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CO2 hydrogenation to high-value products via heterogeneous catalysis

Author

Listed:
  • Run-Ping Ye

    (University of Wyoming
    Chinese Academy of Sciences, Fuzhou
    University of Chinese Academy of Sciences)

  • Jie Ding

    (University of Wyoming
    Nanjing University of Science and Technology)

  • Weibo Gong

    (University of Wyoming)

  • Morris D. Argyle

    (Brigham Young University)

  • Qin Zhong

    (Nanjing University of Science and Technology)

  • Yujun Wang

    (Tsinghua University)

  • Christopher K. Russell

    (University of Wyoming
    Stanford University)

  • Zhenghe Xu

    (Southern University of Science and Technology)

  • Armistead G. Russell

    (Georgia Institute of Technology, Mason Building)

  • Qiaohong Li

    (Chinese Academy of Sciences, Fuzhou)

  • Maohong Fan

    (University of Wyoming
    Georgia Institute of Technology, Mason Building
    University of Wyoming)

  • Yuan-Gen Yao

    (Chinese Academy of Sciences, Fuzhou)

Abstract

Recently, carbon dioxide capture and conversion, along with hydrogen from renewable resources, provide an alternative approach to synthesis of useful fuels and chemicals. People are increasingly interested in developing innovative carbon dioxide hydrogenation catalysts, and the pace of progress in this area is accelerating. Accordingly, this perspective presents current state of the art and outlook in synthesis of light olefins, dimethyl ether, liquid fuels, and alcohols through two leading hydrogenation mechanisms: methanol reaction and Fischer-Tropsch based carbon dioxide hydrogenation. The future research directions for developing new heterogeneous catalysts with transformational technologies, including 3D printing and artificial intelligence, are provided.

Suggested Citation

  • Run-Ping Ye & Jie Ding & Weibo Gong & Morris D. Argyle & Qin Zhong & Yujun Wang & Christopher K. Russell & Zhenghe Xu & Armistead G. Russell & Qiaohong Li & Maohong Fan & Yuan-Gen Yao, 2019. "CO2 hydrogenation to high-value products via heterogeneous catalysis," Nature Communications, Nature, vol. 10(1), pages 1-15, December.
    • Handle: RePEc:nat:natcom:v:10:y:2019:i:1:d:10.1038_s41467-019-13638-9
    DOI: 10.1038/s41467-019-13638-9
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    Cited by:

