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Spatial Distribution, Potential Sources, and Health Risk of Polycyclic Aromatic Hydrocarbons (PAHs) in the Surface Soils under Different Land-Use Covers of Shanxi Province, North China

Author

Listed:
  • Li Ji

    (School of Environment and Resources, Taiyuan University of Science and Technology, Taiyuan 030024, China)

  • Wenwen Li

    (School of Environment and Resources, Taiyuan University of Science and Technology, Taiyuan 030024, China)

  • Yuan Li

    (School of Environment and Resources, Taiyuan University of Science and Technology, Taiyuan 030024, China
    State Key Laboratory of Freshwater Ecology and Biotechnology, Institute of Hydrobiology, Chinese Academy of Sciences, Wuhan 430072, China)

  • Qiusheng He

    (School of Environment and Resources, Taiyuan University of Science and Technology, Taiyuan 030024, China)

  • Yonghong Bi

    (State Key Laboratory of Freshwater Ecology and Biotechnology, Institute of Hydrobiology, Chinese Academy of Sciences, Wuhan 430072, China)

  • Minghua Zhang

    (School of Environment and Resources, Taiyuan University of Science and Technology, Taiyuan 030024, China)

  • Guixiang Zhang

    (School of Environment and Resources, Taiyuan University of Science and Technology, Taiyuan 030024, China)

  • Xinming Wang

    (State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China)

Abstract

Polycyclic aromatic hydrocarbons (PAHs) are widespread in the environment and pose a serious threat to the soil ecosystem. In order to better understand the health risks for residents exposed to PAH-contaminated soil, 173 surface soil samples were collected in Shanxi Province, China, to detect the levels of 16 priority PAHs. The spatial distribution patterns of PAHs were explored using interpolation and spatial clustering analysis, and the probable sources of soil PAHs were identified for different land-use covers. The results indicate that the soil Σ16 PAH concentration ranged from 22.12 to 1337.82 ng g − 1 , with a mean of 224.21 ng g − 1 . The soils were weakly to moderately contaminated by high molecular weight PAHs (3–5 ring) and the Taiyuan–Linfen Basin was the most polluted areas. In addition, the concentration of soil PAHs on construction land was higher than that on other land-use covers. Key sources of soil PAHs were related to industrial activities dominated by coal burning, coking, and heavy traffic. Based on the exposure risk assessment of PAHs, more than 10% of the area was revealed to be likely to suffer from high carcinogenic risks for children. The study maps the high-risk distribution of soil PAHs in Shanxi Province and provides PAH pollution reduction strategies for policy makers to prevent adverse health risks to residents.

Suggested Citation

  • Li Ji & Wenwen Li & Yuan Li & Qiusheng He & Yonghong Bi & Minghua Zhang & Guixiang Zhang & Xinming Wang, 2022. "Spatial Distribution, Potential Sources, and Health Risk of Polycyclic Aromatic Hydrocarbons (PAHs) in the Surface Soils under Different Land-Use Covers of Shanxi Province, North China," IJERPH, MDPI, vol. 19(19), pages 1-14, September.
  • Handle: RePEc:gam:jijerp:v:19:y:2022:i:19:p:11949-:d:921144
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    References listed on IDEAS

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    1. Yihua Xiao & Fuchun Tong & Yuanwen Kuang & Bufeng Chen, 2014. "Distribution and Source Apportionment of Polycyclic Aromatic Hydrocarbons (PAHs) in Forest Soils from Urban to Rural Areas in the Pearl River Delta of Southern China," IJERPH, MDPI, vol. 11(3), pages 1-15, March.
    2. Wei Cao & Liqin Yin & Dan Zhang & Yingying Wang & Jing Yuan & Yi Zhu & Junfeng Dou, 2019. "Contamination, Sources, and Health Risks Associated with Soil PAHs in Rebuilt Land from a Coking Plant, Beijing, China," IJERPH, MDPI, vol. 16(4), pages 1-16, February.
    3. Rongjie Li & Mingchao Cheng & Yang Cui & Qiusheng He & Xiaofang Guo & Laiguo Chen & Xinming Wang, 2020. "Distribution of the Soil PAHs and Health Risk Influenced by Coal Usage Processes in Taiyuan City, Northern China," IJERPH, MDPI, vol. 17(17), pages 1-18, August.
    4. Haihua Jiao & Qi Wang & Nana Zhao & Bo Jin & Xuliang Zhuang & Zhihui Bai, 2017. "Distributions and Sources of Polycyclic Aromatic Hydrocarbons (PAHs) in Soils around a Chemical Plant in Shanxi, China," IJERPH, MDPI, vol. 14(10), pages 1-19, October.
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    Cited by:

    1. Ewa Mackiewicz-Walec & Sławomir Józef Krzebietke & Stanisław Sienkiewicz, 2022. "The Influence of Crops on the Content of Polycyclic Aromatic Hydrocarbons in Soil Fertilized with Manure and Mineral Fertilizers," IJERPH, MDPI, vol. 19(20), pages 1-14, October.
    2. Haolong Cai & Siyu Yao & Jiahui Huang & Xiongkai Zheng & Jianteng Sun & Xueqin Tao & Guining Lu, 2022. "Polycyclic Aromatic Hydrocarbons Pollution Characteristics in Agricultural Soils of the Pearl River Delta Region, China," IJERPH, MDPI, vol. 19(23), pages 1-13, December.

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