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SiC-based structured catalysts for a high-efficiency electrified dry reforming of methane

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  • Meloni, Eugenio
  • Saraceno, Emilia
  • Martino, Marco
  • Corrado, Antonio
  • Iervolino, Giuseppina
  • Palma, Vincenzo

Abstract

The process of dry reforming of methane (DRM) can allow the conversion of methane and carbon dioxide, the two main greenhouse gases (GHG), into syngas which can be either used as feedstock for chemicals production or it can undergo through separation step for H2 recovery. However, the heat required for the reaction is obtained by combustion of fossil fuels, so CO2 footprint of the process is significant. Another problematic aspect of the process concerns the heat transfer to the catalytic volume: for allowing the catalytic bed to reach and maintain the reaction temperature, the heating medium outside the tubes containing the catalyst must have a temperature higher than 1000 °C. A process intensification could be performed by combining two innovative technologies: (i) the use of electrification for the energy supply (microwave heating and direct electrification) and (ii) the adoption of structured catalysts with high thermal conductivity.

Suggested Citation

  • Meloni, Eugenio & Saraceno, Emilia & Martino, Marco & Corrado, Antonio & Iervolino, Giuseppina & Palma, Vincenzo, 2023. "SiC-based structured catalysts for a high-efficiency electrified dry reforming of methane," Renewable Energy, Elsevier, vol. 211(C), pages 336-346.
    • Handle: RePEc:eee:renene:v:211:y:2023:i:c:p:336-346
    DOI: 10.1016/j.renene.2023.04.082
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    References listed on IDEAS

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    1. Jung, Sungyup & Lee, Jechan & Moon, Deok Hyun & Kim, Ki-Hyun & Kwon, Eilhann E., 2021. "Upgrading biogas into syngas through dry reforming," Renewable and Sustainable Energy Reviews, Elsevier, vol. 143(C).
    2. Meloni, Eugenio & Martino, Marco & Palma, Vincenzo, 2022. "Microwave assisted steam reforming in a high efficiency catalytic reactor," Renewable Energy, Elsevier, vol. 197(C), pages 893-901.
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    1. Hanmin Yang & Ilman Nuran Zaini & Ruming Pan & Yanghao Jin & Yazhe Wang & Lengwan Li & José Juan Bolívar Caballero & Ziyi Shi & Yaprak Subasi & Anissa Nurdiawati & Shule Wang & Yazhou Shen & Tianxiang, 2024. "Distributed electrified heating for efficient hydrogen production," Nature Communications, Nature, vol. 15(1), pages 1-10, December.

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