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Parameter Identification of Electrical Equivalent Circuits including Mass Transfer Parameters for the Selection of the Operating Frequencies of Pulsed PEM Water Electrolysis

Author

Listed:
  • Jae-Hoon Kim

    (Power Conversion System Research Center, Korea Electrotechnology Research Institute (KERI), Gwangju-si 61751, Republic of Korea)

  • Chang-Yeol Oh

    (Power Conversion System Research Center, Korea Electrotechnology Research Institute (KERI), Gwangju-si 61751, Republic of Korea)

  • Ki-Ryong Kim

    (Power Conversion System Research Center, Korea Electrotechnology Research Institute (KERI), Gwangju-si 61751, Republic of Korea)

  • Jong-Pil Lee

    (Power Conversion System Research Center, Korea Electrotechnology Research Institute (KERI), Gwangju-si 61751, Republic of Korea)

  • Tae-Jin Kim

    (Power Conversion System Research Center, Korea Electrotechnology Research Institute (KERI), Gwangju-si 61751, Republic of Korea)

Abstract

This paper proposes a parameter identification method for a PEM electrolyzer electrical equivalent circuit for pulse electrolysis. Since general water electrolysis mainly uses DC currents, identifying equivalent circuit parameters using electrical characteristics mostly ignores the operation frequency and unnecessarily adheres to the secondary RC model. However, looking at the Nyquist plot of the PEM electrolyzer, it can be confirmed that identifying the operational frequency is necessary, and the secondary RC model correction is essential. Therefore, the proposed method confirms the necessity of reconstructing an electrical equivalent circuit with a primary RC model by analyzing the transient cell voltage using step current inputs and calculating an appropriate operating frequency by identifying the parameters of the reconstructed equivalent circuit. To verify the proposed parameter identification method, a simulation was constructed from the raw test data of a 400 W commercial PEM electrolyzer. In addition, the hydrogen production amount was compared to DC using a pulse electrolysis experiment at the operating frequency obtained by the proposed method.

Suggested Citation

  • Jae-Hoon Kim & Chang-Yeol Oh & Ki-Ryong Kim & Jong-Pil Lee & Tae-Jin Kim, 2022. "Parameter Identification of Electrical Equivalent Circuits including Mass Transfer Parameters for the Selection of the Operating Frequencies of Pulsed PEM Water Electrolysis," Energies, MDPI, vol. 15(24), pages 1-16, December.
    • Handle: RePEc:gam:jeners:v:15:y:2022:i:24:p:9303-:d:997433
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    References listed on IDEAS

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    1. Damien Guilbert & Gianpaolo Vitale, 2019. "Dynamic Emulation of a PEM Electrolyzer by Time Constant Based Exponential Model," Energies, MDPI, vol. 12(4), pages 1-17, February.
    2. Espinosa-López, Manuel & Darras, Christophe & Poggi, Philippe & Glises, Raynal & Baucour, Philippe & Rakotondrainibe, André & Besse, Serge & Serre-Combe, Pierre, 2018. "Modelling and experimental validation of a 46 kW PEM high pressure water electrolyzer," Renewable Energy, Elsevier, vol. 119(C), pages 160-173.
    3. Frank Gambou & Damien Guilbert & Michel Zasadzinski & Hugues Rafaralahy, 2022. "A Comprehensive Survey of Alkaline Electrolyzer Modeling: Electrical Domain and Specific Electrolyte Conductivity," Energies, MDPI, vol. 15(9), pages 1-20, May.
    4. Jae-Hoon Kim & Chang-Yeol Oh & Ki-Ryong Kim & Jong-Pil Lee & Tae-Jin Kim, 2021. "Electrical Double Layer Mechanism Analysis of PEM Water Electrolysis for Frequency Limitation of Pulsed Currents," Energies, MDPI, vol. 14(22), pages 1-17, November.
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