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Promoting hydrogen-rich syngas production through catalytic cracking of rape straw using Ni-Fe/PAC-γAl2O3 catalyst

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  • Shi, Xunwang
  • Zhang, Kaidi
  • Cheng, Qunpeng
  • Song, Guangsen
  • Fan, Guozhi
  • Li, Jianfen

Abstract

A catalyst loaded Ni-Fe using powder active carbon (PAC) and γ-Al2O3 as the support was prepared for hydrogen-rich syngas production from rape straw pyrolysis in a two-stage fixed reactor. EDX (Energy-dispersive X-ray spectroscopy), SEM (Scanning electron microscope) and N2 isothermal adsorption-desorption were used to characterize the catalysts. The results showed that the support of PAC-γAl2O3 was uniform with large specific surface area. The metals loaded on the support were well dispersed. The performance of Ni-Fe/PAC-γAl2O3 catalysts compared with single support catalyst NiO-Fe2O3/γAl2O3 (NFA) and NiO-Fe2O3/PAC (NFP) was studied. The results showed that the Ni-Fe/PAC-γAl2O3 catalysts showed a good catalytic activity which obviously enhanced the H2 gas yield to 54.23 g/kg Rape straw and reduced the tar yield to 4.06 g/kg. Meanwhile, Ni-Fe/PAC-γAl2O3 catalysts had a stronger ability to prevent the deactivation to keep a longtime stability than the single carrier catalyst.

Suggested Citation

  • Shi, Xunwang & Zhang, Kaidi & Cheng, Qunpeng & Song, Guangsen & Fan, Guozhi & Li, Jianfen, 2019. "Promoting hydrogen-rich syngas production through catalytic cracking of rape straw using Ni-Fe/PAC-γAl2O3 catalyst," Renewable Energy, Elsevier, vol. 140(C), pages 32-38.
    • Handle: RePEc:eee:renene:v:140:y:2019:i:c:p:32-38
    DOI: 10.1016/j.renene.2019.03.060
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    2. Pei, Haipeng & Jin, Baosheng & Huang, Yaji, 2020. "Quantitative analysis of mass and energy flow in rice straw gasification based on mass and carbon balance," Renewable Energy, Elsevier, vol. 161(C), pages 846-857.

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