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Process simulation of bio-dimethyl ether synthesis from tri-reforming of biogas: CO2 utilization

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  • Saebea, Dang
  • Authayanun, Suthida
  • Arpornwichanop, Amornchai

Abstract

The main contributions of this work are to study the suitable condition of biogas tri-reforming for DME synthesis process and to design the systems of the biogas tri-reforming process coupling with the DME synthesis. The effects of operating parameters in terms of boundary of carbon formation, steam to carbon ratio, and oxygen to carbon ratio on the biogas reforming process are firstly investigated. To utilize more CO2 in the system, CO2 produced from the DME synthesis is recycled to use in the biogas tri-reforming process. The H2 and CO yields of the tri-reforming process increase with increasing the CO2 recirculation ratio while the DME yield and system efficiency decrease. The requirement of gas cleaning unit for the DME synthesis coupling with the biogas tri-reforming system is also analyzed. The results indicate that the system with CO2 removal from syngas has more impact on the DME yield than that with H2O removal. On the contrary, the total CO2 emission intensity of the system with H2O removal is lower than that with CO2 removal. When comparing all cases, the system with both H2O and CO2 removals achieves the highest DME yield and system efficiency.

Suggested Citation

  • Saebea, Dang & Authayanun, Suthida & Arpornwichanop, Amornchai, 2019. "Process simulation of bio-dimethyl ether synthesis from tri-reforming of biogas: CO2 utilization," Energy, Elsevier, vol. 175(C), pages 36-45.
    • Handle: RePEc:eee:energy:v:175:y:2019:i:c:p:36-45
    DOI: 10.1016/j.energy.2019.03.062
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    References listed on IDEAS

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    Cited by:

    1. Yang, Qingchun & Xu, Simin & Zhang, Jinliang & Liu, Chenglin & Zhang, Dawei & Zhou, Huairong & Mei, Shumei & Gao, Minglin & Liu, Hongyan, 2021. "Thermodynamic and techno-economic analyses of a novel integrated process of coal gasification and methane tri-reforming to ethylene glycol with low carbon emission and high efficiency," Energy, Elsevier, vol. 229(C).
    2. Gao, Ruxing & Wang, Lei & Zhang, Leiyu & Zhang, Chundong & Jun, Ki-Won & Kim, Seok Ki & Zhao, Tiansheng & Wan, Hui & Guan, Guofeng & Zhu, Yuezhao, 2023. "A multi-criteria sustainability assessment and decision-making framework for DME synthesis via CO2 hydrogenation," Energy, Elsevier, vol. 275(C).
    3. Nakyai, Teeranun & Patcharavorachot, Yaneeporn & Arpornwichanop, Amornchai & Saebea, Dang, 2020. "Comparative exergoeconomic analysis of indirect and direct bio-dimethyl ether syntheses based on air-steam biomass gasification with CO2 utilization," Energy, Elsevier, vol. 209(C).
    4. Su, Bosheng & Han, Wei & He, Hongzhou & Jin, Hongguang & Chen, Zhijie & Zheng, Jieqing & Yang, Shaohui & Zhang, Xiaodong, 2020. "Using moderate carbon dioxide separation to improve the performance of solar-driven biogas reforming process," Applied Energy, Elsevier, vol. 279(C).
    5. Lim, Dongjun & Lee, Boreum & Lee, Hyunjun & Byun, Manhee & Lim, Hankwon, 2022. "Projected cost analysis of hybrid methanol production from tri-reforming of methane integrated with various water electrolysis systems: Technical and economic assessment," Renewable and Sustainable Energy Reviews, Elsevier, vol. 155(C).
    6. Kim, Dongin & Han, Jeehoon, 2020. "Techno-economic and climate impact analysis of carbon utilization process for methanol production from blast furnace gas over Cu/ZnO/Al2O3 catalyst," Energy, Elsevier, vol. 198(C).

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