communications, Nature, vol. 7(1), pages 1-9, April.
    Full references (including those not matched with items on IDEAS)

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. Zengqi Huang & Lin Li & Tingqing Wu & Tangyue Xue & Wei Sun & Qi Pan & Huadong Wang & Hongfei Xie & Jimei Chi & Teng Han & Xiaotian Hu & Meng Su & Yiwang Chen & Yanlin Song, 2023. "Wearable perovskite solar cells by aligned liquid crystal elastomers," Nature Communications, Nature, vol. 14(1), pages 1-11, December.
    2. Alexander D. Snyder & Zachary J. Phillips & Jack S. Turicek & Charles E. Diesendruck & Kalyana B. Nakshatrala & Jason F. Patrick, 2022. "Prolonged in situ self-healing in structural composites via thermo-reversible entanglement," Nature Communications, Nature, vol. 13(1), pages 1-12, December.
    3. Wenle Li & Xiaocun Lu & Jacob M. Diamond & Chengtian Shen & Bo Jiang & Shi Sun & Jeffrey S. Moore & Nancy R. Sottos, 2024. "Photo-modulated activation of organic bases enabling microencapsulation and on-demand reactivity," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    4. Shuxian Du & Hao Huang & Zhineng Lan & Peng Cui & Liang Li & Min Wang & Shujie Qu & Luyao Yan & Changxu Sun & Yingying Yang & Xinxin Wang & Meicheng Li, 2024. "Inhibiting perovskite decomposition by a creeper-inspired strategy enables efficient and stable perovskite solar cells," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    5. Shoieb Shaik & Ziyou Zhou & Zhongliang Ouyang & Rebecca Han & Dawen Li, 2021. "Polymer Additive Assisted Fabrication of Compact and Ultra-Smooth Perovskite Thin Films with Fast Lamp Annealing," Energies, MDPI, vol. 14(9), pages 1-10, May.
    6. Pao-Hsun Huang & Yeong-Her Wang & Jhong-Ciao Ke & Chien-Jung Huang, 2017. "The Effect of Solvents on the Performance of CH 3 NH 3 PbI 3 Perovskite Solar Cells," Energies, MDPI, vol. 10(5), pages 1-8, April.
    7. Zhihao Li & Chunmei Jia & Zhi Wan & Jiayi Xue & Junchao Cao & Meng Zhang & Can Li & Jianghua Shen & Chao Zhang & Zhen Li, 2023. "Hyperbranched polymer functionalized flexible perovskite solar cells with mechanical robustness and reduced lead leakage," Nature Communications, Nature, vol. 14(1), pages 1-12, December.
    8. Jamal, M.S. & Bashar, M.S. & Hasan, A.K. Mahmud & Almutairi, Zeyad A. & Alharbi, Hamad F. & Alharthi, Nabeel H. & Karim, Mohammad R. & Misran, H. & Amin, Nowshad & Sopian, Kamaruzzaman Bin & Akhtaruzz, 2018. "Fabrication techniques and morphological analysis of perovskite absorber layer for high-efficiency perovskite solar cell: A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 98(C), pages 469-488.
    9. FuYao Sun & LongFei Liu & Tong Liu & XueBin Wang & Qi Qi & ZuSheng Hang & Kai Chen & JianHua Xu & JiaJun Fu, 2023. "Vascular smooth muscle-inspired architecture enables soft yet tough self-healing materials for durable capacitive strain-sensor," Nature Communications, Nature, vol. 14(1), pages 1-12, December.
    10. Chee, A. Kuan-Way, 2023. "On current technology for light absorber materials used in highly efficient industrial solar cells," Renewable and Sustainable Energy Reviews, Elsevier, vol. 173(C).

    More about this item

    Statistics

    Access and download statistics

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-31553-4. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: Sonal Shukla or Springer Nature Abstracting and Indexing (email available below). General contact details of provider: http://www.nature.com .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.