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Syngas production by catalytic steam gasification of municipal solid waste in fixed-bed reactor

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  • Luo, Siyi
  • Zhou, Yangmin
  • Yi, Chuijie

Abstract

The catalytic steam gasification of municipal solid waste for syngas production was conducted in a lab-scale fixed-bed reactor. The influence of the reactor temperature, steam to carbon ratio (S/C) and catalyst type (NiO/γ-Al2O3 or calcined dolomite) on the gas yield, gas composition, H2/CO molar ratio and carbon conversion efficiency were investigated. The results indicated that increasing reactor temperature resulted in greater gas production in the initial pyrolysis and improved endothermic reactions (gasification of char, catalytic cracking and reforming of tar), which resulted in the increase of syngas yield. Compared with MSW catalytic pyrolysis, the introduction of steam leads to more tar and char participating in steam gasification, which resulted in a rapid increase of syngas yield and carbon conversion efficiency. NiO/γ-Al2O3 catalyst revealed better catalytic performance for the cracking of tar than calcined dolomite. The highest H2 content (54.22%) and gas yield (1.75N m3/kg) were achieved at 900°C, S/C being 2.41 with NiO/γ-Al2O3 as catalyst.

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  • Luo, Siyi & Zhou, Yangmin & Yi, Chuijie, 2012. "Syngas production by catalytic steam gasification of municipal solid waste in fixed-bed reactor," Energy, Elsevier, vol. 44(1), pages 391-395.
    • Handle: RePEc:eee:energy:v:44:y:2012:i:1:p:391-395
    DOI: 10.1016/j.energy.2012.06.016
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    3. La Villetta, M. & Costa, M. & Massarotti, N., 2017. "Modelling approaches to biomass gasification: A review with emphasis on the stoichiometric method," Renewable and Sustainable Energy Reviews, Elsevier, vol. 74(C), pages 71-88.
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    6. Hu, Mian & Guo, Dabin & Ma, Caifeng & Hu, Zhiquan & Zhang, Beiping & Xiao, Bo & Luo, Siyi & Wang, Jingbo, 2015. "Hydrogen-rich gas production by the gasification of wet MSW (municipal solid waste) coupled with carbon dioxide capture," Energy, Elsevier, vol. 90(P1), pages 857-863.
    7. Ghulamullah Maitlo & Imran Ali & Kashif Hussain Mangi & Safdar Ali & Hubdar Ali Maitlo & Imran Nazir Unar & Abdul Majeed Pirzada, 2022. "Thermochemical Conversion of Biomass for Syngas Production: Current Status and Future Trends," Sustainability, MDPI, vol. 14(5), pages 1-30, February.
    8. Cho, Min-Hwan & Mun, Tae-Young & Choi, Young-Kon & Kim, Joo-Sik, 2014. "Two-stage air gasification of mixed plastic waste: Olivine as the bed material and effects of various additives and a nickel-plated distributor on the tar removal," Energy, Elsevier, vol. 70(C), pages 128-134.
    9. Shane, Agabu & Gheewala, Shabbir H. & Fungtammasan, Bundit & Silalertruksa, Thapat & Bonnet, Sébastien & Phiri, Seveliano, 2016. "Bioenergy resource assessment for Zambia," Renewable and Sustainable Energy Reviews, Elsevier, vol. 53(C), pages 93-104.
    10. Chiang, Kung-Yuh & Lu, Cheng-Han & Lin, Ming-Hui & Chien, Kuang-Li, 2013. "Reducing tar yield in gasification of paper-reject sludge by using a hot-gas cleaning system," Energy, Elsevier, vol. 50(C), pages 47-53.
