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Pyrolysis and gasification kinetics of Jordanian oil-shales

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  • Jaber, J. O.
  • Probert, S. D.

Abstract

Two Jordanian oil-shale samples have been pyrolysed and gasified, non-isothermally, using a thermogravimetric analyser. The controlling parameters studied were the final temperature and influence of particle size as well as the heating rate employed during the process of thermal degradation of the oil-shale sample. The integral method was used in the analysis of weight-loss data to determine the pyrolysis and gasification kinetics. Within experimental error, a slightly greater weight loss occurred during the devolitlization phase when carbon dioxide was used instead of nitrogen to purge the system. The magnitude of the weight loss was dependent on the final temperature, as well as, to a lesser extent, on the heating rate employed. Increasing the latter resulted in the reaction ensuing at higher temperatures. Gasification and pyrolysis of the investigated shales complied with first-order kinetics: the activation energy and temperature at which the maximum reactivity rate occurred decreased slightly as the shale-particle size was reduced.

Suggested Citation

  • Jaber, J. O. & Probert, S. D., 1999. "Pyrolysis and gasification kinetics of Jordanian oil-shales," Applied Energy, Elsevier, vol. 63(4), pages 269-286, August.
    • Handle: RePEc:eee:appene:v:63:y:1999:i:4:p:269-286
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    References listed on IDEAS

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    1. Jaber, J. O. & Probert, S. D. & Williams, P. T., 1998. "Gaseous fuels (derived from oil shale) for heavy-duty gas turbines and combined-cycle power generators," Applied Energy, Elsevier, vol. 60(1), pages 1-20, May.
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    Cited by:

    1. Niu, Shengli & Han, Kuihua & Lu, Chunmei & Sun, Rongyue, 2010. "Thermogravimetric analysis of the relationship among calcium magnesium acetate, calcium acetate and magnesium acetate," Applied Energy, Elsevier, vol. 87(7), pages 2237-2242, July.
    2. Zhang, Yuming & Yu, Deping & Li, Wangliang & Gao, Shiqiu & Xu, Guangwen & Zhou, Huaqun & Chen, Jing, 2013. "Fundamental study of cracking gasification process for comprehensive utilization of vacuum residue," Applied Energy, Elsevier, vol. 112(C), pages 1318-1325.
    3. Al-Ayed, Omar S. & Matouq, M. & Anbar, Z. & Khaleel, Adnan M. & Abu-Nameh, Eyad, 2010. "Oil shale pyrolysis kinetics and variable activation energy principle," Applied Energy, Elsevier, vol. 87(4), pages 1269-1272, April.
    4. Ziad Abu El-Rub & Joanna Kujawa & Samer Al-Gharabli, 2020. "Pyrolysis Kinetic Parameters of Omari Oil Shale Using Thermogravimetric Analysis," Energies, MDPI, vol. 13(16), pages 1-13, August.
    5. Jun-Ho Jo & Seung-Soo Kim & Jae-Wook Shim & Ye-Eun Lee & Yeong-Seok Yoo, 2017. "Pyrolysis Characteristics and Kinetics of Food Wastes," Energies, MDPI, vol. 10(8), pages 1-13, August.
    6. Song, Xianzhi & Zhang, Chengkai & Shi, Yu & Li, Gensheng, 2019. "Production performance of oil shale in-situ conversion with multilateral wells," Energy, Elsevier, vol. 189(C).
    7. Wang, Qing & Zhao, Weizhen & Liu, Hongpeng & Jia, Chunxia & Li, Shaohua, 2011. "Interactions and kinetic analysis of oil shale semi-coke with cornstalk during co-combustion," Applied Energy, Elsevier, vol. 88(6), pages 2080-2087, June.
    8. Al-Ayed, Omar S. & Suliman, Mohd R. & Rahman, Nafi Abdel, 2010. "Kinetic modeling of liquid generation from oil shale in fixed bed retort," Applied Energy, Elsevier, vol. 87(7), pages 2273-2277, July.
    9. Jaber, J. O. & Al-Sarkhi, A. & Akash, B. A. & Mohsen, M. S., 2004. "Medium-range planning economics of future electrical-power generation options," Energy Policy, Elsevier, vol. 32(3), pages 357-366, February.

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