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Improving inorganic perovskite photovoltaic performance via organic cation addition for efficient solar energy utilization

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Listed:
  • Lee, Dong-Gun
  • Pandey, Padmini
  • Parida, Bhaskar
  • Ryu, Jun
  • Cho, SungWon
  • Kim, Jae-Kwang
  • Kang, Dong-Won

Abstract

Organic cations help in executing better crystal growth of halide perovskites. Herein, we have realized improved all-inorganic cesium lead halide perovskite film quality with reduced pinholes and high crystallinity in phenylethylammonium (PEA+) assisted perovskite. Additionally, PEA+ cation acts as an additive to control intermediate perovskite phase and executes pure phase perovskite crystal growth as compared to MA+ and FA+ cations assisted perovskite films. X-ray photoelectron and UV–vis spectroscopy results revealed that adding PEA+ in the perovskite helps in almost uniform distribution of Br− ion after post-annealing process. Furthermore, depth profiling analysis reveals that PEA+ in the intermediate phase perovskite interacts more with the ZnO layer beneath perovskite, which helps in the fabrication of compact film. PEA+ sublimates after post-annealing treatment of 300 °C, as no evidence of PEA+ existence was found in characterizations for post-annealed perovskite films. This brings multiple benefits to inorganic mixed halide perovskite film formation. The best performing perovskite solar cell (PSC) exhibits a high conversion efficiency of 14.75% as well as enhanced stability of maintaining almost 83% of its initial efficiency for 400 h. Electrochemical impedance spectroscopy and space-charge-limited current results suggests reduced recombination loss and defect densities in PEA+ assisted PSC.

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  • Lee, Dong-Gun & Pandey, Padmini & Parida, Bhaskar & Ryu, Jun & Cho, SungWon & Kim, Jae-Kwang & Kang, Dong-Won, 2022. "Improving inorganic perovskite photovoltaic performance via organic cation addition for efficient solar energy utilization," Energy, Elsevier, vol. 257(C).
    • Handle: RePEc:eee:energy:v:257:y:2022:i:c:s0360544222015432
    DOI: 10.1016/j.energy.2022.124640
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