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Spin-optoelectronic devices based on hybrid organic-inorganic trihalide perovskites

Author

Listed:
  • Jingying Wang

    (University of Utah)

  • Chuang Zhang

    (University of Utah)

  • Haoliang Liu

    (University of Utah)

  • Ryan McLaughlin

    (University of Utah)

  • Yaxin Zhai

    (University of Utah)

  • Shai R. Vardeny

    (University of Arizona)

  • Xiaojie Liu

    (University of Utah)

  • Stephen McGill

    (National High Magnetic Field Laboratory)

  • Dmitry Semenov

    (National High Magnetic Field Laboratory)

  • Hangwen Guo

    (Louisiana State University)

  • Ryuichi Tsuchikawa

    (University of Utah)

  • Vikram V. Deshpande

    (University of Utah)

  • Dali Sun

    (University of Utah
    North Carolina State University)

  • Z. Valy Vardeny

    (University of Utah)

Abstract

Recently the hybrid organic-inorganic trihalide perovskites have shown remarkable performance as active layers in photovoltaic and other optoelectronic devices. However, their spin characteristic properties have not been fully studied, although due to the relatively large spin-orbit coupling these materials may show great promise for spintronic applications. Here we demonstrate spin-polarized carrier injection into methylammonium lead bromide films from metallic ferromagnetic electrodes in two spintronic-based devices: a ‘spin light emitting diode’ that results in circularly polarized electroluminescence emission; and a ‘vertical spin valve’ that shows giant magnetoresistance. In addition, we also apply a magnetic field perpendicular to the injected spins orientation for measuring the ‘Hanle effect’, from which we obtain a relatively long spin lifetime for the electrically injected carriers. Our measurements initiate the field of hybrid perovskites spin-related optoelectronic applications.

Suggested Citation

  • Jingying Wang & Chuang Zhang & Haoliang Liu & Ryan McLaughlin & Yaxin Zhai & Shai R. Vardeny & Xiaojie Liu & Stephen McGill & Dmitry Semenov & Hangwen Guo & Ryuichi Tsuchikawa & Vikram V. Deshpande & , 2019. "Spin-optoelectronic devices based on hybrid organic-inorganic trihalide perovskites," Nature Communications, Nature, vol. 10(1), pages 1-6, December.
    • Handle: RePEc:nat:natcom:v:10:y:2019:i:1:d:10.1038_s41467-018-07952-x
    DOI: 10.1038/s41467-018-07952-x
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    Cited by:

    1. E. Kirstein & D. R. Yakovlev & M. M. Glazov & E. A. Zhukov & D. Kudlacik & I. V. Kalitukha & V. F. Sapega & G. S. Dimitriev & M. A. Semina & M. O. Nestoklon & E. L. Ivchenko & N. E. Kopteva & D. N. Di, 2022. "The Landé factors of electrons and holes in lead halide perovskites: universal dependence on the band gap," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    2. E. Kirstein & N. E. Kopteva & D. R. Yakovlev & E. A. Zhukov & E. V. Kolobkova & M. S. Kuznetsova & V. V. Belykh & I. A. Yugova & M. M. Glazov & M. Bayer & A. Greilich, 2023. "Mode locking of hole spin coherences in CsPb(Cl, Br)3 perovskite nanocrystals," Nature Communications, Nature, vol. 14(1), pages 1-7, December.
    3. Sean A. Bourelle & Franco V. A. Camargo & Soumen Ghosh & Timo Neumann & Tim W. J. Goor & Ravichandran Shivanna & Thomas Winkler & Giulio Cerullo & Felix Deschler, 2022. "Optical control of exciton spin dynamics in layered metal halide perovskites via polaronic state formation," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    4. Pei-Nan Ni & Pan Fu & Pei-Pei Chen & Chen Xu & Yi-Yang Xie & Patrice Genevet, 2022. "Spin-decoupling of vertical cavity surface-emitting lasers with complete phase modulation using on-chip integrated Jones matrix metasurfaces," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    5. Sunihl Ma & Young-Kwang Jung & Jihoon Ahn & Jihoon Kyhm & Jeiwan Tan & Hyungsoo Lee & Gyumin Jang & Chan Uk Lee & Aron Walsh & Jooho Moon, 2022. "Elucidating the origin of chiroptical activity in chiral 2D perovskites through nano-confined growth," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    6. Guankui Long & Giorgio Adamo & Jingyi Tian & Maciej Klein & Harish N. S. Krishnamoorthy & Elena Feltri & Hebin Wang & Cesare Soci, 2022. "Perovskite metasurfaces with large superstructural chirality," Nature Communications, Nature, vol. 13(1), pages 1-8, December.

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