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Hydrogen concentration and purification by membrane process: A multistage analysis

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  • Zito, Pasquale Francesco
  • Brunetti, Adele
  • Barbieri, Giuseppe

Abstract

In this work, the concentration and purification of hydrogen from multicomponent gas mixtures, such as syngas and H2:CH4 blends, were investigated by simulations of multi-stage membrane configurations. In particular, the separation performance of carbon, polymeric and Pd-alloy membranes were analyzed for obtaining a final H2 stream completely pure with a recovery higher than 90%. Carbon and polymer membranes in multistage configuration confirmed their suitability to be used as concentration units able to increase the hydrogen content in the gas mixture. A further purification of these pre-concentrated streams was carried out adding Pd-alloy membranes that were able to recover more than 90% of hydrogen fully pure. The use of an integrated process constituted of a concentration stage based on polymer/carbon membranes followed by a purification stage based on a Pd-alloy membrane allowed to drastically reduce the operating pressure and, moreover, save Pd-alloy membrane area.

Suggested Citation

  • Zito, Pasquale Francesco & Brunetti, Adele & Barbieri, Giuseppe, 2023. "Hydrogen concentration and purification by membrane process: A multistage analysis," Renewable Energy, Elsevier, vol. 218(C).
    • Handle: RePEc:eee:renene:v:218:y:2023:i:c:s0960148123011588
    DOI: 10.1016/j.renene.2023.119243
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    References listed on IDEAS

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    1. Tanksale, Akshat & Beltramini, Jorge Norberto & Lu, GaoQing Max, 2010. "A review of catalytic hydrogen production processes from biomass," Renewable and Sustainable Energy Reviews, Elsevier, vol. 14(1), pages 166-182, January.
    2. Francesco Zito, Pasquale & Brunetti, Adele & Barbieri, Giuseppe, 2022. "Renewable biomethane production from biogas upgrading via membrane separation: Experimental analysis and multistep configuration design," Renewable Energy, Elsevier, vol. 200(C), pages 777-787.
    3. Chen, Wei-Hsin & Chen, Chia-Yang, 2020. "Water gas shift reaction for hydrogen production and carbon dioxide capture: A review," Applied Energy, Elsevier, vol. 258(C).
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    1. Anna Król & Monika Gajec & Jadwiga Holewa-Rataj & Ewa Kukulska-Zając & Mateusz Rataj, 2024. "Hydrogen Purification Technologies in the Context of Its Utilization," Energies, MDPI, vol. 17(15), pages 1-38, August.

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