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Development of the direct solar photocatalytic water splitting system for hydrogen production in Northwest China: Design and evaluation of photoreactor

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  • Cao, Fei
  • Wei, Qingyu
  • Liu, Huan
  • Lu, Na
  • Zhao, Liang
  • Guo, Liejin

Abstract

A novel CPC reactor for solar photocatalytic hydrogen production was designed and evaluated in the present study. Two operation models, namely the natural circulation model and the gas disturbance model, are proposed and illustrated from the viewpoints of thermodynamics and hydrodynamics. The designed photoreactor is operated under natural circulation for most of the time, with high pressure gas disturbing the sedimentary photocatalysts from time to time. The CPC parameters are designed according to the local meteorological conditions. The reactor performance such as the radiation distribution on the absorber tube, the absorbed solar irradiation, the critical flow rates and the hydrogen productivity are estimated and analyzed. An east-west orientated, north-south angle adjustable and truncated CPC with the concentration ratio of 4.12 is designed for the photoreactor. The required limiting settling velocity is much larger than the natural circulation velocity, which validates the necessity of gas disturbance. The estimated results show that the ideal mean hydrogen productivities are 2.9 L/h and 4.0 L/h in a typical spring and summer week respectively, with the photocatalyst being Cd0.5Zn0.5S.

Suggested Citation

  • Cao, Fei & Wei, Qingyu & Liu, Huan & Lu, Na & Zhao, Liang & Guo, Liejin, 2018. "Development of the direct solar photocatalytic water splitting system for hydrogen production in Northwest China: Design and evaluation of photoreactor," Renewable Energy, Elsevier, vol. 121(C), pages 153-163.
    • Handle: RePEc:eee:renene:v:121:y:2018:i:c:p:153-163
    DOI: 10.1016/j.renene.2018.01.016
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    References listed on IDEAS

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    1. Ahmad, H. & Kamarudin, S.K. & Minggu, L.J. & Kassim, M., 2015. "Hydrogen from photo-catalytic water splitting process: A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 43(C), pages 599-610.
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    1. Ruiz-Aguirre, A. & Villachica-Llamosas, J.G. & Polo-López, M.I. & Cabrera-Reina, A. & Colón, G. & Peral, J. & Malato, S., 2022. "Assessment of pilot-plant scale solar photocatalytic hydrogen generation with multiple approaches: Valorization, water decontamination and disinfection," Energy, Elsevier, vol. 260(C).
    2. Fei Cao & Jiarui Pang & Xianzhe Gu & Miaomiao Wang & Yanqin Shangguan, 2023. "Performance Simulation of Solar Trough Concentrators: Optical and Thermal Comparisons," Energies, MDPI, vol. 16(4), pages 1-18, February.
    3. Ren, Ting & Ma, Tianzeng & Liu, Sha & Li, Xin, 2022. "Bi-level optimization for the energy conversion efficiency improvement in a photocatalytic-hydrogen-production system," Energy, Elsevier, vol. 253(C).
    4. Chen, Zhang & Yiliang, Xie & Hongxia, Zhang & Yujie, Gu & Xiongwen, Zhang, 2023. "Optimal design and performance assessment for a solar powered electricity, heating and hydrogen integrated energy system," Energy, Elsevier, vol. 262(PA).
    5. Ma, Jing & Dai, Jianan & Duan, Yinli & Zhang, Jiajia & Qiang, Liangsheng & Xue, Juanqin, 2020. "Fabrication of PANI-TiO2/rGO hybrid composites for enhanced photocatalysis of pollutant removal and hydrogen production," Renewable Energy, Elsevier, vol. 156(C), pages 1008-1018.
    6. Marino, C. & Nucara, A. & Panzera, M.F. & Pietrafesa, M. & Varano, V., 2019. "Energetic and economic analysis of a stand alone photovoltaic system with hydrogen storage," Renewable Energy, Elsevier, vol. 142(C), pages 316-329.

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