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Valorizing Waste Lignocellulose-Based Furniture Boards by Phosphoric Acid and Hydrogen Peroxide (Php) Pretreatment for Bioethanol Production and High-Value Lignin Recovery

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  • Jingwen Zhao

    (Institute of Ecological and Environmental Sciences, Sichuan Agricultural University, Chengdu 611130, Sichuan, China
    Rural Environment Protection Engineering & Technology Center of Sichuan Province, Sichuan Agricultural University, Chengdu 611130, Sichuan, China)

  • Dong Tian

    (Institute of Ecological and Environmental Sciences, Sichuan Agricultural University, Chengdu 611130, Sichuan, China
    Rural Environment Protection Engineering & Technology Center of Sichuan Province, Sichuan Agricultural University, Chengdu 611130, Sichuan, China)

  • Fei Shen

    (Institute of Ecological and Environmental Sciences, Sichuan Agricultural University, Chengdu 611130, Sichuan, China
    Rural Environment Protection Engineering & Technology Center of Sichuan Province, Sichuan Agricultural University, Chengdu 611130, Sichuan, China)

  • Jinguang Hu

    (Chemical and Petroleum Engineering, Schulich School of Engineering, the University of Calgary, Calgary, AB T2N 4H9, Canada
    Department of Wood Science, the University of British Columbia, Vancouver, BC V6T 1Z4, Canada)

  • Yongmei Zeng

    (Institute of Ecological and Environmental Sciences, Sichuan Agricultural University, Chengdu 611130, Sichuan, China
    Rural Environment Protection Engineering & Technology Center of Sichuan Province, Sichuan Agricultural University, Chengdu 611130, Sichuan, China)

  • Churui Huang

    (Institute of Ecological and Environmental Sciences, Sichuan Agricultural University, Chengdu 611130, Sichuan, China
    Rural Environment Protection Engineering & Technology Center of Sichuan Province, Sichuan Agricultural University, Chengdu 611130, Sichuan, China)

Abstract

Three typical waste furniture boards (fiberboard, chipboard, and blockboard) were pretreated with phosphoric acid and hydrogen peroxide (PHP). The fractionation process of these feedstocks was attempted in order to harvest the cellulose-rich fraction for enzymatic hydrolysis and bioethanol conversion; further, lignin recovery was also considered in this process. The results indicated that 78.9–91.2% of the cellulose was recovered in the cellulose-rich fraction. The decreased crystallinity, which promoted the water retention capacity and enzyme accessibility, contributed greatly to the excellent hydrolysis performance of the cellulose-rich fraction. Therefore, rather high cellulose–glucose conversions of 83.3–98.0% were achieved by hydrolyzing the pretreated furniture boards, which allowed for harvesting 208–241 g of glucose from 1.0 kg of feedstocks. Correspondingly, 8.1–10.4 g/L of ethanol were obtained after 120 h of simultaneous saccharification and fermentation. The harvested lignin exhibited abundant carboxyl –OH groups (0.61–0.67 mmol g −1 ). In addition, approximately 15–26 g of harvested oligosaccharides were integrated during PHP pretreatment. It was shown that PHP pretreatment is feasible for these highly recalcitrant biomass board materials, which can diversify the bioproducts used in the integrated biorefinery concept.

Suggested Citation

  • Jingwen Zhao & Dong Tian & Fei Shen & Jinguang Hu & Yongmei Zeng & Churui Huang, 2019. "Valorizing Waste Lignocellulose-Based Furniture Boards by Phosphoric Acid and Hydrogen Peroxide (Php) Pretreatment for Bioethanol Production and High-Value Lignin Recovery," Sustainability, MDPI, vol. 11(21), pages 1-14, November.
    • Handle: RePEc:gam:jsusta:v:11:y:2019:i:21:p:6175-:d:283806
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    References listed on IDEAS

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    1. Sahar Safarian & Runar Unnthorsson, 2018. "An Assessment of the Sustainability of Lignocellulosic Bioethanol Production from Wastes in Iceland," Energies, MDPI, vol. 11(6), pages 1-16, June.
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    Cited by:

    1. Maria El Hage & Nicolas Louka & Sid-Ahmed Rezzoug & Thierry Maugard & Sophie Sablé & Mohamed Koubaa & Espérance Debs & Zoulikha Maache-Rezzoug, 2023. "Bioethanol Production from Woody Biomass: Recent Advances on the Effect of Pretreatments on the Bioconversion Process and Energy Yield Aspects," Energies, MDPI, vol. 16(13), pages 1-31, June.
    2. Huang, Caoxing & Jiang, Xiao & Shen, Xiaojun & Hu, Jinguang & Tang, Wei & Wu, Xinxing & Ragauskas, Arthur & Jameel, Hasan & Meng, Xianzhi & Yong, Qiang, 2022. "Lignin-enzyme interaction: A roadblock for efficient enzymatic hydrolysis of lignocellulosics," Renewable and Sustainable Energy Reviews, Elsevier, vol. 154(C).

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