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Spotlighting the boosted energy storage capacity of CoFe2O4/Graphene nanoribbons: A promising positive electrode material for high-energy-density asymmetric supercapacitor

Author

Listed:
  • Xia, Changlei
  • Ren, Tiyao
  • Darabi, Rozhin
  • Shabani-Nooshabadi, Mehdi
  • Jaromír Klemeš, Jiří
  • Karaman, Ceren
  • Karimi, Fatemeh
  • Wu, Yingji
  • Kamyab, Hesam
  • Vasseghian, Yasser
  • Chelliapan, Shreeshivadasan

Abstract

CoFe2O4/Graphene Nanoribbons (GNRs) nanocomposite was successfully fabricated and utilised as an electrode active material for high-energy supercapacitor cells. Thanks to the outstanding physicochemical features of a graphene nanoribbon with excellent electrical conductivity and the synergistic effect with cobalt ferrite, as well as the pseudocapacitive effect. The CoFe2O4/GNRs nanohybrid offered an exceptional specific capacitance of 922 F g−1 (415 C g−1) at 1.0 A g−1 in 3.0 M KOH electrolyte in a standard 3-electrode set-up. Additionally, the impressive supercapacitive performance metrics showed that the suggested electrode had a distinctive morphology and could be a candidate for capacitive energy storage systems. These metrics included good cycle stability and 87% capacitance retention at the end of the 10,000th CV cycle. Moreover, the asymmetric supercapacitor cell (ASC) was designed by assembling CoFe2O4/GNRs and activated carbon (AC). The resultant ASC provided an improved specific capacitance of 487.85 F g−1 (683 C g−1) at 1.0 A g−1. At this current density value, the energy density and the power density values were computed as to be 132.8 Wh.kg−1 and 632.39 W kg−1. The highest power density was discovered to be 6730.76 W kg−1 at 10.0 A g−1, whereas the energy density was determined as 8.75 Wh.kg−1 at this current density. The results of the work proved that CoFe2O4/GNRs nanohybrids are up-and-coming electrode active materials for advanced electrochemical energy storage and conversion technologies.

Suggested Citation

  • Xia, Changlei & Ren, Tiyao & Darabi, Rozhin & Shabani-Nooshabadi, Mehdi & Jaromír Klemeš, Jiří & Karaman, Ceren & Karimi, Fatemeh & Wu, Yingji & Kamyab, Hesam & Vasseghian, Yasser & Chelliapan, Shrees, 2023. "Spotlighting the boosted energy storage capacity of CoFe2O4/Graphene nanoribbons: A promising positive electrode material for high-energy-density asymmetric supercapacitor," Energy, Elsevier, vol. 270(C).
    • Handle: RePEc:eee:energy:v:270:y:2023:i:c:s0360544223003080
    DOI: 10.1016/j.energy.2023.126914
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    References listed on IDEAS

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    1. Olabi, Abdul Ghani & Abbas, Qaisar & Al Makky, Ahmed & Abdelkareem, Mohammad Ali, 2022. "Supercapacitors as next generation energy storage devices: Properties and applications," Energy, Elsevier, vol. 248(C).
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