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Perovskite microcells fabricated using swelling-induced crack propagation for colored solar windows

Author

Listed:
  • Woongchan Lee

    (Institute for Basic Science (IBS)
    Seoul National University)

  • Young Jin Yoo

    (Gwangju Institute of Science and Technology)

  • Jinhong Park

    (Institute for Basic Science (IBS)
    Seoul National University)

  • Joo Hwan Ko

    (Gwangju Institute of Science and Technology)

  • Yeong Jae Kim

    (Gwangju Institute of Science and Technology)

  • Huiwon Yun

    (Institute for Basic Science (IBS)
    Seoul National University)

  • Dong Hoe Kim

    (Korea University)

  • Young Min Song

    (Gwangju Institute of Science and Technology)

  • Dae-Hyeong Kim

    (Institute for Basic Science (IBS)
    Seoul National University
    Seoul National University)

Abstract

Perovskite microcells have a great potential to be applied to diverse types of optoelectronic devices including light-emitting diodes, photodetectors, and solar cells. Although several perovskite fabrication methods have been researched, perovskite microcells without a significant efficiency drop during the patterning and fabrication process could not be developed yet. We herein report the fabrication of high-efficiency perovskite microcells using swelling-induced crack propagation and the application of the microcells to colored solar windows. The key procedure is a swelling-induced lift-off process that leads to patterned perovskite films with high-quality interfaces. Thus, a power conversion efficiency (PCE) of 20.1 % could be achieved with the perovskite microcell, which is nearly same as the PCE of our unpatterned perovskite photovoltaic device (PV). The semi-transparent PV based on microcells exhibited a light utilization efficiency of 4.67 and a color rendering index of 97.5 %. The metal–insulator–metal structure deposited on the semi-transparent PV enabled to fabricate solar windows with vivid colors and high color purity.

Suggested Citation

  • Woongchan Lee & Young Jin Yoo & Jinhong Park & Joo Hwan Ko & Yeong Jae Kim & Huiwon Yun & Dong Hoe Kim & Young Min Song & Dae-Hyeong Kim, 2022. "Perovskite microcells fabricated using swelling-induced crack propagation for colored solar windows," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-29602-z
    DOI: 10.1038/s41467-022-29602-z
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    References listed on IDEAS

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    1. Christopher J. Traverse & Richa Pandey & Miles C. Barr & Richard R. Lunt, 2017. "Emergence of highly transparent photovoltaics for distributed applications," Nature Energy, Nature, vol. 2(11), pages 849-860, November.
    2. Byung-wook Park & Nir Kedem & Michael Kulbak & Do Yoon Lee & Woon Seok Yang & Nam Joong Jeon & Jangwon Seo & Geonhwa Kim & Ki Jeong Kim & Tae Joo Shin & Gary Hodes & David Cahen & Sang Il Seok, 2018. "Understanding how excess lead iodide precursor improves halide perovskite solar cell performance," Nature Communications, Nature, vol. 9(1), pages 1-8, December.
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