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Modeling the Effect of the Loss of Cyclable Lithium on the Performance Degradation of a Lithium-Ion Battery

Author

Listed:
  • Dongcheul Lee

    (Department of Chemical Engineering and Division of Energy Systems Research, Ajou University, Suwon 16499, Korea)

  • Boram Koo

    (Department of Chemical Engineering and Division of Energy Systems Research, Ajou University, Suwon 16499, Korea)

  • Chee Burm Shin

    (Department of Chemical Engineering and Division of Energy Systems Research, Ajou University, Suwon 16499, Korea)

  • So-Yeon Lee

    (Gwangju Bioenergy R & D Center, Korea Institute of Energy Research, Gwangju 61003, Korea)

  • Jinju Song

    (Gwangju Bioenergy R & D Center, Korea Institute of Energy Research, Gwangju 61003, Korea)

  • Il-Chan Jang

    (Gwangju Bioenergy R & D Center, Korea Institute of Energy Research, Gwangju 61003, Korea)

  • Jung-Je Woo

    (Gwangju Bioenergy R & D Center, Korea Institute of Energy Research, Gwangju 61003, Korea)

Abstract

This paper reports a modeling methodology to predict the effect of the loss of cyclable lithium of a lithium-ion battery (LIB) cell comprised of a LiNi 0.6 Co 0.2 Mn 0.2 O 2 cathode, natural graphite anode, and an organic electrolyte on the discharge behavior. A one-dimensional model based on a finite element method is presented to calculate the discharge behaviors of an LIB cell during galvanostatic discharge for various levels of the loss of cyclable lithium. Modeling results for the variation of the cell voltage of the LIB cell are compared with experimental measurements during galvanostatic discharge at various discharge rates for three different levels of the loss of cyclable lithium to validate the model. The calculation results obtained from the model are in good agreement with the experimental measurements. On the basis of the validated modeling approach, the effects of the loss of cyclable lithium on the discharge capacity and available discharge power of the LIB cell are estimated. The modeling results exhibit strong dependencies of the discharge behavior of an LIB cell on the discharge C-rate and the loss of cyclable lithium.

Suggested Citation

  • Dongcheul Lee & Boram Koo & Chee Burm Shin & So-Yeon Lee & Jinju Song & Il-Chan Jang & Jung-Je Woo, 2019. "Modeling the Effect of the Loss of Cyclable Lithium on the Performance Degradation of a Lithium-Ion Battery," Energies, MDPI, vol. 12(22), pages 1-14, November.
    • Handle: RePEc:gam:jeners:v:12:y:2019:i:22:p:4386-:d:288332
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    References listed on IDEAS

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    Cited by:

    1. Davide Clerici & Francesco Mocera & Aurelio Somà, 2020. "Analytical Solution for Coupled Diffusion Induced Stress Model for Lithium-Ion Battery," Energies, MDPI, vol. 13(7), pages 1-20, April.
    2. Dongcheul Lee & Byungmook Kim & Chee Burm Shin & Seung-Mi Oh & Jinju Song & Il-Chan Jang & Jung-Je Woo, 2022. "Modeling the Combined Effects of Cyclable Lithium Loss and Electrolyte Depletion on the Capacity and Power Fades of a Lithium-Ion Battery," Energies, MDPI, vol. 15(19), pages 1-13, September.

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