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Single-step silica nanofluid for improved carbon dioxide flow and reduced formation damage in porous media for carbon utilization

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  • Chaturvedi, Krishna Raghav
  • Trivedi, Japan
  • Sharma, Tushar

Abstract

Water-alternating gas (WAG) is affected by viscous fingering (with too much gas) and trapping of reservoir oil (with too much water) that can be addressed by advanced methods such as nanofluids, those not only increase CO2 capturing but also provide significant control on fingering. Therefore, this study reports the use of single-step silica nanofluids, of controllable nanoparticle (NP) size (below 100 nm), for improved CO2 flow and reduced formation damage in porous and permeable media. Polyacrylamide (PAM, 1000 ppm) was used as viscosifier and found favorable for enhanced dispersion stability (more than 2 months) in nanofluids. The parameters, such as amount of precursor (Tetraethylorthosilicate-TEOS) and catalyst (ammonium hydroxide-NH4OH), and amount of PAM were varied. Silica NPs were highly stable against agglomeration as reported by DLS, FTIR, TEM, SEM, and UV methods. Silica Nanofluids delayed CO2 breakthrough by retaining CO2 in sand-pack for longer duration than water/PAM. CO2 in presence of NPs made stable foam that was viscous and least mobile (than CO2) as confirmed by progressive increase in pressure while CO2 flow with water/PAM was unstable as pressure varied non-uniformly. This is of key importance for CO2 sequestration studies in porous reservoirs. Since NPs are solid substances, they can retain in sand-pack during nanofluid use for CO2 utilization strategies. NP retention was determined experimentally for different (1) sand-pack length, (2) flow rate, (3) NP concertation, and (4) test temperature. NP retention of only 8–12% of total injected amount was reported with Sand-pack length as the most influential variable.

Suggested Citation

  • Chaturvedi, Krishna Raghav & Trivedi, Japan & Sharma, Tushar, 2020. "Single-step silica nanofluid for improved carbon dioxide flow and reduced formation damage in porous media for carbon utilization," Energy, Elsevier, vol. 197(C).
    • Handle: RePEc:eee:energy:v:197:y:2020:i:c:s0360544220303832
    DOI: 10.1016/j.energy.2020.117276
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    Cited by:

    1. Pandey, Anjanay & Sinha, A.S.K. & Chaturvedi, Krishna Raghav & Sharma, Tushar, 2021. "Experimental investigation on effect of reservoir conditions on stability and rheology of carbon dioxide foams of nonionic surfactant and polymer: Implications of carbon geo-storage," Energy, Elsevier, vol. 235(C).
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    4. Shukla, Hari & Hembram, Bidesh Kumar & Vishal, Vikram & Trivedi, Japan & Srivastava, Vimal Chandra & Sharma, Tushar, 2024. "Surface modified single-step nanofluid for improved CO2 absorption and storage Prospects at pore-scale in micromodels: CO2 utilization for saline porous media," Energy, Elsevier, vol. 294(C).
    5. Liang, Fachun & He, Zhennan & Meng, Jia & Zhao, Jingwen & Yu, Chao, 2023. "Effects of microfracture parameters on adaptive pumping in fractured porous media: Pore-scale simulation," Energy, Elsevier, vol. 263(PC).
    6. Liu, Ang & Liu, Shimin, 2022. "Mechanical property alterations across coal matrix due to water-CO2 treatments: A micro-to-nano scale experimental study," Energy, Elsevier, vol. 248(C).
    7. Singh, Alpana & Sharma, Tushar, 2023. "Implications of sand mobilization on stability and rheological properties of carbon dioxide foam and its transport mechanism in unconsolidated sandstone," Energy, Elsevier, vol. 263(PB).
    8. Chaturvedi, Krishna Raghav & Narukulla, Ramesh & Amani, Mahmood & Sharma, Tushar, 2021. "Experimental investigations to evaluate surfactant role on absorption capacity of nanofluid for CO2 utilization in sustainable crude mobilization," Energy, Elsevier, vol. 225(C).
    9. Chen, Hao & Liu, Xiliang & Zhang, Chao & Tan, Xianhong & Yang, Ran & Yang, Shenglai & Yang, Jin, 2022. "Effects of miscible degree and pore scale on seepage characteristics of unconventional reservoirs fluids due to supercritical CO2 injection," Energy, Elsevier, vol. 239(PC).

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