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Hybrid exciton-plasmon-polaritons in van der Waals semiconductor gratings

Author

Listed:
  • Huiqin Zhang

    (University of Pennsylvania)

  • Bhaskar Abhiraman

    (University of Pennsylvania
    University of Pennsylvania)

  • Qing Zhang

    (National University of Singapore)

  • Jinshui Miao

    (University of Pennsylvania)

  • Kiyoung Jo

    (University of Pennsylvania)

  • Stefano Roccasecca

    (University of Pennsylvania)

  • Mark W. Knight

    (NG Next, Northrop Grumman Corporation)

  • Artur R. Davoyan

    (University of California)

  • Deep Jariwala

    (University of Pennsylvania)

Abstract

Van der Waals materials and heterostructures that manifest strongly bound exciton states at room temperature also exhibit emergent physical phenomena and are of great promise for optoelectronic applications. Here, we demonstrate that nanostructured, multilayer transition metal dichalcogenides (TMDCs) by themselves provide an ideal platform for excitation and control of excitonic modes, paving the way to exciton-photonics. Hence, we show that by patterning the TMDCs into nanoresonators, strong dispersion and avoided crossing of exciton, cavity photons and plasmon polaritons with effective separation energy exceeding 410 meV can be controlled with great precision. We further observe that inherently strong TMDC exciton absorption resonances may be completely suppressed due to excitation of hybrid light-matter states and their interference. Our work paves the way to the next generation of integrated exciton optoelectronic nano-devices and applications in light generation, computing, and sensing.

Suggested Citation

  • Huiqin Zhang & Bhaskar Abhiraman & Qing Zhang & Jinshui Miao & Kiyoung Jo & Stefano Roccasecca & Mark W. Knight & Artur R. Davoyan & Deep Jariwala, 2020. "Hybrid exciton-plasmon-polaritons in van der Waals semiconductor gratings," Nature Communications, Nature, vol. 11(1), pages 1-9, December.
    • Handle: RePEc:nat:natcom:v:11:y:2020:i:1:d:10.1038_s41467-020-17313-2
    DOI: 10.1038/s41467-020-17313-2
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    References listed on IDEAS

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    1. Koray Aydin & Vivian E. Ferry & Ryan M. Briggs & Harry A. Atwater, 2011. "Broadband polarization-independent resonant light absorption using ultrathin plasmonic super absorbers," Nature Communications, Nature, vol. 2(1), pages 1-7, September.
    2. Yuanmu Yang & Ivan I. Kravchenko & Dayrl P. Briggs & Jason Valentine, 2014. "All-dielectric metasurface analogue of electromagnetically induced transparency," Nature Communications, Nature, vol. 5(1), pages 1-7, December.
    3. Long Zhang & Rahul Gogna & Will Burg & Emanuel Tutuc & Hui Deng, 2018. "Photonic-crystal exciton-polaritons in monolayer semiconductors," Nature Communications, Nature, vol. 9(1), pages 1-8, December.
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