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Effects of mixture of CO2 /CH4 as pyrolysis atmosphere on pine wood pyrolysis products

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Listed:
  • Xu, Bang
  • Argyle, Morris D.
  • Shi, Xiufeng
  • Goroncy, Alexander K.
  • Rony, Asif Hasan
  • Tan, Gang
  • Fan, Maohong

Abstract

The aim of the present work is to provide a preliminary support and research foundation for developing integrated technology of methane dry reforming and pine wood pyrolysis to produce high value chemicals and fuels. The chemical properties of bio-oil produced by pine wood pyrolysis under traditional N2, H2, CO2, CH4 atmospheres and mixtures of CH4 and CO2 were investigated. Experimental studies were conducted in a fixed bed reactor at a temperature of 500 °C. The results show that pine wood pyrolysis under mixtures of methane and CO2 can promote bio-oil production (0.98% increase) compared with traditional pyrolysis (under N2). GC-MS results show that the contents of phenols and sugars in bio-oil decreased, while the amount of alcohols, aldehydes, ketones, and furans increased. NMR spectroscopy provides additional support of the results. Results indicate that bio-oil can be used as a source of value-added chemicals. High proportions of CO were obtained in the gas products from pine wood pyrolysis under CH4 and mixtures of CH4 and CO2. Finally, a possible reaction pathway of pine wood pyrolysis under mixtures of methane and CO2 is proposed. Methane bi-reforming with CO2 and steam from pine wood pyrolysis could promote the production of high value oxygen-containing chemicals during pine wood pyrolysis under mixtures of CH4 and CO2.

Suggested Citation

  • Xu, Bang & Argyle, Morris D. & Shi, Xiufeng & Goroncy, Alexander K. & Rony, Asif Hasan & Tan, Gang & Fan, Maohong, 2020. "Effects of mixture of CO2 /CH4 as pyrolysis atmosphere on pine wood pyrolysis products," Renewable Energy, Elsevier, vol. 162(C), pages 1243-1254.
    • Handle: RePEc:eee:renene:v:162:y:2020:i:c:p:1243-1254
    DOI: 10.1016/j.renene.2020.08.069
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    References listed on IDEAS

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    1. Sun, Zhao & Chen, Shiyi & Russell, Christopher K. & Hu, Jun & Rony, Asif H. & Tan, Gang & Chen, Aimin & Duan, Lunbo & Boman, John & Tang, Jinke & Chien, TeYu & Fan, Maohong & Xiang, Wenguo, 2018. "Improvement of H2-rich gas production with tar abatement from pine wood conversion over bi-functional Ca2Fe2O5 catalyst: Investigation of inner-looping redox reaction and promoting mechanisms," Applied Energy, Elsevier, vol. 212(C), pages 931-943.
    2. Kan, Tao & Strezov, Vladimir & Evans, Tim J., 2016. "Lignocellulosic biomass pyrolysis: A review of product properties and effects of pyrolysis parameters," Renewable and Sustainable Energy Reviews, Elsevier, vol. 57(C), pages 1126-1140.
    3. Akhtar, Javaid & Saidina Amin, NorAishah, 2012. "A review on operating parameters for optimum liquid oil yield in biomass pyrolysis," Renewable and Sustainable Energy Reviews, Elsevier, vol. 16(7), pages 5101-5109.
    4. Tang, Mingchen & Xu, Long & Fan, Maohong, 2015. "Progress in oxygen carrier development of methane-based chemical-looping reforming: A review," Applied Energy, Elsevier, vol. 151(C), pages 143-156.
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    1. Xu, Donghua & Lin, Junhao & Ma, Rui & Fang, Lin & Sun, Shichang & Luo, Juan, 2022. "Microwave pyrolysis of biomass for low-oxygen bio-oil: Mechanisms of CO2-assisted in-situ deoxygenation," Renewable Energy, Elsevier, vol. 184(C), pages 124-133.
    2. Thoharudin, & Hsiau, Shu-San & Chen, Yi-Shun & Yang, Shouyin, 2022. "Numerical modeling of biomass fast pyrolysis by using an improved comprehensive reaction scheme for energy analysis," Renewable Energy, Elsevier, vol. 181(C), pages 355-364.

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