    1. Xiaodong Li & Li Li & Xingyuan Chu & Xiaohui Liu & Guangbo Chen & Quanquan Guo & Zhen Zhang & Mingchao Wang & Shuming Wang & Alexander Tahn & Yongfu Sun & Xinliang Feng, 2024. "Photothermal CO2 conversion to ethanol through photothermal heterojunction-nanosheet arrays," Nature Communications, Nature, vol. 15(1), pages 1-12, December.
    2. Zhongling Li & Wenlong Wu & Menglin Wang & Yanan Wang & Xinlong Ma & Lei Luo & Yue Chen & Kaiyuan Fan & Yang Pan & Hongliang Li & Jie Zeng, 2022. "Ambient-pressure hydrogenation of CO2 into long-chain olefins," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    3. Jiaming Liang & Jiangtao Liu & Lisheng Guo & Wenhang Wang & Chengwei Wang & Weizhe Gao & Xiaoyu Guo & Yingluo He & Guohui Yang & Shuhei Yasuda & Bing Liang & Noritatsu Tsubaki, 2024. "CO2 hydrogenation over Fe-Co bimetallic catalysts with tunable selectivity through a graphene fencing approach," Nature Communications, Nature, vol. 15(1), pages 1-13, December.
    4. Zahra Gholami & Fatemeh Gholami & Zdeněk Tišler & Martin Tomas & Mohammadtaghi Vakili, 2021. "A Review on Production of Light Olefins via Fluid Catalytic Cracking," Energies, MDPI, vol. 14(4), pages 1-36, February.
    5. Sigmund Jensen & Mathias H. R. Mammen & Martin Hedevang & Zheshen Li & Lutz Lammich & Jeppe V. Lauritsen, 2024. "Visualizing the gas-sensitive structure of the CuZn surface in methanol synthesis catalysis," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    6. Zhao, Jinyang & Yu, Yadong & Ren, Hongtao & Makowski, Marek & Granat, Janusz & Nahorski, Zbigniew & Ma, Tieju, 2022. "How the power-to-liquid technology can contribute to reaching carbon neutrality of the China's transportation sector?," Energy, Elsevier, vol. 261(PA).
    7. Runping Ye & Lixuan Ma & Jianing Mao & Xinyao Wang & Xiaoling Hong & Alessandro Gallo & Yanfu Ma & Wenhao Luo & Baojun Wang & Riguang Zhang & Melis Seher Duyar & Zheng Jiang & Jian Liu, 2024. "A Ce-CuZn catalyst with abundant Cu/Zn-OV-Ce active sites for CO2 hydrogenation to methanol," Nature Communications, Nature, vol. 15(1), pages 1-14, December.
    8. Xinyi Sun & Xiaowei Mu & Wei Zheng & Lei Wang & Sixie Yang & Chuanchao Sheng & Hui Pan & Wei Li & Cheng-Hui Li & Ping He & Haoshen Zhou, 2023. "Binuclear Cu complex catalysis enabling Li–CO2 battery with a high discharge voltage above 3.0 V," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    9. Hermesmann, M. & Grübel, K. & Scherotzki, L. & Müller, T.E., 2021. "Promising pathways: The geographic and energetic potential of power-to-x technologies based on regeneratively obtained hydrogen," Renewable and Sustainable Energy Reviews, Elsevier, vol. 138(C).
    10. Si Woo Lee & Mauricio Lopez Luna & Nikolay Berdunov & Weiming Wan & Sebastian Kunze & Shamil Shaikhutdinov & Beatriz Roldan Cuenya, 2023. "Unraveling surface structures of gallium promoted transition metal catalysts in CO2 hydrogenation," Nature Communications, Nature, vol. 14(1), pages 1-7, December.
    11. Li, Sha & Haussener, Sophia, 2023. "Design and operational guidelines of solar-driven catalytic conversion of CO2 and H2 to fuels," Applied Energy, Elsevier, vol. 334(C).
    12. Gao, Ruxing & Zhang, Leiyu & Wang, Lei & Zhang, Chundong & Jun, Ki-Won & Kim, Seok Ki & Park, Hae-Gu & Gao, Ying & Zhu, Yuezhao & Wan, Hui & Guan, Guofeng & Zhao, Tiansheng, 2022. "Efficient production of renewable hydrocarbon fuels using waste CO2 and green H2 by integrating Fe-based Fischer-Tropsch synthesis and olefin oligomerization," Energy, Elsevier, vol. 248(C).
    13. Daniel Chuquin-Vasco & Francis Parra & Nelson Chuquin-Vasco & Juan Chuquin-Vasco & Vanesa Lo-Iacono-Ferreira, 2021. "Prediction of Methanol Production in a Carbon Dioxide Hydrogenation Plant Using Neural Networks," Energies, MDPI, vol. 14(13), pages 1-18, July.
    14. Lopes, J.V.M. & Bresciani, A.E. & Carvalho, K.M. & Kulay, L.A. & Alves, R.M.B., 2021. "Multi-criteria decision approach to select carbon dioxide and hydrogen sources as potential raw materials for the production of chemicals," Renewable and Sustainable Energy Reviews, Elsevier, vol. 151(C).
    15. Gui Liu & Pengfei Liu & Deming Meng & Taotao Zhao & Xiaofeng Qian & Qiang He & Xuefeng Guo & Jizhen Qi & Luming Peng & Nianhua Xue & Yan Zhu & Jingyuan Ma & Qiang Wang & Xi Liu & Liwei Chen & Weiping , 2023. "COx hydrogenation to methanol and other hydrocarbons under mild conditions with Mo3S4@ZSM-5," Nature Communications, Nature, vol. 14(1), pages 1-11, December.

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