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An Overview on Transport Phenomena within Solid Electrolyte Interphase and Their Impact on the Performance and Durability of Lithium-Ion Batteries

Author

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  • Roberta Cappabianca

    (Department of Energy “Galileo Ferraris”, Politecnico di Torino, Corso Duca Degli Abruzzi 24, 10129 Torino, Italy)

  • Paolo De Angelis

    (Department of Energy “Galileo Ferraris”, Politecnico di Torino, Corso Duca Degli Abruzzi 24, 10129 Torino, Italy)

  • Matteo Fasano

    (Department of Energy “Galileo Ferraris”, Politecnico di Torino, Corso Duca Degli Abruzzi 24, 10129 Torino, Italy)

  • Eliodoro Chiavazzo

    (Department of Energy “Galileo Ferraris”, Politecnico di Torino, Corso Duca Degli Abruzzi 24, 10129 Torino, Italy)

  • Pietro Asinari

    (Department of Energy “Galileo Ferraris”, Politecnico di Torino, Corso Duca Degli Abruzzi 24, 10129 Torino, Italy
    Istituto Nazionale di Ricerca Metrologica, Strada Delle Cacce 91, 10135 Torino, Italy)

Abstract

The nature of the electrode–electrolyte interface has an impact on the performance and durability of lithium-ion batteries (LIBs). The initial electrolyte’s thermodynamic instability at the anode–electrolyte interface in LIBs results in the formation of a passivation layer, called solid electrolyte interphase (SEI). The initial dense and intact layer allows Li + transport and restricts electron tunneling, thus preventing electrolyte decomposition and ensuring the electrochemical stability of a battery. However, the growth of this layer can reduce the availability of active lithium and electrolyte, and ultimately lead to an irreversible battery capacity fade. Investigating the transport phenomena of lithium ions within SEI is crucial for understanding its formation and growth. Nonetheless, accurately describing all relevant mechanisms is challenging due to its complex and multiscale nature. An overview of current computational efforts to study Li + transport within SEI is given in this article, ranging from electronic/atomistic scale simulations to macroscopic models. The drawbacks and advantages of the proposed numerical approaches are summarized along with the obstacles that need to be overcome to obtain accurate experimental data, identified on the basis of the most recent literature evidence. We highlight collaboration gaps between modeling and experimental approaches, as well as the urgent need for new multiscale models, to gain a better understanding of such a crucial transport phenomenon.

Suggested Citation

  • Roberta Cappabianca & Paolo De Angelis & Matteo Fasano & Eliodoro Chiavazzo & Pietro Asinari, 2023. "An Overview on Transport Phenomena within Solid Electrolyte Interphase and Their Impact on the Performance and Durability of Lithium-Ion Batteries," Energies, MDPI, vol. 16(13), pages 1-30, June.
  • Handle: RePEc:gam:jeners:v:16:y:2023:i:13:p:5003-:d:1181491
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    References listed on IDEAS

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    1. J.-M. Tarascon & M. Armand, 2001. "Issues and challenges facing rechargeable lithium batteries," Nature, Nature, vol. 414(6861), pages 359-367, November.
    2. Pastor-Fernández, Carlos & Yu, Tung Fai & Widanage, W. Dhammika & Marco, James, 2019. "Critical review of non-invasive diagnosis techniques for quantification of degradation modes in lithium-ion batteries," Renewable and Sustainable Energy Reviews, Elsevier, vol. 109(C), pages 138-159.
    3. Alice J. Merryweather & Christoph Schnedermann & Quentin Jacquet & Clare P. Grey & Akshay Rao, 2021. "Operando optical tracking of single-particle ion dynamics in batteries," Nature, Nature, vol. 594(7864), pages 522-528, June.
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