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Degradation issues of PEM electrolysis MEAs

Author

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  • Siracusano, S.
  • Van Dijk, N.
  • Backhouse, R.
  • Merlo, L.
  • Baglio, V.
  • Aricò, A.S.

Abstract

One of main challenge of proton exchange membrane (PEM) water electrolysis is the achievement of a long-term durability exceeding 100 khours. Accordingly, degradation mechanisms of membrane electrode assemblies (MEAs) and stack components of PEM electrolysers deserve large attention. An important objective of the EU ELECTROHYPEM project was to develop components for PEM electrolysers with enhanced activity and stability in order to reduce stack and system costs and to improve efficiency, performance and durability. The focus of the project was concerning mainly with electrocatalysts and membranes development and validation of these materials in a PEM electrolyser. In this work, a first set of MEAs, used for 3500–5700 h in a PEM electrolyser, was investigated using electrochemical and physico-chemical techniques. The goal was to individuate key degradation issues and to provide a reliable estimation of the MEA endurance under real life operation. Specific approaches to mitigate the degradation mechanisms are discussed.

Suggested Citation

  • Siracusano, S. & Van Dijk, N. & Backhouse, R. & Merlo, L. & Baglio, V. & Aricò, A.S., 2018. "Degradation issues of PEM electrolysis MEAs," Renewable Energy, Elsevier, vol. 123(C), pages 52-57.
    • Handle: RePEc:eee:renene:v:123:y:2018:i:c:p:52-57
    DOI: 10.1016/j.renene.2018.02.024
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    References listed on IDEAS

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    1. Siracusano, Stefania & Baglio, Vincenzo & Van Dijk, Nicholas & Merlo, Luca & Aricò, Antonino Salvatore, 2017. "Enhanced performance and durability of low catalyst loading PEM water electrolyser based on a short-side chain perfluorosulfonic ionomer," Applied Energy, Elsevier, vol. 192(C), pages 477-489.
    2. Götz, Manuel & Lefebvre, Jonathan & Mörs, Friedemann & McDaniel Koch, Amy & Graf, Frank & Bajohr, Siegfried & Reimert, Rainer & Kolb, Thomas, 2016. "Renewable Power-to-Gas: A technological and economic review," Renewable Energy, Elsevier, vol. 85(C), pages 1371-1390.
    3. Mesfun, Sennai & Sanchez, Daniel L. & Leduc, Sylvain & Wetterlund, Elisabeth & Lundgren, Joakim & Biberacher, Markus & Kraxner, Florian, 2017. "Power-to-gas and power-to-liquid for managing renewable electricity intermittency in the Alpine Region," Renewable Energy, Elsevier, vol. 107(C), pages 361-372.
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    Cited by:

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    2. Pantò, Fabiola & Siracusano, Stefania & Briguglio, Nicola & Aricò, Antonino Salvatore, 2020. "Durability of a recombination catalyst-based membrane-electrode assembly for electrolysis operation at high current density," Applied Energy, Elsevier, vol. 279(C).
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    5. Hughes, J.P. & Clipsham, J. & Chavushoglu, H. & Rowley-Neale, S.J. & Banks, C.E., 2021. "Polymer electrolyte electrolysis: A review of the activity and stability of non-precious metal hydrogen evolution reaction and oxygen evolution reaction catalysts," Renewable and Sustainable Energy Reviews, Elsevier, vol. 139(C).
    6. Papakonstantinou, Georgios & Algara-Siller, Gerardo & Teschner, Detre & Vidaković-Koch, Tanja & Schlögl, Robert & Sundmacher, Kai, 2020. "Degradation study of a proton exchange membrane water electrolyzer under dynamic operation conditions," Applied Energy, Elsevier, vol. 280(C).
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