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Catalytic co-pyrolysis of wet-torrefied bamboo sawdust and plastic over the zeolite H-ZSM-5: Synergistic effects and kinetics

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  • Alam, Mahboob
  • Rammohan, Draksharapu
  • Peela, Nageswara Rao

Abstract

In the present study, the hemicellulose from bamboo sawdust (BSD) was selectively removed in the form of xylose and acetic acid using the wet-torrefaction technique in presence of formic acid and NaCl as catalysts. The best torrefaction activity, with xylose yield 85% and complete removal of hemicellulose, was obtained with formic acid:BSD 1:1 and NaCl:BSD 3:1 w/w. The torrefied BSD (TBSD) was catalytically co-pyrolyzed with linear low-density polyethylene (LLDPE) over HZSM-5. The apparent activation energies (Em) of catalytic pyrolysis (CP) of TBSD, and LLDPE were 187 and 147 kJ mol−1, respectively, from Kissinger–Akahira–Sunose (KAS) model. Those of catalytic co-pyrolysis (CCP) of blends TBP3:1, TBP1:1 and TBP1:3 were 163, 135 and 133 kJ mol−1, respectively. The CCP of TBP1:3 and TBP1:1 showed synergism between TBSD and LLDPE in terms of Em and TBP1:3 (TBSD: LLDPE 1:3 w/w) showed the highest synergism with the least Em. The CCP mechanism of samples with a higher fraction of TBSD was more complex, as depicted from Criado's master plot.

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  • Alam, Mahboob & Rammohan, Draksharapu & Peela, Nageswara Rao, 2021. "Catalytic co-pyrolysis of wet-torrefied bamboo sawdust and plastic over the zeolite H-ZSM-5: Synergistic effects and kinetics," Renewable Energy, Elsevier, vol. 178(C), pages 608-619.
    • Handle: RePEc:eee:renene:v:178:y:2021:i:c:p:608-619
    DOI: 10.1016/j.renene.2021.06.109
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    References listed on IDEAS

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    1. Safar, Michal & Lin, Bo-Jhih & Chen, Wei-Hsin & Langauer, David & Chang, Jo-Shu & Raclavska, H. & Pétrissans, Anélie & Rousset, Patrick & Pétrissans, Mathieu, 2019. "Catalytic effects of potassium on biomass pyrolysis, combustion and torrefaction," Applied Energy, Elsevier, vol. 235(C), pages 346-355.
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    5. Alam, Mahboob & Bhavanam, Anjireddy & Jana, Ashirbad & Viroja, Jaimin kumar S. & Peela, Nageswara Rao, 2020. "Co-pyrolysis of bamboo sawdust and plastic: Synergistic effects and kinetics," Renewable Energy, Elsevier, vol. 149(C), pages 1133-1145.
    6. Liu, Xuan & Burra, Kiran Raj G. & Wang, Zhiwei & Li, Jinhu & Che, Defu & Gupta, Ashwani K., 2021. "Towards enhanced understanding of synergistic effects in co-pyrolysis of pinewood and polycarbonate," Applied Energy, Elsevier, vol. 289(C).
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    Cited by:

    1. Rammohan, Draksharapu & Kishore, Nanda & Uppaluri, Ramagopal V.S., 2022. "Pyro–catalytic co–pyrolysis of Delonix regia and butyl rubber tube: Kinetic modelling and thermodynamic insights," Renewable Energy, Elsevier, vol. 201(P1), pages 194-203.
    2. Chakraborty, Sourabh & Mohanty, Kaustubha & Vinu, Ravikrishnan, 2024. "Co-pyrolysis of bamboo biomass with polypropylene coverall: Distributed activation energy modeling and pyrolysate composition studies," Renewable Energy, Elsevier, vol. 220(C).
    3. Tariq, Rumaisa & Mohd Zaifullizan, Yasmin & Salema, Arshad Adam & Abdulatif, Atiqah & Ken, Loke Shun, 2022. "Co-pyrolysis and co-combustion of orange peel and biomass blends: Kinetics, thermodynamic, and ANN application," Renewable Energy, Elsevier, vol. 198(C), pages 399-414.

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