    11. Usmani, Zeba & Sharma, Minaxi & Karpichev, Yevgen & Pandey, Ashok & Chander Kuhad, Ramesh & Bhat, Rajeev & Punia, Rajesh & Aghbashlo, Mortaza & Tabatabaei, Meisam & Gupta, Vijai Kumar, 2020. "Advancement in valorization technologies to improve utilization of bio-based waste in bioeconomy context," Renewable and Sustainable Energy Reviews, Elsevier, vol. 131(C).
    12. Thuan Duc Mai & Tamás Koós & Emese Sebe & Zoltán Siménfalvi & András Arnold Kállay, 2023. "Efficiency Enhancement of the Single Line Multi-Stage Gasification of Hungarian Low-Rank Coal: Effects of Gasification Temperature and Steam/Carbon (S/C) Ratio," Energies, MDPI, vol. 16(11), pages 1-16, May.
    13. Patrik Šuhaj & Jakub Husár & Juma Haydary, 2020. "Gasification of RDF and Its Components with Tire Pyrolysis Char as Tar-Cracking Catalyst," Sustainability, MDPI, vol. 12(16), pages 1-14, August.
    14. Liu, Hui & Cattolica, Robert J. & Seiser, Reinhard & Liao, Chang-hsien, 2015. "Three-dimensional full-loop simulation of a dual fluidized-bed biomass gasifier," Applied Energy, Elsevier, vol. 160(C), pages 489-501.
    15. Ascher, Simon & Sloan, William & Watson, Ian & You, Siming, 2022. "A comprehensive artificial neural network model for gasification process prediction," Applied Energy, Elsevier, vol. 320(C).
    16. Déparrois, N. & Singh, P. & Burra, K.G. & Gupta, A.K., 2019. "Syngas production from co-pyrolysis and co-gasification of polystyrene and paper with CO2," Applied Energy, Elsevier, vol. 246(C), pages 1-10.
    17. Jia, Dongqing & Li, Xingmei & Gong, Xu & Lv, Xiaoyan & Shen, Zhong, 2024. "Bi-level strategic bidding model of novel virtual power plant aggregating waste gasification in integrated electricity and hydrogen markets," Applied Energy, Elsevier, vol. 357(C).
    18. Watson, Jamison & Zhang, Yuanhui & Si, Buchun & Chen, Wan-Ting & de Souza, Raquel, 2018. "Gasification of biowaste: A critical review and outlooks," Renewable and Sustainable Energy Reviews, Elsevier, vol. 83(C), pages 1-17.
    19. Benedikt, F. & Schmid, J.C. & Fuchs, J. & Mauerhofer, A.M. & Müller, S. & Hofbauer, H., 2018. "Fuel flexible gasification with an advanced 100 kW dual fluidized bed steam gasification pilot plant," Energy, Elsevier, vol. 164(C), pages 329-343.
    20. Król, Danuta & Poskrobko, Sławomir, 2016. "High-methane gasification of fuels from waste – Experimental identification," Energy, Elsevier, vol. 116(P1), pages 592-600.
    21. Song, Guohui & Xiao, Jun & Yan, Chao & Gu, Haiming & Zhao, Hao, 2022. "Quality of gaseous biofuels: Statistical assessment and guidance on production technologies," Renewable and Sustainable Energy Reviews, Elsevier, vol. 169(C).
    22. Włodzimierz Szczepaniak & Monika Zabłocka-Malicka & Rafał Wysokiński & Piotr Rutkowski, 2020. "Intensity of the Process Gas Emission from the Thermal Treatment of the 60–340 mm MSW Fraction under Steam," Sustainability, MDPI, vol. 12(19), pages 1-17, September.
    23. Mendiburu, Andrés Z. & Carvalho, João A. & Coronado, Christian J.R., 2014. "Thermochemical equilibrium modeling of biomass downdraft gasifier: Stoichiometric models," Energy, Elsevier, vol. 66(C), pages 189-201.
    24. Ranwei Ren & Haiming Wang & Changfu You, 2022. "Steam Gasification of Refuse-Derived Fuel with CaO Modification for Hydrogen-Rich Syngas Production," Energies, MDPI, vol. 15(21), pages 1-16, November.

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