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A high-thermal-conductivity, high-durability phase-change composite using a carbon fibre sheet as a supporting matrix

Author

Listed:
  • Dong, Kaixin
  • Sheng, Nan
  • Zou, Deqiu
  • Wang, Cheng
  • Shimono, Kenji
  • Akiyama, Tomohiro
  • Nomura, Takahiro

Abstract

The practical application of low-temperature latent heat storage systems is limited by the low thermal conductivity of the phase-change material (PCM). We fabricated a phase-change composite (PCC) with high thermal conductivity (k) and a high thermal-conductivity-retention rate (k/k0) during thermal cycles to solve this problem. A new type of high-thermal-conductivity carbon fibre sheet (CFS) material was used to enhance the thermal conductivity of erythritol PCM. CFSs were stacked and compressed to form a 3D network structure of high thermal conductivity carbon fibre, then the porous structure was impregnated with liquid erythritol PCM in a vacuum. The thermal conductivity of the PCC was measured by using the laser flash method, and the microstructures were analysed by energy dispersive spectroscopy using a scanning electron microscope. Durability tests of 5 and 100 cycles, using differently shaped PCC samples, were conducted to investigate the thermal conductivity of the PCC. With the addition of 14.8 vol% CFS, the thermal conductivity of the PCC was improved to 24.4 W·m−1·K−1 (32.4 times higher than that of a pure PCM), and the thermal conductivity retention rate after 100 thermal cycles reached 89.4%. High-thermal-conductivity carbon fibre network structures with high connectivity were established in the PCC before the durability test and after 100 thermal cycles. The fabricated PCC exhibited a high thermal conductivity with less enhancement material and prolonged durability.

Suggested Citation

  • Dong, Kaixin & Sheng, Nan & Zou, Deqiu & Wang, Cheng & Shimono, Kenji & Akiyama, Tomohiro & Nomura, Takahiro, 2020. "A high-thermal-conductivity, high-durability phase-change composite using a carbon fibre sheet as a supporting matrix," Applied Energy, Elsevier, vol. 264(C).
    • Handle: RePEc:eee:appene:v:264:y:2020:i:c:s0306261920301975
    DOI: 10.1016/j.apenergy.2020.114685
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    4. Liu, Lu & Zhang, Xuelai & Xu, Xiaofeng & Lin, Xiangwei & Zhao, Yi & Zou, Lingeng & Wu, Yifan & Zheng, Huifan, 2021. "Development of low-temperature eutectic phase change material with expanded graphite for vaccine cold chain logistics," Renewable Energy, Elsevier, vol. 179(C), pages 2348-2358.
    5. Sheng Yang & Hong-Yi Shi & Jia Liu & Yang-Yan Lai & Özgür Bayer & Li-Wu Fan, 2024. "Supercooled erythritol for high-performance seasonal thermal energy storage," Nature Communications, Nature, vol. 15(1), pages 1-13, December.
    6. Li, Hongyang & Hu, Chengzhi & He, Yichuan & Tang, Dawei & Wang, Kuiming & Hu, Xianfeng, 2021. "Visualized-experimental investigation on the energy storage performance of PCM infiltrated in the metal foam with varying pore densities," Energy, Elsevier, vol. 237(C).

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