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Hydrogen rich gas production from catalytic gasification of biomass

Author

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  • Hamad, Mohamed A.
  • Radwan, Aly M.
  • Heggo, Dalia A.
  • Moustafa, Tarek

Abstract

Production of hydrogen rich gas from gasification of biomass was studied at bench-scale using oxygen as the gasifying agent. A series of experiments were performed to investigate the effects of different operating parameters on the performance of the gasification process. These included the oxygen to fuel equivalence ratio (0.12–0.4), reaction temperature (700–850 °C), reaction residence time (45–120 min), and catalyst type. The catalysts selected are marly clay, calcium hydroxide, dolomite, and cement kiln dust. Within the range of the experimental conditions tested, the results suggest that the best operating conditions for the gasification process are; temperature, 800 °C, an oxygen to fuel ratio of 0.25, a reaction time of 90 min, and calcined cement kiln dust as a catalyst. The results have also demonstrated that the product gas from gasification of cotton stalks with calcium hydroxide has higher H2 and CO concentration (45 and 33%). In addition gasification of cotton stalks with calcined cement kiln dust resulted in higher hydrogen and CO enrichment as well as higher overall gas yield (39vol%, 33vol%, and 1.5 m3/kg) compared to other agriculture residues of corn stalks and rice straw.

Suggested Citation

  • Hamad, Mohamed A. & Radwan, Aly M. & Heggo, Dalia A. & Moustafa, Tarek, 2016. "Hydrogen rich gas production from catalytic gasification of biomass," Renewable Energy, Elsevier, vol. 85(C), pages 1290-1300.
    • Handle: RePEc:eee:renene:v:85:y:2016:i:c:p:1290-1300
    DOI: 10.1016/j.renene.2015.07.082
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    Cited by:

    1. Yuan, Hongyou & Wu, Shubin & Yin, Xiuli & Huang, Yanqin & Guo, Daliang & Wu, Chuangzhi, 2018. "Adjustment of biomass product gas to raise H2/CO ratio and remove tar over sodium titanate catalysts," Renewable Energy, Elsevier, vol. 115(C), pages 288-298.
    2. Nakamura, Shunsuke & Kitano, Shigeru & Yoshikawa, Kunio, 2016. "Biomass gasification process with the tar removal technologies utilizing bio-oil scrubber and char bed," Applied Energy, Elsevier, vol. 170(C), pages 186-192.
    3. Antonio Molino & Vincenzo Larocca & Simeone Chianese & Dino Musmarra, 2018. "Biofuels Production by Biomass Gasification: A Review," Energies, MDPI, vol. 11(4), pages 1-31, March.
    4. Pio, D.T. & Gomes, H.G.M.F. & Ruivo, L.C.M. & Matos, M.A.A. & Monteiro, J.F. & Frade, J.R. & Tarelho, L.A.C., 2021. "Concrete as low-cost catalyst to improve gas quality during biomass gasification in a pilot-scale gasifier," Energy, Elsevier, vol. 233(C).
    5. Shivangi Jha & Sonil Nanda & Bishnu Acharya & Ajay K. Dalai, 2022. "A Review of Thermochemical Conversion of Waste Biomass to Biofuels," Energies, MDPI, vol. 15(17), pages 1-23, August.
    6. Sooraj Kumar & Suhail Ahmed Soomro & Khanji Harijan & Mohammad Aslam Uqaili & Laveet Kumar, 2023. "Advancements of Biochar-Based Catalyst for Improved Production of Biodiesel: A Comprehensive Review," Energies, MDPI, vol. 16(2), pages 1-20, January.
    7. Couto, Nuno Dinis & Silva, Valter Bruno & Monteiro, Eliseu & Rouboa, Abel & Brito, Paulo, 2017. "An experimental and numerical study on the Miscanthus gasification by using a pilot scale gasifier," Renewable Energy, Elsevier, vol. 109(C), pages 248-261.
    8. Watson, Jamison & Zhang, Yuanhui & Si, Buchun & Chen, Wan-Ting & de Souza, Raquel, 2018. "Gasification of biowaste: A critical review and outlooks," Renewable and Sustainable Energy Reviews, Elsevier, vol. 83(C), pages 1-17.
    9. Król, Danuta & Poskrobko, Sławomir, 2016. "High-methane gasification of fuels from waste – Experimental identification," Energy, Elsevier, vol. 116(P1), pages 592-600.
    10. Elena David, 2020. "Evaluation of Hydrogen Yield Evolution in Gaseous Fraction and Biochar Structure Resulting from Walnut Shells Pyrolysis," Energies, MDPI, vol. 13(23), pages 1-17, December.
    11. Al-Rahbi, Amal S. & Williams, Paul T., 2017. "Hydrogen-rich syngas production and tar removal from biomass gasification using sacrificial tyre pyrolysis char," Applied Energy, Elsevier, vol. 190(C), pages 501-509.
    12. Ricardo A. Narváez C. & Richard Blanchard & Roger Dixon & Valeria Ramírez & Diego Chulde, 2018. "Low-Cost Syngas Shifting for Remote Gasifiers: Combination of CO 2 Adsorption and Catalyst Addition in a Novel and Simplified Packed Structure," Energies, MDPI, vol. 11(2), pages 1-16, February.
    13. Ghulamullah Maitlo & Imran Ali & Kashif Hussain Mangi & Safdar Ali & Hubdar Ali Maitlo & Imran Nazir Unar & Abdul Majeed Pirzada, 2022. "Thermochemical Conversion of Biomass for Syngas Production: Current Status and Future Trends," Sustainability, MDPI, vol. 14(5), pages 1-30, February.
    14. Yan, Linbo & Wang, Ziqi & Cao, Yang & He, Boshu, 2020. "Comparative evaluation of two biomass direct-fired power plants with carbon capture and sequestration," Renewable Energy, Elsevier, vol. 147(P1), pages 1188-1198.
    15. Huang, Xiaoyuan & Cheng, Dang-guo & Chen, Fengqiu & Zhan, Xiaoli, 2016. "Reaction pathways of hemicellulose and mechanism of biomass pyrolysis in hydrogen plasma: A density functional theory study," Renewable Energy, Elsevier, vol. 96(PA), pages 490-497.
    16. Hrnčič, Maša Knez & Kravanja, Gregor & Knez, Željko, 2016. "Hydrothermal treatment of biomass for energy and chemicals," Energy, Elsevier, vol. 116(P2), pages 1312-1322.
    17. Ahsanullah Soomro & Shiyi Chen & Shiwei Ma & Wenguo Xiang, 2018. "Catalytic activities of nickel, dolomite, and olivine for tar removal and H2-enriched gas production in biomass gasification process," Energy & Environment, , vol. 29(6), pages 839-867, September.
    18. Wądrzyk, Mariusz & Grzywacz, Przemysław & Janus, Rafał & Michalik, Marek, 2021. "A two-stage processing of cherry pomace via hydrothermal treatment followed by biochar gasification," Renewable Energy, Elsevier, vol. 179(C), pages 248-261.
    19. Shahbaz, Muhammad & Al-Ansari, Tareq & Inayat, Muddasser & Sulaiman, Shaharin A. & Parthasarathy, Prakash & McKay, Gordon, 2020. "A critical review on the influence of process parameters in catalytic co-gasification: Current performance and challenges for a future prospectus," Renewable and Sustainable Energy Reviews, Elsevier, vol. 134(C).

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