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A polymer scaffold for self-healing perovskite solar cells

Author

Listed:
  • Yicheng Zhao

    (State Key Laboratory for Mesoscopic Physics, School of Physics, Peking University
    Collaborative Innovation Center of Quantum Matter)

  • Jing Wei

    (State Key Laboratory for Mesoscopic Physics, School of Physics, Peking University
    Collaborative Innovation Center of Quantum Matter)

  • Heng Li

    (State Key Laboratory for Mesoscopic Physics, School of Physics, Peking University
    Collaborative Innovation Center of Quantum Matter)

  • Yin Yan

    (State Key Laboratory for Mesoscopic Physics, School of Physics, Peking University
    Collaborative Innovation Center of Quantum Matter)

  • Wenke Zhou

    (State Key Laboratory for Mesoscopic Physics, School of Physics, Peking University
    Collaborative Innovation Center of Quantum Matter)

  • Dapeng Yu

    (State Key Laboratory for Mesoscopic Physics, School of Physics, Peking University
    Collaborative Innovation Center of Quantum Matter)

  • Qing Zhao

    (State Key Laboratory for Mesoscopic Physics, School of Physics, Peking University
    Collaborative Innovation Center of Quantum Matter)

Abstract

Advancing of the lead halide perovskite solar cells towards photovoltaic market demands large-scale devices of high-power conversion efficiency, high reproducibility and stability via low-cost fabrication technology, and in particular resistance to humid environment for long-time operation. Here we achieve uniform perovskite film based on a novel polymer-scaffold architecture via a mild-temperature process. These solar cells exhibit efficiency of up to ∼16% with small variation. The unencapsulated devices retain high output for up to 300 h in highly humid environment (70% relative humidity). Moreover, they show strong humidity resistant and self-healing behaviour, recovering rapidly after removing from water vapour. Not only the film can self-heal in this case, but the corresponding devices can present power conversion efficiency recovery after the water vapour is removed. Our work demonstrates the value of cheap, long chain and hygroscopic polymer scaffold in perovskite solar cells towards commercialization.

Suggested Citation

  • Yicheng Zhao & Jing Wei & Heng Li & Yin Yan & Wenke Zhou & Dapeng Yu & Qing Zhao, 2016. "A polymer scaffold for self-healing perovskite solar cells," Nature Communications, Nature, vol. 7(1), pages 1-9, April.
    • Handle: RePEc:nat:natcom:v:7:y:2016:i:1:d:10.1038_ncomms10228
    DOI: 10.1038/ncomms10228
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    Cited by:

    1. Yong Min Kim & Jin Han Kwon & Seonho Kim & U Hyeok Choi & Hong Chul Moon, 2022. "Ion-cluster-mediated ultrafast self-healable ionoconductors for reconfigurable electronics," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    2. Jamal, M.S. & Bashar, M.S. & Hasan, A.K. Mahmud & Almutairi, Zeyad A. & Alharbi, Hamad F. & Alharthi, Nabeel H. & Karim, Mohammad R. & Misran, H. & Amin, Nowshad & Sopian, Kamaruzzaman Bin & Akhtaruzz, 2018. "Fabrication techniques and morphological analysis of perovskite absorber layer for high-efficiency perovskite solar cell: A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 98(C), pages 469-488.
    3. Pao-Hsun Huang & Yeong-Her Wang & Jhong-Ciao Ke & Chien-Jung Huang, 2017. "The Effect of Solvents on the Performance of CH 3 NH 3 PbI 3 Perovskite Solar Cells," Energies, MDPI, vol. 10(5), pages 1-8, April.
    4. Chee, A. Kuan-Way, 2023. "On current technology for light absorber materials used in highly efficient industrial solar cells," Renewable and Sustainable Energy Reviews, Elsevier, vol. 173(C).
    5. Zengqi Huang & Lin Li & Tingqing Wu & Tangyue Xue & Wei Sun & Qi Pan & Huadong Wang & Hongfei Xie & Jimei Chi & Teng Han & Xiaotian Hu & Meng Su & Yiwang Chen & Yanlin Song, 2023. "Wearable perovskite solar cells by aligned liquid crystal elastomers," Nature Communications, Nature, vol. 14(1), pages 1-11, December.
    6. Shuxian Du & Hao Huang & Zhineng Lan & Peng Cui & Liang Li & Min Wang & Shujie Qu & Luyao Yan & Changxu Sun & Yingying Yang & Xinxin Wang & Meicheng Li, 2024. "Inhibiting perovskite decomposition by a creeper-inspired strategy enables efficient and stable perovskite solar cells," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    7. Shoieb Shaik & Ziyou Zhou & Zhongliang Ouyang & Rebecca Han & Dawen Li, 2021. "Polymer Additive Assisted Fabrication of Compact and Ultra-Smooth Perovskite Thin Films with Fast Lamp Annealing," Energies, MDPI, vol. 14(9), pages 1-10, May.

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