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Chitosan-assisted reassembled hierarchical HZSM-5 for selective production of monocyclic aromatics in catalytic co-pyrolysis of biomass and plastic

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  • Fu, Peng
  • Tang, Binbin
  • Li, Hongtao
  • Liu, Shanjian
  • Wang, Lihong
  • Lin, Xiaona

Abstract

Biomass presents significant potential as an alternative template agent for assisting zeolites in developing new pore structure during recrystallization to enhance their catalytic performance. In this study, a new hierarchical HZSM-5 was synthesized through the in-situ reassembly of alkali-treated HZSM-5 with chitosan as an assisting agent. The impact of chitosan dosage on the catalytic performance of the hierarchical HZSM-5, as well as the influences of temperature, catalyst dosage, and corn stover (CS) to high-density polyethylene (HDPE) mass ratio on the content and selectivity of monocyclic aromatic hydrocarbons (MAHs) during the catalytic co-pyrolysis process, were thoroughly investigated. The results indicated that chitosan exhibited great potential as a template in the reassembly of hierarchical HZSM-5 during NaOH treatment, promoting the formation of weak acid sites and micro-mesoporous structures. Compared to the parent HZSM-5, the chitosan-assistant reassembled hierarchical HZSM-5 significantly enhanced the production of MAHs and inhibited the formation of polycyclic aromatic hydrocarbons (PAHs). The highest carbon yield of MAHs reached 36.9 % at 550 °C with a chitosan dosage of 15 %. Furthermore, the chitosan-modified HZSM-5 notably enhanced the synergistic production of MAHs by 38.2 %, while preventing the formation of PAHs and coke. This study contributes insights into the sustainable synthesis of hierarchical HZSM-5 for improved production of high-value products in the co-pyrolysis of biomass and waste plastics.

Suggested Citation

  • Fu, Peng & Tang, Binbin & Li, Hongtao & Liu, Shanjian & Wang, Lihong & Lin, Xiaona, 2024. "Chitosan-assisted reassembled hierarchical HZSM-5 for selective production of monocyclic aromatics in catalytic co-pyrolysis of biomass and plastic," Renewable Energy, Elsevier, vol. 236(C).
    • Handle: RePEc:eee:renene:v:236:y:2024:i:c:s096014812401560x
    DOI: 10.1016/j.renene.2024.121492
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    References listed on IDEAS

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    1. Li, Xiaohua & Sun, Jiayuan & Shao, Shanshan & Yan, Jinlong & Cai, Yixi, 2023. "Preparation of composite HZSM-5 catalyst by green template and catalytic the pyrolysis of biomass to produce aromatics," Renewable Energy, Elsevier, vol. 206(C), pages 506-513.
    2. Zhang, Yayun & Duan, Dengle & Lei, Hanwu & Villota, Elmar & Ruan, Roger, 2019. "Jet fuel production from waste plastics via catalytic pyrolysis with activated carbons," Applied Energy, Elsevier, vol. 251(C), pages 1-1.
    3. Lin, Xiaona & Kong, Lingshuai & Ren, Xiajin & Zhang, Donghong & Cai, Hongzhen & Lei, Hanwu, 2021. "Catalytic co-pyrolysis of torrefied poplar wood and high-density polyethylene over hierarchical HZSM-5 for mono-aromatics production," Renewable Energy, Elsevier, vol. 164(C), pages 87-95.
    4. Lopez, Gartzen & Artetxe, Maite & Amutio, Maider & Bilbao, Javier & Olazar, Martin, 2017. "Thermochemical routes for the valorization of waste polyolefinic plastics to produce fuels and chemicals. A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 73(C), pages 346-368.
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