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Protective Coatings for Ferritic Stainless Steel Interconnect Materials in High Temperature Solid Oxide Electrolyser Atmospheres

Author

Listed:
  • Jyrki Mikkola

    (Fuel Cells and Hydrogen Team, VTT Technical Research Centre of Finland Ltd., P.O. Box 1000, 02044 Espoo, Finland)

  • Karine Couturier

    (CEA (Atomic Energy and Alternative Energies Commission)-LITEN (Innovative Laboratory for New Energies Technologies and Nanomaterials), Université Grenoble Alpes, 38054 Grenoble, France)

  • Belma Talic

    (Department of Energy Conversion and Storage, Technical University of Denmark, Anker Engelunds Vej 301, 2800 Kongens Lyngby, Denmark
    Current address: SINTEF Industry, Sustainable Energy Technology, P.O. Box 124, Blindern, 0314 Oslo, Norway.)

  • Stefano Frangini

    (ENEA (Energia Nucleare ed Energie Alternative), CR (Casaccia Centro Ricerche), TERIN-PSU-ABI, 00123 Rome, Italy)

  • Nathalie Giacometti

    (CEA (Atomic Energy and Alternative Energies Commission)-LITEN (Innovative Laboratory for New Energies Technologies and Nanomaterials), Université Grenoble Alpes, 38054 Grenoble, France)

  • Nathalie Pelissier

    (CEA (Atomic Energy and Alternative Energies Commission)-LITEN (Innovative Laboratory for New Energies Technologies and Nanomaterials), Université Grenoble Alpes, 38054 Grenoble, France)

  • Bhaskar Reddy Sudireddy

    (Department of Energy Conversion and Storage, Technical University of Denmark, Anker Engelunds Vej 301, 2800 Kongens Lyngby, Denmark)

  • Olivier Thomann

    (Fuel Cells and Hydrogen Team, VTT Technical Research Centre of Finland Ltd., P.O. Box 1000, 02044 Espoo, Finland
    Current address: Neste Oyj, Innovation, Discovery and External Collaboration, P.O. Box 310, 06101 Porvoo, Finland.)

Abstract

Stainless steel interconnect materials used in solid oxide fuel cells and electrolysers need to be coated to improve oxidation resistance and to mitigate Cr-vaporization. This work aimed to explore the optimal steel/coating combinations suitable for use in reversible solid oxide stacks and evaluated (Co,Mn) 3 O 4 spinel, LaFeO 3 perovskite, Ce/Co and Y-based coatings, on AISI441 and Crofer 22 APU steels. The coatings were evaluated based on measurements of mass gain and oxide scale thickness after exposure at 700 and 800 °C to fuel side (90 vol.% H 2 O/10 vol.% H 2 ) and air/oxygen side (pure O 2 ) atmospheres. In pure O 2 , the most efficient coatings for limiting oxide scale formation and Cr evaporation, compared to the bare steel, were (Co,Mn) 3 O 4 and CeCo on Crofer 22 APU. In 90 vol.% H 2 O/10 vol.% H 2 , the Y-based coating showed the largest improvement in oxidation resistance.

Suggested Citation

  • Jyrki Mikkola & Karine Couturier & Belma Talic & Stefano Frangini & Nathalie Giacometti & Nathalie Pelissier & Bhaskar Reddy Sudireddy & Olivier Thomann, 2022. "Protective Coatings for Ferritic Stainless Steel Interconnect Materials in High Temperature Solid Oxide Electrolyser Atmospheres," Energies, MDPI, vol. 15(3), pages 1-24, February.
    • Handle: RePEc:gam:jeners:v:15:y:2022:i:3:p:1168-:d:742791
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    References listed on IDEAS

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    1. Buttler, Alexander & Spliethoff, Hartmut, 2018. "Current status of water electrolysis for energy storage, grid balancing and sector coupling via power-to-gas and power-to-liquids: A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 82(P3), pages 2440-2454.
    2. Lund, Peter D. & Lindgren, Juuso & Mikkola, Jani & Salpakari, Jyri, 2015. "Review of energy system flexibility measures to enable high levels of variable renewable electricity," Renewable and Sustainable Energy Reviews, Elsevier, vol. 45(C), pages 785-807.
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    Cited by:

    1. Athanasios Zarkadoulas & Vassilis N. Stathopoulos, 2022. "Perovskites: Versatile Weaponry in the Arsenal of Energy Storage and Conversion," Energies, MDPI, vol. 15(18), pages 1-3, September.
    2. Mao, Jingwen & Wang, Enhua & Wang, Hewu & Ouyang, Minggao & Chen, Youpeng & Hu, Haoran & Lu, Languang & Ren, Dongsheng & Liu, Yadi, 2023. "Progress in metal corrosion mechanism and protective coating technology for interconnect and metal support of solid oxide cells," Renewable and Sustainable Energy Reviews, Elsevier, vol. 185(C).

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